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The phase diagram of Ca$_{2-x}$Sr$_x$RuO$_4$ has been studied by neutron diffraction on powder and single-crystalline samples. The experiments reveal antiferromagnetic order and structural distortions characterized by tilts and rotations of…

Superconductivity · Physics 2009-10-31 O. Friedt , M. Braden , G. Andre , P. Adelmann , S. Nakatsuji , Y. Maeno

The tetragonal-to-orthorhombic structural phase transition (SPT) in LaFeAsO (La-1111) and SmFeAsO (Sm-1111) single crystals measured by high resolution x-ray diffraction is found to be sharp while the RFeAsO (R=La, Nd, Pr, Sm)…

The heavy-fermion compound CeCu$_{6-x}$Au$_x$ has become a model system for unconventional magnetic quantum criticality. For small Au concentrations $0 \leq x < 0.16$, the compound undergoes a structural transition from orthorhombic to…

Strongly Correlated Electrons · Physics 2018-08-29 K. Grube , L. Pintschovius , F. Weber , J. -P. Castellan , S. Zaum , S. Kuntz , P. Schweiss , O. Stockert , S. Bachus , Y. Shimura , V. Fritsch , H. v. Löhneysen

Theoretically, materials that break multiple symmetries allow, under certain conditions, the formation of four-fermion condensates above the superconducting critical temperature. Such states can be stabilized by phase fluctuations. Recently…

The temperature dependence of the elastic properties of antiferroelectric PbHfO3 was investigated by Brillouin scattering. The two structural phase transitions of antiferroelectric-antiferroelectric-paraelectric phases were clearly…

Materials Science · Physics 2015-06-18 Jae-Hyeon Ko , Krystian Roleder , Andrzej Majchrowski , Annette Bussmann-Holder

We report X-ray structural studies of the metal-insulator phase transition in bismuth ferrite, BiFeO3, both as a function of temperature and of pressure (931 oC at atmospheric pressure and ca. 45 GPa at ambient temperature). Based on the…

Materials Science · Physics 2009-02-05 S. A. T. Redfern , J. N. Walsh , S. M. Clark , G. Catalan , J. F. Scott

We investigate the transient electronic structure of BaFe2As2, a parent compound of iron-based superconductors, by time- and angle-resolved photoemission spectroscopy. In order to probe the entire Brillouin zone, we utilize extreme…

The origin of successive phase transitions observed in the layered perovskite $\alpha$-Sr$_2$CrO$_4$ is studied by the density-functional-theory-based electronic structure calculation and mean-field analysis of the proposed low-energy…

Strongly Correlated Electrons · Physics 2017-02-08 T. Ishikawa , T. Toriyama , T. Konishi , H. Sakurai , Y. Ohta

The crystal structures of the quasi-one-dimensional organic salts (TMTTF)$_2$PF$_6$ and (TMTSF)$_2$PF$_6$ were studied by pressure-dependent x-ray diffraction up to 10 GPa at room temperature. The unit-cell parameters exhibit a clear…

Strongly Correlated Electrons · Physics 2009-10-05 A. Pashkin , M. Dressel , S. G. Ebbinghaus , M. Hanfland , C. A. Kuntscher

Ba2CaMoO6 was synthesized by solid state method. The crystal structure adopts cubic Fm-3m space group at room temperature with lattice parameters of 8.378231(5) {angstroms}. Upon cooling, Ba2CaMoO6 was determined to have a structural phase…

Materials Science · Physics 2020-11-03 Loi T. Nguyen , Robert J. Cava , Allyson M. Fry-Petit

The 5d pyrochlore oxide Cd2Re2O7 exhibits successive phase transitions from a cubic pyrochlore structure (phase I) to a tetragonal structure without inversion symmetry below Ts1 of ~200 K (phase II) and further to another noncentrosymmetric…

We report investigation of structural phase transitions in technologically important material sodium niobate as a function of temperature on heating over 300-1075 K. Our high resolution powder neutron diffraction data show variety of…

Materials Science · Physics 2015-05-20 S. K. Mishra , R. Mittal , V. Yu. Pomjakushin , S. L. Chaplot

Motivated by the search for type-II multiferroics, we present a comprehensive optical study of a complex oxide family of type-II multiferroic candidates: RbFe(MoO4)2, RbFe(SeO4)2, and RbFe(SO4)2. We employ rotational-anisotropy second…

Results of high resolution x-ray diffraction experiments are presented for single crystals of the spin gap compound BaCuSi$_2$O$_6$ in the temperature range from 16 to 300 K. The data show clear evidence of a transition from the room…

Strongly Correlated Electrons · Physics 2009-11-11 E. C. Samulon , Z. Islam , S. E. Sebastian , P. B. Brooks , M. K. McCourt , J. Ilavsky , I. R. Fisher

We present a joint theoretical and experimental study to investigate polymorphism in $\alpha$-sexithiophene (6T) crystals. By means of density-functional theory calculations, we clarify that the low-temperature phase is favorable over the…

Materials Science · Physics 2016-06-29 Bernhard Klett , Caterina Cocchi , Linus Pithan , Stefan Kowarik , Claudia Draxl

We present a detailed low-temperature investigation of the statics and dynamics of the anions and methyl groups in the organic conductors (TMTSF)$_2$PF$_6$ and (TMTSF)$_2$AsF$_6$ (TMTSF : tetramethyl-tetraselenafulvalene). The 4 K neutron…

Strongly Correlated Electrons · Physics 2013-08-01 P. Foury-Leylekian , S. Petit , I. Mirebeau , G. Andre , M. de Souza , M. Lang , E. Ressouche , A. Moradpour , J. -P. Pouget

We present the specific heat, magnetization, optical spectroscopy measurements and the firstprinciple calculations on the Weberite structure Ca2Os2O7 single crystal/polycrystalline sample. The Ca2Os2O7 shows a Curie-Weiss nature at high…

Strongly Correlated Electrons · Physics 2015-06-11 P. Zheng , Y. G. Shi , Q. S. Wu , G. Xu , T. Dong , Z. G. Chen , R. H. Yuan , B. Cheng , K. Yamaura , J. L. Luo , N. L. Wang

Group theoretical aspects of the three temperature-dependent and temperature-reversible experimentally observed phase transitions in the KNbO3 crystal (cubic-tetragonal, tetragonal-orthorhombic, orthorhombic-rhombohedral) in the framework…

Materials Science · Physics 2024-11-05 R. A. Evarestov , Yu. E. Kitaev , S. S. Novikov

MnSb$_{2}$O$_{6}$ is based on the structural chiral $P$321 space group #150 where the magnetic Mn$^{2+}$ moments ($S=5/2$, $L\approx 0$) order antiferromagnetically at $T_\mathrm{N}=12$ K. Unlike the related iron based langasite…

Comprehensive x-ray scattering studies, including resonant scattering at Mn L-edge, Tb L- and M-edges, were performed on single crystals of TbMn2O5. X-ray intensities were observed at a forbidden Bragg position in the ferroelectric phases,…