Related papers: High-pressure X-ray photon correlation spectroscop…
We report X-ray Photon Correlation Spectroscopy (XPCS) results on a bidimensional (2D) gel formed by a Langmuir monolayer of gold nanoparticles. The system allows an experimental determination of the fourth order time correlation function…
The unprecedented brilliance of X-ray free-electron lasers (XFELs) [1, 2] has enabled first studies of nonlinear interactions in the hard X-ray range. In particular, X-ray-optical mixing [3], X-ray second harmonic generation (XSHG) [4] and…
Investigating electronic structure and excitations under extreme conditions gives access to a rich variety of phenomena. High pressure typically induces behavior such as magnetic collapse and the insulator-metal transition in 3d transition…
We have recently demonstrated a very favorable, inexpensive modernization of lab-based x-ray absorption fine structure (XAFS) and high-resolution x-ray emission spectroscopy (XES) using only commercially-available optics and x-ray tube…
X-ray photon correlation is used to probe the slow dynamics of the glass-former B2O3 across the glass transition. In the undercooled liquid phase the decay times of the measured correlation functions are consistent with visible light…
Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…
In the laboratory study of extreme conditions of temperature and density, the exposure of matter to high intensity radiation sources has been of central importance. Here we interrogate the performance of multi-layered targets in experiments…
Diffusion of proteins on length scales of their own diameter in highly concentrated solutions is essential for understanding the cellular machinery of living cells, but its experimental characterization remains a challenge. While X-ray…
A design for a compact x-ray light source (CXLS) with flux and brilliance orders of magnitude beyond existing laboratory scale sources is presented. The source is based on inverse Compton scattering of a high brightness electron bunch on a…
The characterization of the electronic structure and chemical states of gases, solids, and liquids can be effectively performed using ambient pressure X-ray photoelectron spectroscopy (AP-XPS). However, the acquisition of electronic and…
Multiphase flows where particles, bubbles, or droplets are suspended in a fluid govern critical processes in biology, medicine, materials processing, and geophysics. However, observing their microscale dynamics in opaque systems has…
In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…
Sub-femtosecond x-ray burst is powerful tool for probing and imaging electronic and concomitant atomic motion in attosecond physics. For years, x-ray source (above 2 keV) had mainly been obtained from X-ray free electron laser (XFEL) or…
Many magnetic equilibrium states and phase transitions are characterized by fluctuations. Such magnetic fluctuation can in principle be detected with scattering-based x-ray photon correlation spectroscopy (XPCS). However, in the established…
Pressure provides a powerful parameter to control the protein conformation state, which at sufficiently high values can lead to unfolding. Here, we investigate the effects of increasing pressure up to $0.4$ GPa on hydrated lysozyme…
We performed an analysis of coherence properties of the 4-th generation high-energy storage rings with emittance values of 10 pmrad. It is presently expected that a storage ring with these low emittance values will reach diffraction limit…
This study explores the possibility to measure dynamics of proteins in solution using X-ray photon correlation spectroscopy (XPCS) at nearly diffraction limited storage rings (DLSR). We calculate the signal to noise ratio (SNR) of XPCS…
Bright sources of high energy electromagnetic radiation are widely employed in fundamental research as well as in industry and medicine. This steadily growing interest motivated the construction of several facilities aiming at the…
In this article we report on the design, manufacture and testing of a high-pressure cell for doing simultaneous dielectric and neutron spectroscopy. This cell is a unique tool for studying dynamics on different timescales, from kilo- to…
Glass forming liquids exhibit structural relaxation behaviors, reflecting underlying atomic rearrangements on a wide range of timescales. These behaviors play a crucial role in determining many material properties. However, the relaxation…