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We use a numerically exact real-time path integral Monte Carlo scheme to compute electron transfer dynamics between two redox sites within a spin-boson approach. The case of asymmetric reactions is studied in detail in the least understood…

Condensed Matter · Physics 2009-11-10 L. Muehlbacher , R. Egger

The existence and properties of low Mach-number ($M \gtrsim 1$) electrostatic collisionless shocks are investigated with a semi-analytical solution for the shock structure. We show that the properties of the shock obtained in the…

We report on the direct observation of the thermoelectric transport in a nondegenerate correlated electron system formed on the surface of liquid helium. We find that the microwave-induced excitation of the vertical transitions of electrons…

Other Condensed Matter · Physics 2021-11-10 Ivan Kostylev , A. A. Zadorozhko , M. Hatifi , Denis Konstantinov

A new scheme is proposed for modeling molecular nonadiabatic dynamics near metal surfaces. The charge-transfer character of such dynamics is exploited to construct an efficient reduced representation for the electronic structure. In this…

Chemical Physics · Physics 2020-09-24 Zuxin Jin , Joseph E. Subotnik

We explore electron pre-acceleration at high Mach-number nonrelativistic perpendicular shocks at, e.g., young supernova remnants, which are a prerequisite of further acceleration to very high energies via diffusive shock acceleration. Using…

High Energy Astrophysical Phenomena · Physics 2019-11-06 Artem Bohdan , Jacek Niemiec , Martin Pohl , Yosuke Matsumoto , Takanobu Amano , Masahiro Hoshino

Electron bulk heating during magnetic reconnection with symmetric inflow conditions is examined using kinetic particle-in-cell (PIC) simulations. The degree of electron heating is well correlated with the inflowing Alfv\'en speed $c_{Ar}$…

Plasma Physics · Physics 2015-06-23 M. A. Shay , C. C. Haggerty , T. D. Phan , J. F. Drake , P. A. Cassak , P. Wu , M. Oieroset , M. Swisdak , K. Malakit

We address the problem of overheating of electrons trapped on the liquid helium surface by cyclotron resonance excitation. Previous experiments, suggest that electrons can be heated to temperatures up to 1000K more than three order of…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 A. D. Chepelianskii , Masamitsu Watanabe , Kimitoshi Kono

Electric, thermal and thermoelectric transport in correlated electron systems probe different aspects of the many-body dynamics, and thus provide complementary information. These are well studied in the low- and high-temperature limits,…

Strongly Correlated Electrons · Physics 2020-02-19 Woo-Ram Lee , Alexander M. Finkel'stein , Karen Michaeli , Georg Schwiete

In the dynamics of atoms and molecules at metal surfaces, electron-hole pair excitations can play a crucial role. In the case of hyperthermal hydrogen atom scattering, they lead to nonadiabatic energy loss and highly inelastic scattering.…

Materials Science · Physics 2024-12-02 Connor L. Box , Nils Hertl , Wojciech G. Stark , Reinhard J. Maurer

The analysis of the wave content inside a perpendicular bow shock indicates that heating of ions is related to the Lower-Hybrid-Drift (LHD) instability, and heating of electrons to the Electron-Cyclotron-Drift (ECD) instability. Both…

Space Physics · Physics 2020-05-19 Krzysztof Stasiewicz

Thermodynamics of a pseudospin-electron model without correlations is investigated. The correlation functions, the mean values of pseudospin and particle number, as well as the thermodynamic potential are calculated. The calculation is…

Superconductivity · Physics 2014-02-17 I. V. Stasyuk , A. M. Shvaika , K. V. Tabunshchyk

Does overall thermal equilibrium exist between ions and electrons in a weakly collisional, magnetised, turbulent plasma---and, if not, how is thermal energy partitioned between ions and electrons? This is a fundamental question in plasma…

Plasma Physics · Physics 2019-01-17 Yohei Kawazura , Michael Barnes , Alexander A. Schekochihin

Weakly magnetized shock waves are paramount to a large diversity of environments, including supernova remnants, blazars, and binary-neutron-star mergers. Understanding the distribution of energy between electrons and ions within these…

High Energy Astrophysical Phenomena · Physics 2024-10-22 Arno Vanthieghem , Vasileios Tsiolis , Frederico Fiuza , Kazuhiro Sekiguchi , Anatoly Spitkovsky , Yasushi Todo

The early acceleration of protons and electrons in the nonrelativistic collisionless shocks with three obliquities are investigated through 1D particle-in-cell simulations. In the simulations, the charged particles possessing a velocity of…

High Energy Astrophysical Phenomena · Physics 2020-05-06 Jun Fang , Chun-Yan Lu , Jing-Wen Yan , Huan Yu

A statistical-type model is developed to describe the ion production and electron emission in collisions of (molecular) ions with atoms. The model is based on the Boltzmann population of the bound electronic energy levels of the quasi…

Atomic Physics · Physics 2016-08-19 Zoltán Juhász

Collisionless shocks tend to send charged particles into the upstream, driving electric currents through the plasma. Using kinetic particle-in-cell simulations, we investigate how the background thermal plasma neutralizes such currents in…

High Energy Astrophysical Phenomena · Physics 2023-12-22 Siddhartha Gupta , Damiano Caprioli , Anatoly Spitkovsky

The non-equilibrium dynamics of electrons is of a great experimental and theoretical value providing important microscopic parameters of the Coulomb and electron-phonon interactions in metals and other cold plasmas. Because of the…

Superconductivity · Physics 2008-11-19 V. V. Kabanov , A. S. Alexandrov

The course of non-thermal electron ejection in relativistic unmagnetized electron-ion shocks is investigated by performing self-consistent particle-in-cell simulations. The shocks are excited through the injection of relativistic jet into…

High Energy Astrophysical Phenomena · Physics 2016-08-24 Kazem Ardaneh , Dongsheng Cai , Ken-Ichi Nishikawa

Electron transfer is an important and fundamental process in chemistry, biology and physics, and has received significant attention in recent years. Perhaps one of the most intriguing questions concerns with the realization of the…

Mesoscale and Nanoscale Physics · Physics 2023-05-30 Bokang Hou , Michael Thoss , Uri Banin , Eran Rabani

In this work we develop a theory of correlated many-electron dynamics dressed by the presence of a finite-temperature harmonic bath. The theory is based on the ab-initio Hamiltonian, and thus well-defined apart from any phenomenological…

Quantum Physics · Physics 2015-06-05 John A. Parkhill , Thomas Markovich , David G. Tempel , Alan Aspuru-Guzik