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Second-order optical nonlinear effects (second-harmonic and sum-frequency generation) are demonstrated in the telecommunication band by periodic poling of thin films of lithium niobate wafer-bonded on silicon substrates and rib-loaded with…

Spectroscopy of magnetization-induced second-harmonic generation (MSHG) is studied in magnetic Co$_{x}$Ag$_{1-x}$ granular films containing Co nanoparticles. A strong resonance of the magnetic contrast of the second-harmonic generation…

Adaptation and Self-Organizing Systems · Physics 2007-05-23 E. M. Kim , T. V. Murzina , A. F. Kravets , M. Inoue , G. Marowsky , O. A. Aktsipetrov

Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different…

On the basis of the Edward-Kornfeld formulation, we study the effective susceptibility of secondharmonic generation (SHG) in colloidal crystals, which are made of graded metallodielectric nanoparticles with an intrinsic SHG susceptibility…

Optics · Physics 2008-03-24 J. P. Huang , Y. C. Jian , C. Z. Fan , K. W. Yu

Extended defects with one dimensionality smaller than that of the host, such as 2D grain boundaries in 3D materials or 1D grain boundaries in 2D materials, can be particularly damaging since they directly impede the transport of charge,…

The random laser action with coherent feedback by second-harmonic generation (SHG) was experimentally demonstrated in this paper. Compared with the conventional random laser action based on photoluminescence effect, which needs strong…

Optics · Physics 2016-11-24 Yanqi Qiao , Yuanlin Zheng , Zengyan Cai , Xianfeng Chen

Second harmonic generation (SHG) microscopy is a valuable tool for optical microscopy. SHG microscopy is normally performed as a point scanning imaging method, which lacks phase information and is limited in spatial resolution by the…

Layered NbOX$_2$ ($X=\mathrm{Cl,\,Br,\,I}$), a member of the van der Waals ferroelectric family, exhibits intrinsic ferroelectricity and pronounced nonlinear optical responses, making it a promising candidate for integrated nanophotonics…

Symmetry governs the selection rules of light-matter interactions in crystalline materials, making symmetry manipulation a powerful tool for tuning their optical properties. Here, we demonstrate that the hot-electron injection from a…

Optics · Physics 2025-04-02 Zhizi Guan , Zhiwei Peng , David J. Srolovitz , Jacob Khurgin , Dangyuan Lei

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

Mesoscale and Nanoscale Physics · Physics 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

Optical harmonic generation on excitons is found in ZnSe/BeTe quantum wells with type-II band alignment. Two experimental approaches with spectrally-broad femtosecond laser pulses and spectrally-narrow picosecond pulses are used for…

Femtosecond time-resolved second harmonic generation (SHG) measurements were performed at room temperature on a single crystal of LuFe2O4, which has recently attracted attention as an electronic ferroelectric material in which polarization…

Materials Science · Physics 2024-05-13 H. Yu , Y. Fukada , G. Nishida , K. Takubo , T. Ishikawa , S. Koshihara , N. Ikeda , Y. Okimoto

We show that second harmonic generation can be enhanced by Fano resonant coupling of asymmetric plasmonic metal nanostructures. We develop a theoretical model examining the effects of electromagnetic interaction between two metal…

Systematic exploration of amorphous ABC heterostructures revealed that nanoscale morphological modifications markedly improved their artificial bulk second-order susceptibility. These amorphous birefringent heterostructures were fabricated…

Second-harmonic generation (SHG) is a fundamental tool in modern laser technology, enabling coherent frequency conversion to remote optical bands, serving as the basis for self-referenced femtosecond lasers and quadrature-squeezed light…

Optics · Physics 2025-12-10 Nikolai Kuznetsov , Zihan Li , Tobias J. Kippenberg

Nonlinear optics of semiconductors is an important field of fundamental and applied research, but surprisingly the role of excitons in the coherent processes leading to harmonics generation has remained essentially unexplored. Here we…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 M. Lafrentz , D. Brunne , A. V. Rodina , V. V. Pavlov , R. V. Pisarev , D. R. Yakovlev , A. Bakin , M. Bayer

Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…

The nonlinear process of second harmonic generation (SHG) in monolayer (1L) transition metal dichalcogenides (TMD), like $WS_2$, strongly depends on the polarization state of the excitation light. Combining plasmonic nanostructures with…

Optics · Physics 2021-10-08 Florian Spreyer , Claudia Ruppert , Philip Georgi , Thomas Zentgraf

Second harmonic generation (SHG) with a material of large transparency is an attractive way of generating coherent light sources at exotic wavelength range such as VUV, UV and visible light. It is of critical importance to improve nonlinear…

Since de discovery of graphene, the family of 2-dimensional materials has attracted much recent attention. In this work, the nonlinear optical properties of few-layer MoS2 two-dimensional crystals are studied using femtosecond laser pulses.…

Mesoscale and Nanoscale Physics · Physics 2013-06-20 Leandro M. Malard , Thonimar V. Alencar , Ana Paula M. Barboza , Kin Fai Mak , Ana M. de Paula