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We propose a quantum science platform utilizing the dipole-dipole coupling between donor-acceptor pairs (DAPs) in wide bandgap semiconductors to realize optically controllable, long-range interactions between defects in the solid state. We…

Quantum Physics · Physics 2024-01-31 Anil Bilgin , Ian Hammock , Jeremy Estes , Yu Jin , Hannes Bernien , Alexander High , Giulia Galli

The control of the charge state of nitrogen-vacancy (NV) centers in diamond is of primary importance for the stabilization of their quantum-optical properties, in applications ranging from quantum sensing to quantum computing. To this…

Nitrogen vacancy (NV) centers in diamond exhibit long spin coherence times, optical initialization, and optical spin readout under ambient conditions, making them excellent quantum sensors. However, the conventional scheme for charge state…

Nitrogen-Vacancy (NV) centers in diamond have been identified over the past few years as promising systems for a variety of applications, ranging from quantum information science to magnetic sensing. This relies on the unique optical and…

Quantum Physics · Physics 2018-12-19 I. Meirzada , Y. Hovav , S. A. Wolf , N. Bar-Gill

Although the spin properties of superficial shallow nitrogen-vacancy (NV) centers have been the subject of extensive scrutiny, considerably less attention has been devoted to studying the dynamics of NV charge conversion near the diamond…

Mesoscale and Nanoscale Physics · Physics 2018-07-03 Siddharth Dhomkar , Harishankar Jayakumar , Pablo R. Zangara , Carlos A. Meriles

Engineering shallow nitrogen-vacancy (NV) centers in diamond holds the key to unlocking new advances in nanoscale quantum sensing. We find that the creation of near-surface NVs through delta doping during diamond growth allows for tunable…

The charge degree of freedom in solid-state defects fundamentally underpins the electronic spin degree of freedom, a workhorse of quantum technologies. Here we study charge state properties of individual near-surface nitrogen-vacancy (NV)…

Mesoscale and Nanoscale Physics · Physics 2019-02-26 Dolev Bluvstein , Zhiran Zhang , Ania C. Bleszynski Jayich

Point defects in wide-bandgap semiconductors are emerging as versatile resources for nanoscale sensing and quantum information science but our understanding of the photo-ionization dynamics is presently incomplete. Here we use two-color…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 Siddharth Dhomkar , Pablo R. Zangara , Jacob Henshaw , Carlos A. Meriles

Control over the charge states of color centers in solids is necessary in order to fully utilize them in quantum technologies. However, the microscopic charge dynamics of deep defects in wide-bandgap semiconductors are complex, and much…

Mesoscale and Nanoscale Physics · Physics 2021-09-08 A. Gardill , I. Kemeny , M. C. Cambria , Y. Li , H. T. Dinani , A. Norambuena , J. R. Maze , V. Lordi , S. Kolkowitz

Creation of nitrogen-vacancy (NV) centers at the nanoscale surface region in diamond, while retaining their excellent spin and optical properties, is essential for applications in quantum technology. Here, we demonstrate the extension of…

Materials Science · Physics 2021-03-30 A. Watanabe , T. Nishikawa , H. Kato , M. Fujie , M. Fujiwara , T. Makino , S. Yamasaki , E. D. Herbschleb , N. Mizuochi

The negatively charged nitrogen-vacancy defect (NV)$^-$ in diamond has attracted much attention in recent years in qubit and biological applications. The negative charge is donated from nearby nitrogen donors that could limit or stem the…

Materials Science · Physics 2009-02-16 Adam Gali

Shallow, negatively-charged Nitrogen-Vacancy centers (NV-) in diamond have been proposed for high-sensitivity magnetometry and spin-polarization transfer applications. However, surface effects tend to favor and stabilize the less useful…

Mesoscale and Nanoscale Physics · Physics 2021-05-12 Federico Gorrini , Carla Dorigoni , Domingo Olivares-Postigo , Rakshyakar Giri , Pietro Aprà , Federico Picollo , Angelo Bifone

Charge control of color centers in semiconductors promises opportunities for novel forms of sensing and quantum information processing. Here, we articulate confocal fluorescence microscopy and magnetic resonance protocols to induce and…

Shallow nitrogen-vacancy (NV) centers in diamond offer unique opportunities for studying photochemical reactions at the single-molecule level, such as the photogeneration of radical pairs in proximal molecules. A prerequesite for such…

Spin-based applications of the negatively charged nitrogen-vacancy (NV) center in diamonds require efficient spin readout. One approach is the spin-to-charge conversion (SCC), relying on mapping the spin states onto the neutral (NV$^0$) and…

Thanks to its low or negative surface electron affinity and chemical inertness, diamond is attracting broad attention as a source material of solvated electrons produced by optical excitation of the solid-liquid interface. Unfortunately,…

Nitrogen-vacancy (NV) centers in diamond have attracted considerable interest in sensing of weak magnetic fields, such as those created by biological systems. Detecting such feeble signals requires near-surface NV centers, to reduce the…

Mesoscale and Nanoscale Physics · Physics 2019-05-01 R. Giri , C. Dorigoni , S. Tambalo , F. Gorrini , A. Bifone

Deep defects in wide band gap semiconductors have emerged as leading qubit candidates for realizing quantum sensing and information applications. Due to the spatial localization of the defect states, these deep defects can be considered as…

The nitrogen-vacancy (NV) centre in diamond is emerging as a promising platform for solid-state quantum information processing and nanoscale metrology. Of interest in these applications is the manipulation of the NV charge, which can be…

The charge state of a quantum point defect in a solid state host strongly determines its optical and spin characteristics. Consequently, techniques for controlling the charge state are required to realize technologies such as quantum…

Quantum Physics · Physics 2024-09-02 Christian Pederson , Nicholas S. Yama , Lane Beale , Matthew L. Markham , Kai-Mei C. Fu
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