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Inter-slit interactions across one-dimensional arrays of sub-micro meter rectangular holes in gold films are explored. Using electron energy loss spectroscopy combined with scanning transmission electron microscopy, a series of cavity…

We present first-principles many-body calculations of the dielectric constant, quasiparticle band structure, and optical absorption spectrum of monolayer MoS$_2$ using a supercell approach. As the separation between the periodically…

Materials Science · Physics 2014-01-15 Falco Hüser , Thomas Olsen , Kristian S. Thygesen

Scanning tunneling spectroscopy requires the application of a potential difference between the sample and a tip. In metal-vacuum-metal junctions, one can safely assume that the potential is constant along the metallic substrate. Here, we…

Mesoscale and Nanoscale Physics · Physics 2020-12-22 Nils Krane , Christian Lotze , Nils Bogdanoff , Gael Reecht , Lei Zhang , Alejandro L. Briseno , Katharina J. Franke

We experimentally investigate charge transport through the interface between a gold electrode and a black phosphorus single crystal. The experimental $dI/dV(V)$ curves are characterized by well developed zero-bias conductance peak and two…

Mesoscale and Nanoscale Physics · Physics 2020-06-29 N. N. Orlova , N. S. Ryshkov , A. A. Zagitova , V. I. Kulakov , A. V. Timonina , D. N. Borisenko , N. N. Kolesnikov , E. V. Deviatov

Two-dimensional electron dispersions with peculiar band crossings provide a platform for realizing topological phases of matter. Here we theoretically show that the $e_g$-orbital manifold of honeycomb-layered transition metal compounds…

Materials Science · Physics 2019-01-09 Yusuke Sugita , Yukitoshi Motome

The rational design of single molecule electrical components requires a deep and predictive understanding of structure-function relationships. Here we explore the relationship between chemical substituents and the conductance of…

Graphene devices require electric contacts with metals, particularly with gold. Scanning tunneling spectroscopy studies of electron local density of states performed on mono-, bi- and tri- graphene layer deposited on metallic conductive…

Materials Science · Physics 2009-01-05 Z. Klusek , P. Dabrowski , P. Kowalczyk , W. Kozlowski , P. Blake , M. Szybowicz , T. Runka , W. Olejniczak

We review the binding and energy level alignment of $\pi$-conjugated systems on metals, a field which during the last two decades has seen tremendous progress both in terms of experimental characterization as well as in the depth of…

Materials Science · Physics 2020-05-01 Antoni Franco-Cañellas , Steffen Duhm , Alexander Gerlach , Frank Schreiber

We study level correlations in a two-dimensional system with a long-range random potential and strong spin-orbit (SO) splitting of the spectrum. The level correlations for sufficiently large splitting are shown to be described by orthogonal…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 A. P. Dmitriev , V. Yu. Kachorovskii

Conductance measurements of a molecular wire, contacted between an epitaxial molecule-metal bond and the tip of a scanning tunneling microscope, are reported. Controlled retraction of the tip gradually de-hybridizes the molecule from the…

Strongly Correlated Electrons · Physics 2024-02-05 R. Temirov , A. C. Lassise , F. Anders , F. S. Tautz

The alignment of the Fermi level of a metal electrode within the gap of the hi ghest occupied (HOMO) and lowest unoccupied orbital (LUMO) of a molecule is a key quantity in molecular electronics, which can vary the electron transparency of…

Materials Science · Physics 2009-11-11 R. Stadler , K. W. Jacobsen

Estimating the relative alignment between the frontier molecular orbitals that dominates the charge transport through single-molecule junctions represents a challenge for theory. This requires approaches beyond the widely employed framework…

Mesoscale and Nanoscale Physics · Physics 2015-09-22 Ioan Baldea

Among different topological and related phases of condensed matter, nodal semimetals occupy a special place - the electronic band topology in these materials is related to three-dimensional bulk, rather than to surface, states. A great…

Mesoscale and Nanoscale Physics · Physics 2021-04-28 A. V. Pronin , M. Dressel

Electromagnetic fields with complex spatial variation routinely arise in Nature. We study the response of a small molecule to monochromatic fields of arbitrary three-dimensional geometry. First, we consider the allowed configurations of the…

Optics · Physics 2010-11-23 Nan Yang , Adam E. Cohen

Recent experiments by Venkatamaran {\em et al.} [Nature (London) {\bf 442}, 904 (2006)] on a series of molecular wires with varying chemical compositions, revealed a linear dependence of the conductance on $\mathrm{cos}^2\theta$, where…

The effect of structural constriction on molecular mobility is investigated by broadband dielectric spectroscopy (BDS) within three types of molecular arrangements: monomers, oligomers and self-assembled monolayers (SAMs). While disordered…

We considered the question of applying the multiscale entanglement renormalization ansatz (MERA) to describe chiral topological phases. We defined a functional for each layer in the MERA, which captures the correlation length. With some…

Mesoscale and Nanoscale Physics · Physics 2019-06-12 Zhi Li , Roger S. K. Mong

Electronic level alignment at the interface between an adsorbed molecular layer and a semiconducting substrate determines the activity and efficiency of many photocatalytic materials. We perform $G_0W_0$ calculations to determine the…

Materials Science · Physics 2014-08-28 Annapaola Migani , Duncan J. Mowbray

Li and Haldane conjectured and numerically substantiated that the entanglement spectrum of the reduced density matrix of ground-states of time-reversal breaking topological phases (fractional quantum Hall states) contains information about…

Strongly Correlated Electrons · Physics 2013-02-05 A. Chandran , M. Hermanns , N. Regnault , B. A. Bernevig

Excitons in thin layers of semiconducting transition metal dichalcogenides are highly subject to the strongly modified Coulomb electron-hole interaction in these materials. Therefore, they do not follow the model system of a two-dimensional…