Related papers: Electron Paramagnetic Resonance spectroscopy of a …
Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been proposed as a sensitive method for electron paramagnetic resonance (EPR) spectroscopy, enabled by the development of…
Electron spin resonance (ESR) spectroscopy is the method of choice for characterizing paramagnetic impurities, with applications ranging from chemistry to quantum computing, but it gives access only to ensemble-averaged quantities due to…
Progress in the emerging field of engineered quantum systems requires the development of devices that can act as quantum memories. The realisation of such devices by doping solid state cavities with paramagnetic ions imposes a trade-off…
We present experimental observations of dilute ion spin ensemble defects in a low-loss single crystal cylindrical sample of CaWO$_4$ cooled to $30$ mK in temperature. Crystal field perturbations were elucidated by constructing a…
Rare-earth spin ensembles are a promising platform for microwave quantum memory applications due to their hyperfine transitions, which can exhibit exceptionally long coherence times when using an operation point with zero first-order Zeeman…
The development of a new era of quantum devices requires an understanding of how paramagnetic dopants or impurity spins behave in crystal hosts. Here, we describe a new spectroscopic technique which uses traditional Electron Spin Resonance…
We report magnetic resonance spectroscopy measurements of individual nuclear spins in a crystal coupled to a neighbouring paramagnetic center, detected using microwave fluorescence at millikelvin temperatures. We observe real-time quantum…
The investigation of paramagnetic species (such as point defects, dopants, and impurities) in solid-state electronic devices is significant because of their effect on device performance. Conventionally, these species are detected and imaged…
Erbium-doped crystals offer a versatile platform for hybrid quantum devices because they combine magnetically-sensitive electron-spin transitions with telecom-wavelength optical transitions. At the high doping concentrations necessary for…
Coherent spin resonance methods, such as nuclear magnetic resonance and electron spin resonance spectroscopy, have led to spectrally highly sensitive, non-invasive quantum imaging techniques. Here, we propose a pump-probe spin resonance…
Presented are magnetization measurements on a crystal of Fe8 single-molecule magnets using a Hall probe magnetometer. Irradiation with microwaves at frequencies of 92 and 110-120 GHz leads to the observation of electron paramagnetic…
Rare earth ion (REI)-doped oxide thin films are attractive for the application of quantum interconnects due to their stable optical levels and scalability$^{1-3}$. Among them, Er$^{3+}$ doped CaWO$_{4}$ is promising because it possesses…
We study spin-lattice relaxation times of electron spins in Er$^{3+}$:CaWO$_4$ at millikelvin temperature, detected via their coupling to a low-mode volume superconducting resonator. At large magnetic field supporting strong phonon-emission…
Fe3+ ions in sapphire exhibit an Electron Spin Resonance (ESR) which interacts strongly with high-Q Whispering Gallery (WG) modes at microwave frequencies. We report the first observation of a third-order paramagnetic nonlinear…
Low-loss crystals with defects due to paramagnetic or rare earth impurity ions is a major area of investigation for quantum hybrid systems at both optical and microwave frequencies. In this work we examine the single crystal yttrium…
A new method for detecting the magnetic resonance of electronic spins at low temperature is demonstrated. It consists in measuring the signal emitted by the spins with a superconducting qubit that acts as a single-microwave-photon detector,…
Efficient quantum memory is of paramount importance for long-distance quantum communications, as well as for complex large-scale computing architectures. We investigate the capability of Er$^{3+}$:Y$_2$SiO$_5$ crystal to serve as a quantum…
Single-spin magnetic resonance spectroscopy promises to yield structural and chemical information at the level of individual atoms or molecules, in a non-invasive way. Here, we use an Er3+ paramagnetic center in a CaWO4 crystal, detected by…
Rare-earth ions doped in crystals with low nuclear-spin densities are highly promising candidates for quantum technology applications. In this study, we investigated the spectroscopic properties of the 7F0 - 5 D0 optical and the hyperfine…
We have demonstrated electron-electron and electron-nuclear spin manipulations of Gd3+ ion in CaWO4 crystal. The results suggest that the studied system is perspective for multiqubit implementation in quantum computing.