English
Related papers

Related papers: Electronic dynamics created at conical intersectio…

200 papers

Recently we reported a series of numerical simulations proving that it is possible in principle to create an electronic wave packet and subsequent electronic motion in a neutral molecule photoexcited by a UV pump pulse within a few…

Atomic and Molecular Clusters · Physics 2016-10-24 P. Decleva , N. Quadri , A. Perveaux , D. Lauvergnat , F. Gatti , B. Lasorne , G. J. Halász , Á. Vibók

Chemical activity is known to affect phase coexistence and coarsening in liquid mixtures, most commonly through reaction-induced changes of intermolecular interactions. Here, we analyze a scenario in which chemical reactions regulate…

Soft Condensed Matter · Physics 2026-03-19 Florian Raßhofer , Erwin Frey

Using numerical simulations, we study the dynamical evolution of particles interacting via competing long-range repulsion and short-range attraction in two dimensions. The particles are compressed using a time-dependent quasi-one…

Soft Condensed Matter · Physics 2017-12-06 D. McDermott , C. J. Olson Reichhardt , C. Reichhardt

Understanding the organizing principles of interacting electrons and the emergence of novel electronic phases is a central endeavor of condensed matter physics. Electronic nematicity, in which the discrete rotational symmetry in the…

The spatial distribution of the internal pressure of an electron fluid, which spontaneously arises at the formation of a molecule or a crystal, is linked to the main features of chemical bonding in molecular crystals. The local pressure is…

Chemical Physics · Physics 2016-05-04 Vladimir G. Tsirelson , Adam I. Stash , Ilya V. Tokatly

Fully kinetic simulations are applied to the study of 2D anti-parallel reconnection, elucidating the dynamics by which the electron fluid maintains force balance within both the electron diffusion region (EDR) and the ion diffusion region…

Plasma Physics · Physics 2023-06-16 J. Egedal , H. Gurram , S. Greess , W. Daughton , A. Lê

Among polycyclic aromatic hydrocarbons, pyrene is widely used as an optical probe thanks to peculiar ultraviolet absorption and infrared emission features. Interestingly, this molecule is also an abundant component of the interstellar…

Chemical Physics · Physics 2021-11-19 Katherine R. Herperger , Jannis Krumland , Caterina Cocchi

The dynamical properties and diffusive behavior of a collection of mutually interacting particles are numerically investigated for two types of long-range interparticle interactions: Coulomb-electrostatic and dipole-electrodynamic. It is…

It is important that any dynamics method approaches the correct population distribution at long times. In this paper, we derive a one-body reduced density matrix dynamics for electrons in energetic contact with a bath. We obtain a…

Quantum Physics · Physics 2015-04-09 Triet Nguyen , Ravindra Nanguneri , John Parkhill

The field of synthetic active matter has, thus far, been led by efforts to create point-like, isolated (yet interacting) self-propelled objects (\emph{e.g.} colloids, droplets, microrobots) and understanding their collective dynamics. The…

Soft Condensed Matter · Physics 2024-08-06 Manoj Kumar , Aniruddh Murali , Arvin Gopal Subramaniam , Rajesh Singh , Shashi Thutupalli

Formation of the nonequilibrium subsystem in dynamical processes during defect generation is simulated by means of molecular dynamics. A particular process of dissipation of the low-frequency acoustic emission into high-frequency…

Computational Physics · Physics 2009-12-11 Leonid S. Metlov

Earth's magnetotail is an excellent laboratory to study the interplay of reconnection and turbulence in determining electron energization. The process of formation of a power law tail during turbulent reconnection is a documented fact still…

Plasma Physics · Physics 2020-12-30 Giovanni Lapenta , Jean Berchem , Mostafa El Alaoui , Raymond Walker

The chemical dynamics scene is the most important application of computer simulation. We show that electrons jump between potential holes of different depths (new molecular orbits, hybrid atomic orbits with different energies) under the…

Quantum Physics · Physics 2023-10-17 Chen Ran , Yuri Ozhigov

Dynamics of a dry-rebounding drop was studied experimentally, numerically, and theoretically. Experimental results were reproduced by our computational fluid dynamics simulations, from which time series of kinetic energy, potential energy,…

Fluid Dynamics · Physics 2018-07-03 Akio Nishimura , Henry Weller , Hirokazu Maruoka , Masao Takayanagi , Hideharu Ushiki

A deep understanding of molecular photo-transformations is challenging because of the complex interaction between the configurations of electrons and nuclei. An initial optical excitation dissipates energy into electronic and structural…

We introduce multistate metadynamics for automatic exploration of conical intersection seams between adiabatic Born-Oppenheimer potential energy surfaces in molecular systems. By choosing the energy gap between the electronic states as a…

Chemical Physics · Physics 2018-05-10 Joachim O. Lindner , Merle I. S. Röhr , Roland Mitrić

Chemically active colloids or enzymes cluster into dense droplets driven by their phoretic response to collectively generated chemical gradients. Employing Brownian dynamics simulation techniques, our study of the dynamics of such a…

Soft Condensed Matter · Physics 2024-01-29 K. R. Prathyusha , Suropriya Saha , Ramin Golestanian

We examine the spatial distribution of electrons generated by a fixed energy point source in uniform, parallel electric and magnetic fields. This problem is simple enough to permit analytic quantum and semiclassical solution, and it harbors…

Quantum Physics · Physics 2007-05-23 Christian Bracher , Tobias Kramer , John B. Delos

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

Chemical Physics · Physics 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

There is a large debate on the destabilization mechanism of emulsions. We present a simple technique using mechanical compression to destabilize oil-in-water emulsions. Upon compression of the emulsion, the continuous aqueous phase is…