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In this work we show the advantages of using the Coulomb-hole plus screened-exchange (COHSEX) approach in the calculation of potential energy surfaces. In particular, we demonstrate that, unlike perturbative $GW$ and partial self-consistent…

Chemical Physics · Physics 2021-06-14 J. Arjan Berger , Pierre-François Loos , Pina Romaniello

The GW approximation is widely used for reliable and accurate modeling of single-particle excitations. It also serves as a starting point for many theoretical methods, such as its use in the Bethe-Salpeter equation (BSE) and dynamical…

Computational Physics · Physics 2024-03-25 Weiwei Gao , Zhao Tang , Jijun Zhao , James R. Chelikowsky

An efficient implementation of the self-consistent GW method in the FlapwMBPT code (https://www.bnl.gov/cmpmsd/flapwmbpt/) is presented. It features the evaluation of polarizability and self-energy which scales linearly with respect to the…

Materials Science · Physics 2020-08-05 Andrey L. Kutepov

Common G$_0$W$_0$ implementations rely on numerical or analytical frequency integration to determine the G$_0$W$_0$ self-energy, which results in a variety of practical complications. Recently, we demonstrated an exact connection between…

Chemical Physics · Physics 2023-12-01 Johannes Tölle , Garnet Kin-Lic Chan

We present an approach for self-consistent calculations of the many-body Green function in transition metals. The distinguishing feature of our approach is the use of the one-site approximation and the self-consistent quasiparticle wave…

Strongly Correlated Electrons · Physics 2009-11-07 N. E. Zein , V. P. Antropov

For a three-electron system with finite-strength interactions confined to a one-dimensional harmonic trap, we solve the Schroedinger equation analytically to obtain the exact solutions, from which we construct explicitly the simultaneous…

Mesoscale and Nanoscale Physics · Physics 2018-11-14 Taichi Kosugi , Yu-ichiro Matsushita

Employing the $G_0W_0$ approximation of Hedin's $GW$ approach one can obtain quasi-particle energies of extended systems and molecules with good accuracy. However, for many materials, semi-local exchange-correlation functionals are…

Materials Science · Physics 2016-12-21 Ronaldo Rodrigues Pela , Ute Werner , Dmitrii Nabok , Claudia Draxl

We propose a second version of the van der Waals density functional (vdW-DF2) of Dion et al. [Phys. Rev. Lett. 92, 246401 (2004)], employing a more accurate semilocal exchange functional and the use of a large-N asymptote gradient…

Materials Science · Physics 2010-08-17 Kyuho Lee , Éamonn D. Murray , Lingzhu Kong , Bengt I. Lundqvist , David C. Langreth

The family of Green's function methods based on the $GW$ approximation has gained popularity in the electronic structure theory thanks to its accuracy in weakly correlated systems combined with its cost-effectiveness. Despite this,…

Chemical Physics · Physics 2023-08-31 Antoine Marie , Pierre-François Loos

Quasiparticle spectra of potentially half-metallic Co2MnSi and Co2FeSi Heusler compounds have been calculated within the one-shot GW approximation in an all-electron framework without adjustable parameters. For Co2FeSi the many-body…

Materials Science · Physics 2013-01-04 Markus Meinert , Christoph Friedrich , Günter Reiss , Stefan Blügel

The band gaps of a few selected semiconductors/insulators are obtained from the self-consistent solution of the Hedin's equations. Two different schemes to include the vertex corrections are studied: (i) the vertex function of the…

Strongly Correlated Electrons · Physics 2017-05-17 Andrey L. Kutepov

We have recently implemented a new version of the quasiparticle self-consistent GW (QSGW) method in the ecalj package released at http://github.com/tkotani/ecalj. Since the new version of the ecalj is numerically stable and accurate…

Materials Science · Physics 2016-04-20 Daiki Deguchi , Kazunori Sato , Hiori Kino , Takao Kotani

The $GW$-Bethe-Salpeter Equation (BSE) method is promising for calculating the low-lying excited states of molecular systems. So far, it has only been applied to rather small molecules, and in the commonly implemented diagonal…

Chemical Physics · Physics 2022-08-10 Arno Förster , Lucas Visscher

A quasi-two-dimensional (Q2D) electron liquid (EL) is formed at the interface of a semiconductor heterojunction. For an accurate characterization of the Q2D EL, many-body effects need to be taken into account beyond the random phase…

Condensed Matter · Physics 2009-10-28 C. Bulutay , M. Tomak

We investigate the effect of long-range Coulomb interaction on the quasiparticle properties and the dielectric function of clean three-dimensional Weyl semimetals at zero temperature using a functional renormalization group (FRG) approach.…

Strongly Correlated Electrons · Physics 2018-03-15 Anand Sharma , Arthur Scammell , Jan Krieg , Peter Kopietz

The Perdew-Zunger(PZ) self-interaction correction (SIC) was designed to correct the one-electron limit of any approximate density functional for the exchange-correlation (xc) energy, while yielding no correction to the exact functional.…

We present a complete prescription for the numerical calculation of surface Green's functions and self-energies of semi-infinite quasi-onedimensional systems. Our work extends the results of Sanvito et al. [1] generating a robust algorithm…

Materials Science · Physics 2007-12-11 Ivan Rungger , Stefano Sanvito

Just like the weakly interacting QED can support non-perturbative phenomena, like atoms, so can the weak and Higgs interactions. Especially, there are strong field-theoretical arguments that only bound states can be the (quasi-)asymptotic…

High Energy Physics - Lattice · Physics 2013-08-07 Axel Maas , Tajdar Mufti

Starting with Hedins equations, simple expressions for the irreducible self-energy are derived. The derivation with vertex effects included in the self-energy results in a number of terms beyond GW such as second-order screened exchange…

Computational Physics · Physics 2024-12-17 Brian Cunningham

The second-order Matsubara Green's function method (GF2) is a robust temperature dependent quantum chemistry approach, extending beyond the random-phase approximation. However, till now the scope of GF2 applications was quite limited as…

Chemical Physics · Physics 2017-09-20 Daniel Neuhauser , Roi Baer , Dominika Zgid