Related papers: Floquet Nonadiabatic Mixed Quantum-Classical Dynam…
For a system without spin-orbit coupling, the (i) nuclear plus electronic linear momentum and (ii) nuclear plus orbital electronic angular momentum are good quantum numbers. Thus, when a molecular system undergoes a nonadiabatic transition,…
Strong laser light drives complex quantum electron dynamics in solids, which is captured by the high-harmonic generation (HHG) process. Here we report the observation of laser-dressed Floquet-Bloch states (FBSs) at the edge of the Brillouin…
We describe vacuum fluctuations and photon-field correlations in interacting quantum mechanical light-matter systems, by generalizing the application of mixed quantum-classical dynamics techniques. We employ the multi-trajectory…
Dissociative chemisorption is a key process in hydrogen-metal surface chemistry, where nonadiabatic effects due to low-lying electron-hole-pair excitations may affect reaction outcomes. Molecular dynamics with electronic friction…
Nonadiabatic molecular dynamics is a key technique for investigating a broad range of photochemical and photophysical processes. Among the established approaches, surface hopping schemes are widely used and can be easily integrated with…
Chemical relaxation phenomena, including photochemistry and electron transfer processes, form a vigorous area of research in which nonadiabatic dynamics plays a fundamental role. Here, we show that for nonadiabatic dynamics with two…
Accurate description of nonadiabatic dynamics of molecules at metal surfaces involving electron transfer has been a longstanding challenge for theory. Here, we tackle this problem by first constructing high-dimensional neural network…
We benchmark a set of quantum-chemistry methods, including multitrajectory Ehrenfest, fewest-switches surface-hopping, and multiconfigurational-Ehrenfest dynamics, against exact quantum-many-body techniques by studying real-time dynamics in…
We investigate the rich non-equilibrium physics arising in periodically driven open quantum systems, specifically those realized within microcavity resonators, whose dynamics are governed by a non-Hermitian Hamiltonian hosting Floquet…
We present a novel semiclassical phase-space surface hopping approach that goes beyond the Born-Oppenheimer approximation and all existing surface hopping formalisms. We demonstrate that working with a correct phase-space electronic…
We study the dynamics and timescales of a periodically driven Fermi-Hubbard model in a three-dimensional hexagonal lattice. The evolution of the Floquet many-body state is analyzed by comparing it to an equivalent implementation in undriven…
We propose a `Floquet engineering' formalism to systematically design a periodic driving protocol in order to stroboscopically realize the desired system starting from a given static Hamiltonian. The formalism is applicable to quantum…
We consider Mott insulators driven by periodic coherent laser radiation, using both single orbital and multi-orbital models, noting that the latter is of more interest in solid state systems. We derive general expressions for the resulting…
We propose a method to obtain Floquet states---also known as light-induced states---and their quasi-energies from real-time wavefunctions without solving the Floquet equation. This is useful for the analysis of various phenomena in…
The combination of solid state single-photon emitters and mechanical excitations on a common platform is a promising approach for the development of hybrid quantum technologies. In this topical review we discuss state-of-the-art platforms…
Mixed quantum-classical methods, such as surface hopping and Ehrenfest dynamics, have proven useful for describing molecular processes involving multiple electronic states. These methods require propagating many independent trajectories,…
Flux attachment provides a powerful conceptual framework for understanding certain forms of topological order, including most notably the fractional quantum Hall effect. Despite its ubiquitous use as a theoretical tool, directly realizing…
In this work, we study a space-time modulated electro-mechanical system, consisting of an array of coupled cantilevers with their on-site potential provided by electromagnets driven by AC currents. Model equations are derived, and the…
We generalize the Schrieffer-Wolff transformation to periodically driven systems using Floquet theory. The method is applied to the periodically driven, strongly interacting Fermi-Hubbard model, for which we identify two regimes resulting…
An iterative algorithm is established which enables one to compute individual Floquet states even for many-body systems with high-dimensional Hilbert spaces that are not accessible to commonly employed conventional methods. A strategy is…