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We develop a framework to describe collective buckling in metal-organic frameworks (MOFs). Starting from the microscopic structure of a single organic linker, we define a buckling coordinate governed by an effective double-well potential.…

Statistical Mechanics · Physics 2026-03-27 Nico Hahn , Lars Öhrström , R. Matthias Geilhufe

The search for sustainable alternatives to established materials is a sensitive topic in materials science. Due to their unique structural and physical characteristics, the composition of metal-organic frameworks (MOFs) can be tuned by the…

Understanding how structural flexibility affects the properties of metal-organic frameworks (MOFs) is crucial for the design of better MOFs for targeted applications. Flexible MOFs can be studied with molecular dynamics simulations, whose…

Materials Science · Physics 2024-05-13 Abhishek Sharma , Stefano Sanvito

The storage of hydrogen gas (H$_2$) has presented a significant challenge that has hindered its use as a fuel source for transportation. To meet the Department of Energy's ambitious goals of achieving $50$ g L$^{-1}$ volumetric and $6.5$ wt…

Chemical Physics · Physics 2023-06-21 Marcus Djokic , Jose L. Mendoza-Cortes

Long-lived emissive materials based on room temperature phosphorescence (RTP) and thermally activated delayed fluorescence (TADF) are considered as the cornerstone of the development of optical sensors, security systems and solid-state…

Materials Science · Physics 2021-10-26 Mario Gutiérrez , Cristina Martín , Johan Hofkens , Jin-Chong Tan

By combining metal nodes with organic linkers we can potentially synthesize millions of possible metal organic frameworks (MOFs). At present, we have libraries of over ten thousand synthesized materials and millions of in-silico predicted…

Materials Science · Physics 2020-06-12 Kevin Maik Jablonka , Daniele Ongari , Seyed Mohamad Moosavi , Berend Smit

Due the alarming rate of climate change, the implementation of efficient CO$_2$ capture has become crucial. This project aims to create an algorithm that predicts the uptake of CO$_2$ adsorbing Metal-Organic Frameworks (MOFs) by using…

Machine Learning · Computer Science 2021-10-13 Mahati Manda

Mofasa is an all-atom latent diffusion model with state-of-the-art performance for generating Metal-Organic Frameworks (MOFs). These are highly porous crystalline materials used to harvest water from desert air, capture carbon dioxide,…

We combine infrared spectroscopy, nano-indentation measurements, and \emph{ab initio} simulations to study the evolution of structural, elastic, thermal, and electronic responses of the metal organic framework MOF-74-Zn when loaded with…

Materials Science · Physics 2014-12-23 Pieremanuele Canepa , Kui Tan , Yingjie Du , Hongbing Lu , Yves J. Chabal , T. Thonhauser

The properties of metal-organic frameworks (MOFs) are expected to be sensitive to external pressures because of their inherently flexible structures. Although pressure-driven structural transitions have been intensively studied, the…

Materials Science · Physics 2025-03-10 Shuang Liu , Na Su , Huixia Fu , Yan Liu , Young Sun

The presence of open active metal sites in Metal-Organic Frameworks (MOFs) exhibit higher catalytic activity. However, rational accomplishment of MOFs in heterogeneous catalysis is limited due to coordination bonds. Recently balanced…

The electronic properties of interfaces between two different solids can differ strikingly from those of the constituent materials. For instance, metallic conductivity, and even superconductivity, have been recently discovered at interfaces…

Materials Science · Physics 2009-11-13 H. Dias Alves , A. S. Molinari , H. Xie , A. F. Morpurgo

This study leverages density function theory (DFT) accompanied with Boltzmann transport equation approaches to investigate the electronic mobility as a function of inorganic substitution and functionalization in a thermally stable UiO-66…

Materials Science · Physics 2018-05-09 Terence D. Musho , Alhassan S. Yasin

Metal-organic frameworks (MOFs) have emerged as promising materials for various applications due to their unique structural properties and versatile functionalities. This study presents a comprehensive investigation of machine learning…

Machine Learning · Computer Science 2025-07-08 Zhuo Zheng , Keyan Liu , Xiyuan Zhu

Correlated electron systems are among the centerpieces of modern condensed matter sciences, where many interesting physical phenomena, such as metal-insulator transition and high-Tc superconductivity appear. Recent efforts have been focused…

Strongly Correlated Electrons · Physics 2013-08-05 You Zhou , Shriram Ramanathan

We study the energetic stability and structural features of bimetallic metal-organic frameworks. Such heterometallic MOFs, which can result from partial substitutions between two types of cations, can have specific physical or chemical…

Materials Science · Physics 2019-04-22 Fabien Trousselet , Aurélien Archereau , Anne Boutin , François-Xavier Coudert

Designing metal-organic frameworks (MOFs) synthesis protocols is currently largely driven by trial-and-error, since we lack fundamental understanding of the molecular level mechanisms that underlie their self-assembly processes. Previous…

Materials Science · Physics 2025-12-04 Sahar Andarzi Gargari , Emilio Méndez , Rocio Semino

Na-ion batteries (NIBs) are increasingly looked at as a viable alternative to Li-ion batteries due to the abundance, low cost, and thermal stability of Na-based systems. To improve the practical utilization of NIBs in applications, it is…

Materials Science · Physics 2024-12-17 Debolina Deb , Gopalakrishnan Sai Gautam

Through rational chemical design, and thanks to the hybrid nature of metal-organic frameworks (MOFs), it is possible to prepare molecule-based 2D magnetic materials stable at ambient conditions. Here, we illustrate the versatility of this…

Ultra-sensitive and highly selective iodine gas sensors play a crucial role during the nuclear radiation leak for a timely detection and mitigation of pollution, ensuring the safety of a vast number of operators and subsequent integrity of…

Instrumentation and Detectors · Physics 2022-02-23 Arun S. Babal , Samraj Mollick , Waqas Kamal , Steve Elston , Alfonso A. Castrejón-Pita , Stephen M. Morris , Jin-Chong Tan
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