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Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…

Infrared Imaging Spectrograph (IRIS) is the first light instrument for the Thirty Meter Telescope (TMT) that consists of a near-infrared (0.84 to 2.4 micron) imager and integral field spectrograph (IFS) which operates at the…

Coherent anti-Stokes Raman scattering (CARS) microspectroscopy has demonstrated significant potential for biological and materials imaging. To date, however, the primary mechanism of disseminating CARS spectroscopic information is through…

Optics · Physics 2015-10-08 Charles H. Camp , Young Jong Lee , Marcus T. Cicerone

We present results of Raman spectroscopic studies of urine to determine the suitability of near-infrared Raman spectroscopy for quantitative estimation of urinary urea. The Raman spectra were acquired from the urine samples with an inbuilt…

Medical Physics · Physics 2014-12-24 S. Kumar , S. K. Majumdar

Coherent anti-Stokes Raman scattering (CARS) spectroscopy with time-delayed ultrashort pulses and a single-pixel photodetector has shown great potential for spectroscopic imaging and transient studies in chemistry and biological research.…

Optics · Physics 2023-12-05 Tianjian Lv , Bing Han , Ming Yan , Zhaoyang Wen , Kun Huang , Kangwen Yang , Heping Zeng

Angle-resolved Raman spectroscopy (ARRS) is an effective method to analyze the symmetry of phonons and other excitations in molecules and solid-state crystals. While there are several configurations of ARRS instruments, the measurement…

Spectral compression of femtosecond pulses by second harmonic generation in the presence of substantial group velocity dispersion provides a convenient source of narrowband Raman pump pulses for femtosecond stimulated Raman spectroscopy…

Optics · Physics 2015-06-12 E. Pontecorvo , C. Ferrante , C. G. Elles , T. Scopigno

Impact collision ion scattering spectroscopy (ICISS), which is a variation of low energy ion scattering (LEIS) that employs large scattering angles, is performed on Bi2Se3 surfaces prepared by ion bombardment and annealing (IBA). ICISS…

Materials Science · Physics 2017-07-24 Weimin Zhou , Haoshan Zhu , Jory A. Yarmoff

Terahertz spectroscopy allows for identifying different isomers of materials, for drug discrimination as well as for detecting hazardous substances. As many dielectric materials used for packaging are transparent in the terahertz spectral…

Optics · Physics 2020-11-06 Mirco Kutas , Björn Haase , Jens Klier , Daniel Molter , Georg von Freymann

Surface-enhanced Raman scattering (SERS) combines analyte-specificity and single-molecule sensitivity, but its potential is limited by slow readout where sophisticated nanosensors are analysed in a serial fashion, one particle at a time. We…

We propose and demonstrate a novel technique that combines Raman scattering and optical cycling in molecules with diagonal Franck-Condon factors. This resonance Raman optical cycling manipulates molecules to behave like efficient…

Atomic Physics · Physics 2021-08-26 J. C. Shaw , J. C. Schnaubelt , D. J. McCarron

We report on the first demonstration of nonlinear dual-frequency-comb spectroscopy. In multi-heterodyne femtosecond Raman-induced Kerr-effect spectroscopy, the Raman gain resulting from the coherent excitation of molecular vibrations by a…

By measuring the thermal effects resulting from stimulated Raman excitations, stimulated Raman photothermal (SRP) microscope offers a new access to spatially and temporally resolved Raman signatures across various sample types. Unlike…

Optics · Physics 2026-03-03 Yifan Zhu , Hongli Ni , Hongjian He , Yueming Li , Meng Zhang , Ji-Xin Cheng

The range of stimulated Raman scattering (SRS) frequencies covers a domain which at the low end abuts half the laser frequency, omega_0 / 2, according to the simplest SRS theories, corresponding to scatter from electron densities near 1/4…

Plasma Physics · Physics 2015-05-20 Harvey A. Rose , Philippe Mounaix

Plasmon-enhanced Raman scattering (PERS) becomes nonlinear when phonon pumping and phonon-stimulated scattering come into play. It is fundamental to the understanding of PERS and its photobleaching behavior. By quantization of the molecular…

Mesoscale and Nanoscale Physics · Physics 2017-05-31 Tian Yang , Jing Long , Xiaodan Wang

Infrared (IR) spectroscopy is an indispensable tool for many practical applications including material analysis and sensing. Existing IR spectroscopy techniques face challenges related to the inferior performance and the high cost of…

Optics · Physics 2017-03-13 Anna Paterova , Shaun Lung , Dmitry Kalashnikov , Leonid Krivitsky

Spontaneous Raman spectroscopy (SRS) is a conventional in-situ laser diagnostic method that has been widely used for measurements of temperature and major species. However, SRS in sooting flames suffers from strong interference including…

Optics · Physics 2023-02-15 Hu Meng , Yihua Ren , Heinz Pitsch

IRIS is a near-infrared (0.84 to 2.4 microns) integral field spectrograph and wide-field imager being developed for first light with the Thirty Meter (TMT). It mounts to the advanced optics (AO) system NFIRAOS and has integrated…

Pump-probe time-resolved x-ray diffraction of allowed and nearly forbidden reflections in InSb is used to follow the propagation of a coherent acoustic pulse generated by ultrafast laser-excitation. The surface and bulk components of the…

In this paper, we investigate the integration of integrated sensing and communication (ISAC) and reconfigurable intelligent surfaces (RIS) for providing wide-coverage and ultra-reliable communication and high-accuracy sensing functions. In…

Signal Processing · Electrical Eng. & Systems 2025-02-17 Rang Liu , Ming Li , Qian Liu , A. Lee Swindlehurst