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A multitude of observed boron-based materials have outstanding superconducting, mechanical, and refractory properties. Yet, the structure, the composition, and the very existence of some reported metal boride (M-B) compounds have been a…

Materials Science · Physics 2014-10-03 A. G. Van Der Geest , A. N. Kolmogorov

We have used density-functional-theory methods and the ab initio random structure searching (AIRSS) approach to predict stable structures and stoichiometries of mixtures of iron and oxygen at high pressures. Searching was performed for 12…

Materials Science · Physics 2015-08-24 Gihan L. Weerasinghe , R. J. Needs , Chris J. Pickard

We present our findings of a large-scale screening for new synthesizable materials in five M-Sn binaries, M = Na, Ca, Cu, Pd, and Ag. The focus on these systems was motivated by the known richness of M-Sn properties with potential…

Materials Science · Physics 2025-07-10 Aidan Thorn , Daviti Gochitashvili , Saba Kharabadze , Aleksey N. Kolmogorov

Group I/II materials exhibit unexpected structural phase transitions at high pressures, providing potential insight into the origins of elemental superconductivity. We present here a computational study of elemental barium and binary…

Materials Science · Physics 2012-07-16 Joshua A. Taillon , William W. Tipton , Richard G. Hennig

Following the idea that hydrogen-rich compounds might be high-T$_c$ superconductors at high pressures, and the very recent breakthrough in predicting and synthesizing hydrogen sulfide with record-high T$_c$ = 203 K, ab initio evolutionary…

Superconductivity · Physics 2017-04-19 M. M. Davari Esfahani , A. R. Oganov , H. Niu , J. Zhang

Since graphene was synthesized the interest for building new 2D and 3D structures based on the carbon allotropes has been growing every day. One of these 3D structures is know as carbon schwarzites. Schwarzites consist of carbon…

Materials Science · Physics 2020-08-26 Raphael M. Tromer , Levi C. Felix , Cristiano F. Woellner , Douglas S. Galvao

Density-functional-theory (DFT) calculations have been performed on the Li-Si and Li-Ge systems. Lithiated Si and Ge, including their metastable phases, play an important technological r\^ole as Li-ion battery (LIB) anodes. The calculations…

Materials Science · Physics 2015-06-18 Andrew J. Morris , C. P. Grey , C. J Pickard

We study the electronic and lattice dynamical properties of compressed solid germane in the pressure range up to 200 GPa with density functional theory. A stable metallic structure, Aba2, with a base-centered orthorhombic symmetry was found…

Superconductivity · Physics 2008-05-01 Chao Zhang , Yanling Li , Xiaojia Chen , Ruiqin Zhang , Haiqing Lin

First thermoelectric properties measurements on bulk nanostructured Ba8Ga16Ge30 clathrate-I are presented. A sol-gel-calcination route was developed for preparing amorphous nanosized precursor oxides. The further reduction of the oxides led…

Hexagonal SiGe is a promising material for combining electronic and photonic technologies. In this work, the energetic, structural, elastic and electronic properties of the hexagonal polytypes (2$H$, 4$H$ and 6$H$) of silicon and germanium…

We performed a systematic search for low-energy structures of binary iron silicide over a wide range of compositions using the crystal structure prediction method based on adaptive genetic algorithm. 36 structures with formation energies…

Mesoscale and Nanoscale Physics · Physics 2018-08-29 Zejin Yang , Shunqing Wu , Xin Zhao , Manh Cuong Nguyen , Shu Yu , Tongqi Wen , Ling Tang , Fuxiang Li , Kai-Ming Ho , Cai-Zhuang Wang

A growing body of theoretical and experimental evidence suggests that inert gases (He, Ne, Ar, Kr, Xe, Rn) become less and less inert under increasing pressure. Here we use the ab initio evolutionary algorithm to predict stable compounds of…

Two novel three-dimensional (3D) crystal structures of carbon (C) and germanium carbide (GeC2) were predicted using first-principles density-functional theory (DFT) calculations. These newly discovered 3D carbon allotrope and GeC2 are in…

Materials Science · Physics 2020-12-15 Ying Yang , Guang Yang , Xihong Peng

We have developed an efficient crystal structure prediction (CSP) method for desired chemical compositions, specifically suited for compounds featuring recurring molecules or rigid bodies. We applied this method to two metal chalcogenides:…

Materials Science · Physics 2024-08-01 Qi Zhang , Amitava Choudhury , Aleksandr Chernatynskiy

The simple alkali metal Na, that crystallizes in a body-centred cubic structure at ambient pressure, exhibits a wealth of complex phases at extreme conditions as found by experimental studies. The analysis of the mechanism of stabilization…

Materials Science · Physics 2009-09-25 V F Degtyareva , O Degtyareva

\emph{Ab-initio} calculations were performed on the scheelite type MGeO$_4$ (M = Hf, and Zr) compounds which find wide range of applications such as in x-ray imaging. We have studied the high pressure structural stability, elastic…

Materials Science · Physics 2014-05-30 G. Shwetha , V. Kanchana , K. Ramesh Babu , G. Vaitheeswaran , M. C. Valsakumar

We calculate the thermoelectric figure of merit, zT=S^2GT/(\kappa_l+\kappa_e), for p-type Si nanowires with axial Ge heterostructures using a combination of first-principles density-functional theory, interatomic potentials, and…

Materials Science · Physics 2011-11-29 Matthew Shelley , Arash A. Mostofi

The complex structures and electronic properties of alkali metals and their alloys provide a natural laboratory for studying the interelectronic interactions of metals under compression. A recent theoretical study (J. Phys. Chem. Lett.…

Materials Science · Physics 2021-01-12 Yangmei Chen , Xiaozhen Yan , Huayun Geng , Xiaowei Sheng , Leilei Zhang , Hao Wang , Jinglong Li , Ye Cao , Xiaolong Pan

Crystal structure prediction has traditionally relied on prototype-based seeding, approaches that often bias sampling toward known low-energy basins and overlook metastable polymorphs with unconventional symmetries. Here, we introduce…

Materials Science · Physics 2026-04-24 Jiexi Song , Diwei Shi , Aixian She , Chongde Cao , Fengyuan Xuan

We have performed first principles study for bismuth crystal structure at pressure from 0~14 GPa based on structure search and quasi-harmonic approximation. A new stable phase with Pbcm symmetry is predicted by structure search method. We…

Materials Science · Physics 2019-03-08 Ya-Fan Zhao , Shou-Rui Li , Xing-Yu Gao , Ming-Feng Tian , Hai-Feng Song
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