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X-ray photoelectron spectra provide a wealth of information on the electronic structure. The extraction of molecular details requires adequate theoretical methods, which in case of transition metal complexes has to account for effects due…

The motion of fast electrons through the crystal during axial channeling could be regular and chaotic. The dynamical chaos in quantum systems manifests itself in both statistical properties of energy spectra and morphology of wave functions…

Accelerator Physics · Physics 2018-02-26 N. F. Shul'ga , V. V. Syshchenko , A. I. Tarnovsky , I. I. Solovyev , A. Yu. Isupov

Dynamics of ionic-to-neutral and neutral-to-ionic phase transitions induced by intrachain charge-transfer photoexcitations are studied in a quasi-one-dimensional extended Hubbard model with alternating potentials and an electron-lattice…

Strongly Correlated Electrons · Physics 2007-05-23 Kenji Yonemitsu

A new approach has been used to explain the experimental data for the $^{12}$C+$^{12}$C system over a wide energy range in the laboratory system from 32.0 MeV to 126.7 MeV. This new coupled-channels based approach involves replacing the…

Nuclear Theory · Physics 2009-11-07 I. Boztosun , W. D. M. Rae

Quantum interference arising from superposition of states is a striking evidence of the validity of Quantum Mechanics, confirmed in many experiments and also exploited in applications. However, as for any scientific theory, Quantum…

Energy levels, radiative rates and lifetimes are reported for four S-like ions, namely Sc~VI, V VIII, Cr IX, and Mn~X. Two independent atomic structure codes, namely the general-purpose relativistic atomic structure package ({\sc grasp})…

Atomic Physics · Physics 2020-01-08 Kanti Aggarwal

It has been shown that to calculate the parameters of the electrostatic field of the ion crystal lattice it sufficient to take into account ions located at a distance of 1-2 lattice spacings. More distant ions make insignificant…

General Physics · Physics 2010-01-26 Alexander Ivanchin

The wavelengths and radiative transition probabilities for transitions 2lnl'-1snl", 2lnl'-1s2l", 1s2lnl'-1s^2.nl", 1s2lnl'-1s^2.2l", and the autoionization decay probabilities for doubly excited states 2lnl', 1s2lnl' were calculated in ions…

Atomic Physics · Physics 2007-05-23 F. F. Goryayev , A. M. Urnov , L. A. Vainshtein

Gas phase C$_{70}$ molecules have been ionized with single photons of energies between 16 eV and 70 eV and the electron spectra measured with velocity map imaging in coincidence with the ions. The doubly ionized and unfragmented species was…

Magnetic reconnection is a leading mechanism for magnetic energy conversion and high-energy non-thermal particle production in a variety of high-energy astrophysical objects, including ones with relativistic ion-electron plasmas (e.g.,…

High Energy Astrophysical Phenomena · Physics 2014-11-05 Mickaël Melzani , Rolf Walder , Doris Folini , Christophe Winisdoerffer , Jean M. Favre

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…

We introduce and benchmark a systematically improvable route for excited-state calculations, state-specific configuration interaction ($\Delta$CI), \alert{which is a particular realization of multiconfigurational self-consistent field and…

Chemical Physics · Physics 2023-08-31 Fábris Kossoski , Pierre-François Loos

For a given electronic excited state, the 0-0 energy ($T_0$ or $T_{00}$) is the simplest property allowing straightforward and physically-sound comparisons between theory and (accurate) experiment. However, the computation of 0-0 energies…

Chemical Physics · Physics 2020-06-05 Pierre-François Loos , Denis Jacquemin

Multireference electron correlation methods describe static and dynamical electron correlation in a balanced way, and therefore, can yield accurate and predictive results even when single-reference methods or multiconfigurational…

Chemical Physics · Physics 2019-11-19 Jae Woo Park , Rachael Al-Saadon , Matthew K. MacLeod , Toru Shiozaki , Bess Vlaisavljevich

Electronic excitations and ionisations produced by electron impact are key processes in the radiation-induced damage mechanisms in materials of biological relevance, underlying important medical and technological applications, including…

Chemical Physics · Physics 2021-08-04 Pablo de Vera , Isabel Abril , Rafael Garcia-Molina

The periodic changes in physical and chemical properties of the chemical elements is caused by the periodic change of the ionization energies. The ionization energy of each element is constant and this manifests itself in the periodic…

Energy levels, wavelengths, magnetic-dipole and electric-quadrupole transition rates between the low-lying states are evaluated for W$^{51+}$ to W$^{54+}$ ions with $3d^n$ (n = 2 to 5) electronic configurations using an approach combining…

Atomic Physics · Physics 2018-01-10 M. S. Safronova , U. I. Safronova , S. G. Porsev , M. G. Kozlov , Yu. Ralchenko

Energy levels and fine-structure intervals of the $1s2l2l'$ core-excited states are calculated for ions along the Li isoelectronic sequence from argon to uranium. The calculation is performed by the relativistic configuration-interaction…

Atomic Physics · Physics 2018-07-17 V. A. Yerokhin , A. Surzhykov

The variational quantum eigensolver (VQE) algorithm, designed to calculate the energy of molecular ground states on near-term quantum computers, requires specification of symmetries that describe the system, e.g. spin state and number of…

Quantum Physics · Physics 2020-06-18 Gabriel Greene-Diniz , David Muñoz Ramo

We calculate, via variational techniques, single- and two-photon Rydberg microwave transitions, as well as scalar and tensor polarizabilities of sodium atom using the parametric one-electron valence potential, including the spin-orbit…

Atomic Physics · Physics 2024-02-20 Mariusz Pawlak , Eve L. Schoen , Justin E. Albert , H. R. Sadeghpour