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We consider pure dephasing of Bell states of electron spin qubits interacting with a sparse bath of nuclear spins. Using the newly developed two-qubit generalization of cluster correlation expansion method, we calculate the spin echo decay…

Mesoscale and Nanoscale Physics · Physics 2018-10-09 Damian Kwiatkowski , Łukasz Cywiński

The study of spin decoherence is often performed by assuming that spin-phonon interactions lead to relaxation at high temperatures, and spin-spin dipolar interactions instead contribute to pure dephasing at low temperatures. This has…

Quantum Physics · Physics 2026-02-17 Conor Ryan , Alessandro Lunghi

The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectroscopy and hampers the use of molecules for quantum information processing. At low…

Quantum Physics · Physics 2025-04-28 Conor Ryan , Valerio Briganti , Cathal Hogan , Mark O'Neill , Alessandro Lunghi

The central spin decoherence problem has been researched for over 50 years in the context of both nuclear magnetic resonance and electron spin resonance. Until recently, theoretical models have employed phenomenological stochastic…

Mesoscale and Nanoscale Physics · Physics 2012-08-03 Wayne M. Witzel , Malcolm S. Carroll , Lukasz Cywinski , S. Das Sarma

We theoretically study the longitudinal relaxation of a nitrogen-vacancy (NV) center surrounded by a 13C nuclear spin bath in diamond. By incorporating electron spin in the cluster, we generalize the cluster-correlation expansion (CCE) to…

Quantum Physics · Physics 2020-01-22 Zhi-Sheng Yang , Yan-Xiang Wang , Ming-Jie Tao , Wen Yang , Mei Zhang , Qing Ai , Fu-Guo Deng

We present a cluster expansion method for approximating quantum spin-bath dynamics in terms of a classical Gaussian stochastic process. The cluster expansion produces the two-point correlation function of the approximate classical bath,…

Mesoscale and Nanoscale Physics · Physics 2014-09-30 Wayne M. Witzel , Kevin Young , Sankar Das Sarma

The clock transitions (CTs) of central spins have long coherence times because their frequency fluctuations vanish in the linear order of external field noise (such as Overhauser fields from nuclear spin baths). Therefore, CTs are useful…

Quantum Physics · Physics 2021-01-04 Geng-Li Zhang , Wen-Long Ma , Ren-Bao Liu

The dominant source of decoherence for an electron spin in a quantum dot is the hyperfine interaction with the surrounding bath of nuclear spins. The decoherence process may be slowed down by subjecting the electron spin to suitable…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Wenxian Zhang , V. V. Dobrovitski , Lea F. Santos , Lorenza Viola , B. N. Harmon

We analyze the unitary time evolution of a conduction electron, described by a two-level system, interacting with two-level systems (spins) through a spin-spin interaction and prove that coherent spin states of the conduction electron are…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Marco Frasca

The problem of dipole-dipole decoherence of nuclear spins is considered for strongly entangled spin cluster. Our results show that its dynamics can be described as the decoherence due to interaction with a composite bath consisting of fully…

Quantum Physics · Physics 2007-05-23 A. Fedorov , L. Fedichkin

We study an extended central spin model with an isotropic nearest-neighbour spin-exchange interaction among the bath spins. The system is controllable by external magnetic fields applied on the central spin and the bath, respectively. We…

Strongly Correlated Electrons · Physics 2020-07-08 Pengcheng Lu , Hai-Long Shi , Like Cao , Xiao-Hui Wang , Tao Yang , Junpeng Cao , Wen-Li Yang

Decoherence of a center spin or qubit in a spin bath is essentially determined by the many-body bath evolution. We develop a cluster-correlation expansion (CCE) theory for the spin bath dynamics relevant to the qubit decoherence problem. A…

Mesoscale and Nanoscale Physics · Physics 2008-08-25 Wen Yang , Ren-bao Liu

Molecular spins offer promise in emerging quantum technologies such as quantum sensing and computing. At low temperatures, nuclear spin-spin interactions affect electron spin coherence lifetimes through pure dephasing. Nuclear-spin noise…

Quantum Physics · Physics 2026-05-06 Timothy J. Krogmeier , James Bradley , Anthony W. Schlimgen , Kade Head-Marsden

We consider the decoherence of a single localized electron spin due to its coupling to the lattice nuclear spin bath in a semiconductor quantum computer architecture. In the presence of an external magnetic field and at low temperatures,…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. M. Witzel , S. Das Sarma

We present a quantum solution to the electron spin decoherence by a nuclear pair-correlation method for the electron-nuclear spin dynamics under a strong magnetic field and a temperature high for the nuclear spins but low for the electron.…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Wang Yao , Ren-Bao Liu , L. J. Sham

The coherence time of an electron spin decohered by the nuclear spin environment in a quantum dot can be substantially increased by subjecting the electron to suitable dynamical decoupling sequences. We analyze the performance of high-level…

Mesoscale and Nanoscale Physics · Physics 2008-03-27 Wenxian Zhang , N. P. Konstantinidis , V. V. Dobrovitski , B. N. Harmon , Lea F. Santos , Lorenza Viola

We study a system of two electron spins each interacting with its small nuclear spin environment (NSE), which is a prototype system of two electron spin quantum dot (QD) qubits. We propose a way to counteract the decay of entanglement in…

Mesoscale and Nanoscale Physics · Physics 2021-10-27 Igor Bragar

We propose a new approach to simulate the decoherence of a central spin coupled to an interacting dissipative spin bath with cluster-correlation expansion techniques. We benchmark the approach on generic 1D and 2D spin baths and find…

Quantum Physics · Physics 2023-12-05 Mykyta Onizhuk , Yu-Xin Wang , Jonah Nagura , Aashish A. Clerk , Giulia Galli

In this work, we studied the relaxation dynamics of coherences of different order present in a system of two coupled nuclear spins. We used a previously designed model for intrinsic noise present in such systems which considers the Lindblad…

Quantum Physics · Physics 2022-07-12 Harpreet Singh , Arvind , Kavita Dorai

Spin decoherence poses a significant challenge in molecular magnets, with the nuclear spin bath serving as a prominent source. Intriguingly, spin qubits at the clock transition exhibit remarkable insensitivity to the surrounding nuclear…

Quantum Physics · Physics 2025-10-14 Xiao Chen , Haechan Park , Silas Hoffman , Shuanglong Liu , Hai-Ping Cheng
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