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We analyze the capillarity-driven thinning dynamics of entangled polymer solutions described by the Doi-Edwards-Marrucci-Grizzuti (DEMG) model and the Rolie-Poly (RP) model. Both models capture polymer reptation, finite rates of chain…

Soft Condensed Matter · Physics 2022-06-15 Jianyi Du , Hiroko Ohtani , Alper Kiziltas , Kevin Ellwood , Gareth H. McKinley

Polymers and rod-like colloids (PaRC) adopt a favorable orientation under sufficiently strong flows. However, how the flow kinematics affect the alignment of such nanostructures according to their extensibility remains unclear. By analysing…

The deformation and break-up of Newtonian/viscoelastic droplets are studied in confined shear flow. Our numerical approach is based on a combination of Lattice-Boltzmann models (LBM) and finite difference schemes, the former used to model…

Soft Condensed Matter · Physics 2016-11-15 A. Gupta , M. Sbragaglia

Encapsulation of chemicals using polymer membranes enables to control their transport and delivery for applications such as agrochemistry or detergency. To rationalize the design of polymer capsules, it is necessary to understand how the…

Soft Condensed Matter · Physics 2018-12-18 Corentin Tregouët , Thomas Salez , Mathilde Reyssat , Cécile Monteux

We extend classical Flory-Rehner theory for the expansion and compression of porous materials such as cross-linked polymer networks. The theory includes volume exclusion, affinity with the solvent, and finite stretching of the polymer…

Chemical Physics · Physics 2023-09-28 P. M. Biesheuvel , H. Fan , M. Elimelech

The surface of a thin liquid film with nonconstant curvature is unstable, as the Laplace pressure drives a flow mediated by viscosity. We present the results of experiments on one of the simplest variable curvature surfaces: a stepped…

Soft Condensed Matter · Physics 2015-06-11 Joshua D. McGraw , Thomas Salez , Oliver Bäumchen , Elie Raphaël , Kari Dalnoki-Veress

We study experimentally the interfacial instability between a layer of dilute polymer solution and water flowing in a thin capillary. The use of microfluidic devices allows us to observe and quantify in great detail the features of the…

Fluid Dynamics · Physics 2015-05-20 Oriane Bonhomme , Alexander Morozov , Jacques Leng , Annie Colin

We investigate the rheological characteristics of human blood plasma in shear and elongational flows. While we can confirm a Newtonian behavior in shear flow within experimental resolution, we find a viscoelastic behavior of blood plasma in…

Biological Physics · Physics 2013-02-19 M. Brust , C. Schaefer , L. Pan , M. Garcia , P. E. Arratia , C Wagner

In this study, we delve into the intricacies of elastoviscoplastic (EVP) fluids, particularly focusing on how polymer additives influence their extensional behavior. Our findings reveal that polymer additives significantly alter the…

Fluid Dynamics · Physics 2024-06-11 Mohamed S. Abdelgawad , Simon J. Haward , Amy Q. Shen , Marco E. Rosti

Liquid bridges form between particles during wet mixing with binders or by condensation due to ambient humidity. The consequences of capillary bridges can be quite drastic, creating macroscopic cohesion, as seen in sandcastles and in the…

Soft Condensed Matter · Physics 2026-04-10 Sreeram Rajesh , Riley S. Tinianov , Jooyeon Park , Alban Sauret

When injected through a contraction, high molecular weight polymer solutions exhibit a sharp increase of apparent viscosity which originates from stretching polymer chains above a critical extension rate. This chain stretching can also…

Fluid Dynamics · Physics 2020-04-22 Sandeep Garrepally , Stephane Jouenne , Peter D. Olmsted , Francois Lequeux

The velocity and friction properties of laminar pipe flow of a viscoelastic solution are bounded by the corresponding values for two Newtonian fluids, namely, the solvent and a fluid with a viscosity identical to the total viscosity of the…

Fluid Dynamics · Physics 2022-09-28 M Malik , Roland Bouffanais , Martin Skote

The extensional rheology of dilute suspensions of spheres in viscoelastic or polymeric liquids is studied computationally. At low polymer concentration (c) and Deborah number (De), a wake of highly stretched polymers forms downstream of the…

Fluid Dynamics · Physics 2025-09-10 Arjun Sharma , Donald L. Koch

Extensional flows of complex fluids are pivotal in industrial applications like spraying, atomisation, and microfluidic drop deposition. The Dripping-on-Substrate (DoS) technique is a conceptually simple, but dynamically-complex, probe of…

Fluid Dynamics · Physics 2024-04-11 Konstantinos Zinelis , Thomas Abadie , Gareth H. McKinley , Omar K. Matar

We study the linear instability with respect to necking of a filament of polymeric fluid undergoing uniaxial extension. Contrary to the widely discussed Considere criterion, we find the onset of instability to relate closely to the onset of…

Soft Condensed Matter · Physics 2015-05-30 Suzanne M. Fielding

The growing importance of microfluidic and nanofluidic devices to the study of biological processes has highlighted the need to better understand how confinement affects the behavior of polymers in flow. In this paper we explore one aspect…

Soft Condensed Matter · Physics 2015-06-05 Pinaki Bhattacharyya , Binny J. Cherayil

We present a simple method for accessing the elastic properties of microscopic deformable particles. This method is based on measuring the pressure-induced deformation of soft particles as they are forced through a tapered glass…

Soft Condensed Matter · Physics 2012-09-04 Hans M. Wyss , Thomas Franke , Elisa Mele , David A. Weitz

In Part I of this paper [Haward et al. submitted (2023)], we presented a new three-dimensional microfluidic device (the optimized uniaxial and biaxial extensional rheometer, OUBER) for generating near-homogeneous uniaxial and biaxial…

The non-equilibrium structural and dynamical properties of semiflexible polymers confined to two dimensions are investigated by molecular dynamics simulations. Three different scenarios are considered: The force-extension relation of…

Soft Condensed Matter · Physics 2013-01-08 A. Lamura , R. G. Winkler

Viscoelastic liquid transfer from one surface to another is a process that finds applications in many technologies, primarily in printing. Here, cylindrical shaped capillary bridges pinned between two parallel disks are considered.…

Fluid Dynamics · Physics 2025-05-13 Hrishikesh Pingulkar , Jorge Peixinho , Olivier Crumeyrolle