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In the field of photocatalytic water splitting, no current studies have explicitly investigated the coexistence of multiple band-edge alignments in two-dimensional (2D) materials with intrinsic electric fields. In this Letter, we designed…

Materials Science · Physics 2024-09-17 Zhi-Qiang Wen , Qiu Yang , Shu-Hao Cao , Zhao-Yi Zeng , Hua-Yun Geng , Xiang-Rong Chen

A caloritronic device setup is proposed that harnesses the intrinsic spin-valley locking of two-dimensional honeycomb lattices with graphene-like valleys, for instance, silicene and stanene. Combining first-principles and analytic…

Materials Science · Physics 2020-03-18 Parijat Sengupta , Shaloo Rakheja

The illumination of a single-layer transition metal dichalcogenide with an elliptically-polarized light beam is shown to give rise to a differential rate of inter-band carrier excitation between the valence and conduction states around the…

Materials Science · Physics 2017-03-28 Parijat Sengupta , Yaohua Tan , Dmitris Pavlidis , Junxia Shi

Valley, as a new degree of freedom for electrons, has drawn considerable attention due to its significant potential for encoding and storing information. Lifting the energy degeneracy to achieve valley polarization is necessary for…

Materials Science · Physics 2020-03-11 Pei Zhaos , Yandong Ma , Hao Wang , Baibiao Huang , Liangzhi Kou , Ying Dai

Two-dimensional (2D) noncentrosymmetric systems offer potential opportunities for exploiting the valley degrees of freedom for advanced information processing, owing to non-zero Berry curvature. However, such valley polarization in 2D…

Materials Science · Physics 2023-10-10 Souren Adhikary , Sudipta Dutta

Two-dimensional (2D) materials may have potential applications in thermoelectric devices. In this work, we systematically investigate the thermoelectric properties of orthorhombic group IV-VI monolayers $\mathrm{AB}$ (A=Ge and Sn; B=S and…

Materials Science · Physics 2017-02-01 San-Dong Guo

In a number of widely-studied materials, such as Si, AlAs, Bi, graphene, MoS2, and many transition metal dichalcogenide monolayers, electrons acquire an additional, spin-like degree of freedom at the degenerate conduction band minima, also…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 M. A. Mueed , Md. Shafayat Hossain , I. Jo , L. N. Pfeiffer , K. W. West , K. W. Baldwin , M. Shayegan

In crystals, energy band extrema in momentum space can be identified by their valley index. The internal quantum degree of freedom associated with valley pseudospin indices can act as a useful information carrier analogous to electronic…

Opto-spintronics is an emerging field where ultra-thin magnetic-semiconductors having high spin-valley coupling play an important role. Here, we demonstrate substitutional vanadium (V) doping in MoS$_2$ lattice in different extent, leading…

Valley degrees of freedom offer a potential resource for quantum information processing if they can be effectively controlled. We discuss an optical approach to this problem in which intense light breaks electronic symmetries of a…

Mesoscale and Nanoscale Physics · Physics 2016-01-11 Arijit Kundu , H. A. Fertig , Babak Seradjeh

Valley-based electronics, known as valleytronics, is one of the keys to break through to a new stage of electronics. The valley degree of freedom is ubiquitous in the honeycomb lattice system. The honeycomb lattice structure of silicon…

Mesoscale and Nanoscale Physics · Physics 2013-04-23 Motohiko Ezawa

The strong light matter interaction and the valley selective optical selection rules make monolayer (ML) MoS2 an exciting 2D material for fundamental physics and optoelectronics applications. But so far optical transition linewidths even at…

In recent years, novel materials supporting in-plane anisotropic polaritons have attracted a lot of research interest due to their capability of shaping nanoscale field distributions and controlling nanophotonic energy flows. Here we report…

Optics · Physics 2023-01-30 Yilong Luan , Hamidreza Zobeiri , Xinwei Wang , Eli Sutter , Peter Sutter , Zhe Fei

A monolayer of a transition metal dichalcogenide (TMD) such as WSe$_2$ is a two-dimensional (2D) direct band-gap valley-semiconductor having an effective Honeycomb lattice structure with broken inversion symmetry. The inequivalent valleys…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Ajit Srivastava , Meinrad Sidler , Adrien V. Allain , Dominik S. Lembke , Andras Kis , Atac Imamoglu

Single layers of transition metal dichalcogenides (TMDs) are direct gap semiconductors with nondegenerate valley indices. An intriguing possibility for these materials is the use of their valley index as an alternate state variable. Several…

Transition-metal dichalcogenides can be easily produced as atomically thin sheets, exhibiting the possibility to optically polarize and read out the valley pseudospin of extremely stable excitonic quasiparticles present in these 2D…

Sixfold-degenerate valleys in Si have attracted considerable attention for valleytronics application. Using optical pump-terahertz (THz) probe spectroscopy, we study the dynamics of valley polarization in bulk Si(001) at room temperature.…

Photostriction is predicted for SnS and SnSe monolayers, two-dimensional ferroelectrics with rectangular unit cells (the lattice vector $\mathbf{a}_1$ is larger than $\mathbf{a}_2$) and an intrinsic dipole moment parallel to $\mathbf{a}_1$.…

Mesoscale and Nanoscale Physics · Physics 2017-06-07 Raad Haleoot , Charles Paillard , Mehrshad Mehboudi , Bin Xu , L. Bellaiche , Salvador Barraza-Lopez

We develop a microscopic theory for nonlinear optical response of moir\'e exciton-polaritons in bilayers of transition metal dichalcogenides (TMDs). Our theory allows to study the tunnel-coupled intralayer and interlayer excitonic modes for…

Mesoscale and Nanoscale Physics · Physics 2025-07-16 Kok Wee Song , Oleksandr Kyriienko

The rhombohedral (r) polytypes of transition metal dichalcogenides (TMDs) constitute a novel class of two-dimensional ferroelectric materials, where lateral shifts between parallel layers induce reversible out-of-plane polarization. This…