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We report observation of strong and anisotropic third harmonic generation (THG) in monolayer and multilayer ReS$_2$. The third-order nonlinear optical susceptibility of monolayer ReS$_2$, $\left| \chi^{(3)} \right|$ is on the order of…

Materials Science · Physics 2017-04-12 Qiannan Cui , Rodrigo A. Muniz , J. E. Sipe , Hui Zhao

Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…

Optics · Physics 2010-01-11 Pablo Molina , Mariola O Ramirez , Basilio J. Garcia , Luisa E. Bausa

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

We report the realization of Zinc Sulfide (ZnS) nanowaveguides and the experimental observation of second harmonic generation (SHG) in such structures, demonstrating their potential for integrated nonlinear photonics. ZnS thin films were…

Nonlinear optics, and particularly second harmonic generation (SHG), is increasingly used in many modern disciplines from material characterization in physical sciences to bio-imaging in medicine and optical signal processing in information…

Strongly Correlated Electrons · Physics 2021-03-17 G. van der Laan , S. W. Lovesey

Optical second harmonic generation (SHG) has been measured for the first time in reflection from the nanometer-thick films (6 to 40 nm) of the topological insulator Bi2Se3 using 1.51 eV (820 nm) Ti:Sapphire laser photons and revealed a…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

Optical second-harmonic generation (SHG) is studied for the confined geometry of a circular cylindrical waveguide or optical fiber. A model situation of high symmetry is considered where the material with nonlinear susceptibility is…

Optics · Physics 2013-09-17 B. U. Felderhof , G. Marowsky

Using symmetry arguments we show how optical second harmonic generation (SHG) can be used to detect antiferromagnetism at surfaces and in thin films. Based on the group theoretical analysis of the nonlinear electric susceptibility we…

Condensed Matter · Physics 2007-05-23 A. Daehn , W. Huebner , K. H. Bennemann

Twisting two dissimilar monolayer semiconductors induces structural chirality that remains largely elusive in linear optics but becomes remarkably pronounced in the nonlinear regime. Here we demonstrate that MoS2/WSe2 heterobilayers exhibit…

We investigate second harmonic generation (SHG) from hexagonal periodic arrays of triangular nano-holes of aluminum using a self-consistent methodology based on the hydrodynamics-Maxwell-Bloch approach. It is shown that angular polarization…

Optics · Physics 2021-07-07 Maxim Sukharev , Adi Salomon , Joseph Zyss

Nonlinear optics in whispering-gallery-mode (WGM) microresonators have attracted much attention. Owing to strong confinement of the light in a small volume, a WGM microresonator can dramatically boost the strength of light field, giving…

Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at…

Strongly enhanced third-harmonic generation (THG) by the topological localization of an edge mode in a Su-Schrieffer-Heeger (SSH) chain of silicon photonic crystal nanocavities is demonstrated. The edge mode of the nanocavity chain not only…

Optics · Physics 2021-05-21 Qingchen Yuan , Linpeng Gu , Liang Fang , Xuetao Gan , Zhigang Chen , Jianlin Zhao

Dielectric metasurfaces provide a unique platform for efficient harmonic generation and optical wavefront manipulation at the nanoscale. While several approaches are available for performing wavefront shaping, the one exploiting geometric…

Silicon-based nonlinear metasurfaces were implemented only with third-order nonlinearity due to the crystal centrosymmetry and the efficiencies are considerably low, which hinders their practical applications with low-power lasers. Here, we…

We have investigated second harmonic generation (SHG) from Ag-coated LiNbO3 (LN) core-shell nanocuboids and found that giant SHG can occur via deliberately designed double plasmonic resonances. By controlling the aspect ratio, we can tune…

Optics · Physics 2014-11-19 Ming-Liang Ren , Si-Yuan Liu , Ben-Li Wang , Bao-Qin Chen , Jiafang Li , Zhi-Yuan Li

Since the first observation of second harmonic generation (SHG), there have been extensive studies on this nonlinear phenomenon not only to clarify its physical origin but also to realize unconventional functionalities. Nonetheless, a…

It is generally argued that material classes with inversion symmetry do not produce bulk dipole related second harmonic generation (SHG). So, SHG is then either ascribed to surface effects or bulk related electric quadrupole or magnetic…

Breaking inversion symmetry in solids plays a central role in nonlinear optics because it can change material properties, such as producing even-order nonlinear optical (NLO) effects. Although a centrosymmetric diamond has been developed as…

Optics · Physics 2022-03-21 Aizitiaili Abulikemu , Yuta Kainuma , Toshu An , Muneaki Hase

Silicon photonics lacks a second-order nonlinear optical response in general because the typical constituent materials are centro-symmetric and lack inversion symmetry, which prohibits second-order nonlinear processes such as second…

Optics · Physics 2022-07-21 Xiyuan Lu , Gregory Moille , Ashutosh Rao , Daron Westly , Kartik Srinivasan