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In the interstellar medium (ISM), polycylic aromatic hydrocarbons (PAHs) are believed to be an important carbon reservoir, accounting for up to a quarter of all interstellar carbon in our galaxy. This makes the investigation of their…

Astrophysics of Galaxies · Physics 2025-06-23 Karina Sogomonyan , Malek Ben Khalifa , Phoebe Pierré , Jérôme Loreau

Among the numerous molecular systems found in the interstellar medium (ISM), vinyl cyanide is the first identified olephinic nitrile. While it has been observed in various sources, its detection in Sgr B2 is notable as the 2$_{11}$-2$_{12}$…

Astrophysics of Galaxies · Physics 2025-06-23 Karina Sogomonyan , Malek Ben Khalifa , Jérôme Loreau

Modeling of molecular emission from interstellar clouds requires the calculation of rates for excitation by collisions with the most abundant species. The present paper focuses on the calculation of rate coefficients for rotational…

Astrophysics of Galaxies · Physics 2015-05-18 E. Sarrasin , D. Ben Abdallah , M. Wernli , A. Faure , J. Cernicharo , F. Lique

The low temperature reaction between CN and benzene (C$_6$H$_6$) is of significant interest in the astrochemical community due to the recent detection of benzonitrile, the first aromatic molecule identified in the interstellar medium (ISM)…

Astrophysics of Galaxies · Physics 2020-03-25 Ilsa R. Cooke , Divita Gupta , Joseph P. Messinger , Ian R. Sims

Among all closed-shell species observed in molecular clouds, molecules with C$_{3v}$ symmetry play a crucial role, as their rotational spectroscopy allows them to behave as a gas thermometer. In the interstellar medium, methyl cyanide…

Astrophysics of Galaxies · Physics 2023-09-22 M. Ben Khalifa , P. J. Dagdigian , J. Loreau

Recent astronomical observations revealed an increasing molecular complexity in the interstellar medium through the detection of a series of large cyclic carbon species. To correctly interpret these detections, a complex analysis is…

Atomic and Molecular Clusters · Physics 2024-06-05 Sándor Demes , Cheikh Tidiane Bop , Malek Ben Khalifa , François Lique

A detailed interpretation of the detected emission lines of environments in which propyne (or methyl acetylene, CH$_3$CCH) is observed requires a knowledge of its collisional rate coefficients with the most abundant species in the…

Astrophysics of Galaxies · Physics 2024-02-28 M. Ben Khalifa , B. Darna , J. Loreau

Several nitrogen-bearing molecules, such as methyl cyanide (or acetonitrile, CH$_3$CN) and methyl isocyanide (CH$_3$NC) of interest here, have been observed in various astrophysical environments. The accurate modeling of their abundance…

Chemical Physics · Physics 2023-09-14 Malek Ben Khalifa , Paul J. Dagdigian , Jérôme Loreau

Chloronium (H$_2$Cl$^+$) is an important intermediate of Cl-chemistry in space. The accurate knowledge of its collisional properties allows a better interpretation of the corresponding observations in interstellar clouds and therefore a…

Chemical Physics · Physics 2024-12-31 Sándor Demes , Dariusz Kędziera , Alexandre Faure , François Lique

We report new results from quantum calculations of energy-transfer processes taking place in interstellar environments and involving two newly observed molecular species: C$_5$N$^-$ and C$_7$N$^-$ in collision with He atoms and the p-H$_2$…

Rates for rotational excitation of HC3N by collisions with He atoms and H2 molecules are computed for kinetic temperatures in the range 5-20K and 5-100K, respectively. These rates are obtained from extensive quantum and quasi-classical…

Chemical Physics · Physics 2009-11-13 Michael Wernli , Laurent Wiesenfeld , Alexandre Faure , Pierre Valiron

Collisional (de-)excitation of H$_{2}$ by helium plays an important role in the thermal balance and chemistry of various astrophysical environments, making accurate rate coefficients essential for the interpretation of observations of the…

Astrophysics of Galaxies · Physics 2024-05-15 Hubert Jóźwiak , Franck Thibault , Alexandra Viel , Piotr Wcisło , François Lique

Carbon monoxide is a simple molecule present in many astrophysical environments, and collisional excitation rate coefficients due to the dominant collision partners are necessary to accurately predict spectral line intensities and extract…

Astrophysics of Galaxies · Physics 2015-11-17 Kyle M. Walker , L. Song , B. H. Yang , G. C. Groenenboom , A. van der Avoird , N. Balakrishnan , R. C. Forrey , P. C. Stancil

In recent years, several aromatic molecules (benzene-based rings) have been detected in the cold molecular cloud TMC-1, with its CN-derivative, benzonitrile (c-C$_6$H$_5$CN), also identified in other nearby cold sources. However, observed…

Polycyclic aromatic hydrocarbons and polycyclic aromatic nitrogen heterocycles are thought to be widespread throughout the Universe, because these classes of molecules are probably responsible for the unidentified infrared bands, a set of…

Nitric oxide is an open-shell molecule abundantly detected in the interstellar medium. A precise modeling of its radiative and collisional processes opens the path to a precise estimate of its abundance. We present here the first rate…

Astrophysics of Galaxies · Physics 2022-05-11 M. Ben Khalifa , J. Loreau

Ammonia is one of the most widely observed molecules in space, and many observations are able to resolve the hyperfine structure due to the electric quadrupole moment of the nitrogen nucleus. The observed spectra often display anomalies in…

Astrophysics of Galaxies · Physics 2023-09-06 J. Loreau , A. Faure , F. Lique , S. Demes , P. J. Dagdigian

Benzonitrile (c-C6H5CN) has been recently detected in cold and dense regions of the interstellar medium (ISM), where it has been used as a signpost of a rich aromatic organic chemistry that might lead to the production of polycyclic…

Astrophysics of Galaxies · Physics 2022-12-07 Pavlo Maksyutenko , Rafael Martin-Domenech , Elettra Piacentino , Karin I. Oberg , Mahesh Rajappan

The first set of theoretical cross sections for propylene oxide (CH3CHCH2O) colliding with cold He atoms has been obtained at the full quantum level using a high-accuracy potential energy surface. By scaling the collision reduced mass,…

Astrophysics of Galaxies · Physics 2022-02-16 K. Dzenis , A. Faure , B. A. McGuire , A. J. Remijan , P. J. Dagdigian , C. Rist , R. Dawes , E. Quintas-Sanchez , F. Lique , M. Hochlaf

New calculations for rotational excitation of cyanoacetylene by collisions with hydrogen molecules are performed to include the lowest 38 rotational levels of HC3N and kinetic temperatures to 300 K. Calculations are based on the interaction…

Astrophysics of Galaxies · Physics 2016-06-15 A. Faure , F. Lique , L. Wiesenfeld
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