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We applied a tabletop, ultrafast, high-harmonic generation (HHG) source to measure the element-specific ferromagnetic resonance (FMR) in ultra-thin magnetic alloys and multilayers on an opaque Si substrate. We demonstrate a continuous wave…

Materials Science · Physics 2024-04-25 Michael Tanksalvala , Anthony Kos , Jacob Wisser , Scott Diddams , Hans T. Nembach , Justin M. Shaw

Generation of ultrabroadband isolated attosecond pulses (IAPs) is essential for time-resolved applications in chemical and material sciences, as they have the potential to access the spectral water window region of chemical elements, which…

Mesoscale and Nanoscale Physics · Physics 2022-04-20 Younes Adnani , Abdelmalek Taoutioui , Abdelkader Makhoute , Károly Tökési , Hicham Agueny

Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high…

Atomic Physics · Physics 2020-01-08 D. Hammerland , P. Zhang , S. Kuehn , P. Jojart , I. Seres , V. Zuba , Z. Varallyay , K. Osvay , T. T. Luu , H. J. Woerner

A dual color, frequency and pulse duration agile laser system, capable of delivering laser pulses in arbitrary temporal profiles with ~1 ns to ~1 us pulse duration, chirping rates of ~27 MHz/ns with an achievable chirping range of several…

Optics · Physics 2022-11-09 Junhwi Bak , Robert Randolph , Alexandros Gerakis

Cubic boron arsenide (BAs) is attracting greater attention due to the recent experimental demonstration of ultrahigh thermal conductivity \k{appa} above 1000 W/mK. However, its bandgap has not been settled and a simple yet effective method…

We report the development of an instrument combining an ultrafast, high-repetition-rate, polarization-tunable monochromatic extreme ultraviolet (XUV, 21.6 eV) beamline and a next-generation momentum microscope endstation. This setup enables…

We report a broadband terahertz time-domain spectroscopy (THz-TDS) which enables twenty vibrational modes of adenosine nucleoside to be resolved in a wide frequency range of 1-20 THz. The observed spectroscopic features of adenosine are in…

Optics · Physics 2020-08-26 Yao-chun Shen , Xing-yu Yang , Zi-jian Zhang

A large number of current and future experiments in neutrino and dark matter detection use the scintillation light from noble elements as a mechanism for measuring energy deposition. The scintillation light from these elements is produced…

Instrumentation and Methods for Astrophysics · Physics 2015-03-19 V. M. Gehman , S. R. Seibert , K. Rielage , A. Hime , Y. Sun , D. -M. Mei , J. Maassen , D. Moore

The recent demonstration of saturable absorption and negative optical conductivity in the Terahertz range in graphene has opened up new opportunities for optoelectronic applications based on this and other low dimensional materials.…

We present a novel approach to achieve hyper spectral resolution, high sensitive detection, and high speed data acquisition Stimulated Raman Spectroscopy by employing amplified offset-phase controlled fs-pulse bursts. In this approach, the…

Transition Edge Sensor (TES) spectrometers for hard X-ray beamline science will enable improved X-ray emission and absorption spectroscopy in the information-rich 2 to 20 keV energy range. We are building a TES-based instrument for the…

Instrumentation and Detectors · Physics 2020-08-26 Tejas Guruswamy , Lisa M. Gades , Antonino Miceli , Umeshkumar M. Patel , John T. Weizeorick , Orlando Quaranta

X-ray spectroscopy has been a key method to determine ground and excited state properties of quantum materials with atomic specificity. Now, new x-ray facilities are opening the door to the study of pump-probe x-ray spectroscopy -…

Strongly Correlated Electrons · Physics 2025-02-11 Daniel Jost , Eder G. Lomeli , Ta Tang , Joshua J. Kas , John J. Rehr , Wei-Sheng Lee , Hong-Chen Jiang , Brian Moritz , Thomas P. Devereaux

Bragg spectroscopy is one of the best established experimental methods for high energy resolution X-ray measurements and has been widely used in several fields, going from fundamental physics to quantum mechanics tests, synchrotron…

Instrumentation and Detectors · Physics 2019-03-08 A. Scordo , C. Curceanu , M. Miliucci , H. Shi , F. Sirghi , J. Zmeskal

Extreme ultraviolet pulses as generated by high harmonic generation (HHG) are a powerful tool for both time-resolved spectroscopy and coherent diffractive imaging. However, the integration of spectroscopy and microscopy to harness the…

We have studied the O 2p valence-band structure of Nb-doped SrTiO3, in which a dilute concentration of electrons are doped into the d0 band insulator, by angle-resolved photoemission spectroscopy (ARPES) measurements. We found that ARPES…

Materials Science · Physics 2009-03-23 K. Maekawa , M. Takizawa , H. Wadati , T. Yoshida , A. Fujimori , H. Kumigashira , M. Oshima

We propose angle-resolved two-photon photoemission spectroscopy (AR-2PPES) as a technique to detect the location of the bottom of the upper Hubbard band (UHB) in two-dimensional insulating cuprates. The AR-2PPES spectra are numerically…

Strongly Correlated Electrons · Physics 2007-05-23 H. Onodera , T. Tohyama , K. Tsutsui , S. Maekawa

We study the normal state electronic excitations probed by angle resolved photoemission spectroscopy (ARPES) in Bi2201 and Bi2212. Our main goal is to establish explicit criteria for determining the Fermi surface from ARPES data on strongly…

Coherent excitation of materials via ultrafast laser pulses can have interesting, observable dynamics in time-resolved photoemission measurements. The broad spectral width of ultrafast pump pulses can coherently excite multiple exciton…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Avinash Rustagi , Alexander F. Kemper

We present a novel theoretical approach to simulate spin, time and angular-resolved photoelectron spectroscopy (ARPES) from first principles that is applicable to surfaces, thin films, few layer systems, and low-dimensional nanostructures.…

Computational Physics · Physics 2017-01-03 Umberto De Giovannini , Hannes Hübener , Angel Rubio

Angle-resolved photoemission spectroscopy is the leading tool for studying the symmetry and structure of the order parameter in superconductors. The recent improvement of the technique made it possible to detect the superconducting energy…

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