Related papers: Exploring Two-dimensional Coherent Spectroscopy wi…
Electronic energy transfer in photosynthesis occurs over a range of time scales and under a variety of intermolecular coupling conditions. Recent work has shown that electronic coupling between chromophores can lead to coherent oscillations…
Dissipation and decoherence of quantum systems in thermal environments is important to various spectroscopies. It is generally believed that dissipation can broaden the line shape of spectroscopies, and thus stronger system-bath interaction…
Motivated by the recent experimental and theoretical progresses in the exploration of the effect of disorder in interacting system, we examine the effect of two types of correlated disorder, the quasi-periodic potential and speckle disorder…
The entanglement spectroscopy, initially introduced by Li and Haldane in the context of the fractional quantum Hall effects, has stimulated an extensive range of studies. The entanglement spectrum is the spectrum of the reduced density…
The electronic properties of two-dimensional (2D) materials depend sensitively on the underlying atomic arrangement down to the monolayer level. Here we present a novel strategy for the determination of the band gap and complex dielectric…
Unique optical properties of colloidal semiconductor quantum dots (QDs), arising from quantum mechanical confinement of charge within these structures, present a versatile testbed for the study of how high electric fields affect the…
We have presented the theory, implementation, and benchmark results for the one-electronic variant of spin-free exact two-component (SFX2C1e) linear response coupled cluster (LRCCSD) theory for static and dynamic polarizabilities of atoms…
For many real spin-glass materials, the Edwards-Anderson model with continuous-symmetry spins is more realistic than the rather better understood Ising variant. In principle, the nature of an occurring spin-glass phase in such systems might…
We propose phonon spectroscopy by electric measurements of the low-temperature conductance of coupled-quantum dots, specifically employing dephasing of the quantum electronic transport by the phonons. The setup we consider consists of a…
Recent work applying multidimentional coherent electronic spectroscopy at dilute samples in the gas phase is reviewed. The development of refined phase-cycling approaches with improved sensitivity has opened-up new opportunities to probe…
Two-dimensional electronic spectroscopy (2DES) has high spectral resolution and is a useful tool for studying atom dynamics. In this paper, we show a smallest unit of electromagnetically induced transparency (EIT) for 2DES, that is, a…
The photophysics of $\pi$-conjugated polymers has been of considerable interest over the last three decades because of their organic semiconductor properties. Primary photoexcitations, Frenkel excitons, can be probed optically by means of…
Observing constituent particles with fractional quantum numbers in confined and deconfined states is an interesting and challenging problem in quantum many-body physics. Here we further explore a computational scheme [Y. Tang and A. W.…
We numerically study quantum magnetism of ultra-cold alkali and alkaline-earth fermion systems with large hyperfine spin $F=3/2$, which are characterized by a generic $Sp(N)$ symmetry with N=4. The methods of exact diagonalization (ED) and…
The coherent two-dimensional (2D) electronic spectra with respect to the singlet fission (SF) process in organic molecular aggregates are simulated by the Davydov ansatz combined with the Frenkel-Dirac time-dependent variational algorithm.…
Spin noise spectroscopy is a promising technique for revealing the microscopic nature of spin dephasing processes in quantum dots. We compare the spin-noise in an ensemble of singly charged quantum dots calculated by two complementary…
Two-dimensional (2D) spectroscopy uses multiple electromagnetic pulses to infer the properties of a complex system. A paradigmatic class of target systems are molecular aggregates, for which one can obtain information on the eigenstates,…
By using the coupled cluster method (CCM) and the numerical exact diagonalization (ED) method, we investigated the properties of the one quasi-one-dimensional coupled spin triangles. The results of ED disclose that the system is in the…
We obtain an exact solution for the spectral function for one-dimensional Bose-Bose and Fermi- Fermi mixtures with strong repulsive interactions, valid in arbitrary confining potentials and at all frequency scales. For the case of harmonic…
Techniques for coherent multidimensional optical spectroscopy have been developed and utilised to understand many different processes, including energy transfer in photosynthesis and many-body effects in semiconductor nanostructures.…