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Related papers: Internal consistency of multi-tier $GW$+EDMFT

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We perform a systematic {\it ab initio} study of the electronic structure of Sr(V,Mo,Mn)O$_3$ perovskites, using the parameter-free $GW$+EDMFT method. This approach self-consistently calculates effective interaction parameters, taking into…

Strongly Correlated Electrons · Physics 2020-02-26 Francesco Petocchi , Fredrik Nilsson , Ferdi Aryasetiawan , Philipp Werner

We discuss a parameter-free and computationally efficient ab initio simulation approach for moderately and strongly correlated materials, the multitier self-consistent $GW$+EDMFT method. This scheme treats different degrees of freedom, such…

Strongly Correlated Electrons · Physics 2017-10-02 Fredrik Nilsson , Lewin Boehnke , Philipp Werner , Ferdi Aryasetiawan

The reliable {\it ab-initio} description of strongly correlated materials is a long-sought capability in condensed matter physics. The $GW$+EDMFT method is a promising scheme, which provides a self-consistent description of correlations and…

Strongly Correlated Electrons · Physics 2021-12-08 Francesco Petocchi , Viktor Christiansson , Philipp Werner

Strongly correlated transition-metal perovskite oxides pose a fundamental challenge for electronic-structure theory and for large-scale, data-driven materials discovery. While DFT+DMFT provides a quantitatively accurate description of such…

Strongly Correlated Electrons · Physics 2026-05-19 Antik Sihi , Caden Ginter , Kristjan Haule , Subhasish Mandal

Theoretical studies of semiconductors and band insulators are usually based on variants of the $GW$ method without full self-consistency, like single-shot $G^0W^0$ or quasiparticle self-consistent $GW$. Fully self-consistent $GW$ provides a…

Strongly Correlated Electrons · Physics 2024-10-28 Viktor Christiansson , Francesco Petocchi , Philipp Werner

ComDMFT is a parallel computational package designed to study the electronic structure of correlated quantum materials from first principles. Our approach is based on the combination of first-principles methods and dynamical mean field…

Strongly Correlated Electrons · Physics 2024-11-18 Byungkyun Kang , Patrick Semon , Corey Melnick , Mancheon Han , Seongjun Mo , Hoonkyung Lee , Gabriel Kotliar , Sangkook Choi

We investigate the electronic structure of highly conducting perovskite SrMoO$_{3}$ using valence band photoemission spectroscopy and electronic structure calculations. Large intensity corresponding to coherent feature close to Fermi level…

Strongly Correlated Electrons · Physics 2023-01-24 Asif Ali , B. H. Reddy , Ravi Shankar Singh

We present the first dynamical implementation of the combined GW and dynamical mean field scheme ("GW+DMFT") for first principles calculations of the electronic properties of correlated materials. The application to the ternary transition…

Strongly Correlated Electrons · Physics 2012-12-19 Jan M. Tomczak , Michele Casula , Takashi Miyake , Ferdi Aryasetiawan , Silke Biermann

In this work, we use the thermodynamically consistent and conserving self-energy embedding theory (SEET) to study the spectra of the prototypical undistorted cubic perovskites SrVO$_3$ and SrMnO$_3$. In the strongly correlated metallic…

Strongly Correlated Electrons · Physics 2021-06-02 Chia-Nan Yeh , Sergei Iskakov , Dominika Zgid , Emanuel Gull

Phase retrieval from phaseless short-time Fourier transform (STFT) measurements is known to be inherently unstable when measurements are taken with respect to a single window. While an explicit inversion formula exists, it is useless in…

Functional Analysis · Mathematics 2025-06-19 Rima Alaifari , Yunan Yang

First-principles descriptions of correlated quantum materials require a simultaneous treatment of strong local many-body effects and nonlocal dynamical screening. We present an efficient fully self-consistent implementation of $GW$+EDMFT…

Strongly Correlated Electrons · Physics 2026-03-16 Chia-Nan Yeh , Francesco Petocchi , Alexander Hampel , Philipp Werner , Olivier Parcollet , Antoine Georges , Miguel Morales

The $GW$ approximation to many-body perturbation theory is a reliable tool for describing charged electronic excitations, and it has been successfully applied to a wide range of extended systems for several decades using a plane-wave basis.…

Materials Science · Physics 2019-10-23 Young-Moo Byun , Serdar Öğüt

The first-principles calculations have been performed to investigate the ground state properties of cubic scandium trifluoride (ScF$_3$) perovskite. Using modified hybrid exchange-correlation functionals within the density functional theory…

Materials Science · Physics 2012-11-27 P. Zhgun , D. Bocharov , S. Piskunov , A. Kuzmin , J. Purans

Multiple spin density waves and related vortex-type magnetic structures in the itinerant electron system with inversion symmetry have been investigated on the basis of the Hubbard model and the generalized Hartree-Fock approximation…

Strongly Correlated Electrons · Physics 2020-02-19 Yoshiro Kakehashi

The structure and ground state electronic structure of the recently synthesized SrPdO$_3$ perovskite [A. Galal {\em et al.}, J. Power Sources, {\bf 195}, 3806 (2010)] have been studied by means of screened hybrid functional and the GW…

Materials Science · Physics 2015-06-18 Jiangang He , Cesare Franchini

A versatile method for combining density functional theory (DFT) in the local density approximation (LDA) with dynamical mean-field theory (DMFT) is presented. Starting from a general basis-independent formulation, we use Wannier functions…

Strongly Correlated Electrons · Physics 2009-11-11 F. Lechermann , A. Georges , A. Poteryaev , S. Biermann , M. Posternak , A. Yamasaki , O. K. Andersen

We present a detailed calculation of the electronic structure of SrVO$_{3}$ based on the GW+DMFT method. We show that a proper inclusion of the frequency-dependent Hubbard U and the nonlocal self-energy via the GW approximation, as well as…

Strongly Correlated Electrons · Physics 2013-12-13 R. Sakuma , Ph. Werner , F. Aryasetiawan

Quantitative prediction of electronic properties in correlated materials requires simulations without empirical truncations and parameters. We present a method to achieve this goal through a new ab initio formulation of dynamical mean-field…

Strongly Correlated Electrons · Physics 2021-04-08 Tianyu Zhu , Garnet Kin-Lic Chan

The outstanding optoelectronics and photovoltaic properties of metal halide perovskites, including high carrier motilities, low carrier recombination rates, and the tunable spectral absorption range are attributed to the unique electronic…

Materials Science · Physics 2020-08-14 Shuxia Tao , Xi Cao , Peter Bobbert

We present the results of first-principles calculations on two possible terminations of the (001) surfaces of SrTiO3 (STO), BaTiO3 (BTO), and PbTiO3 (PTO) perovskite crystals. Atomic structure and the electronic configurations were…

Materials Science · Physics 2009-09-29 S. Piskunov , E. A. Kotomin , E. Heifets
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