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We present a study of mono(benzene)TM and bis(benzene)TM systems, where TM={Mo,W}. We calculate the binding energies by quantum Monte Carlo (QMC) approaches and compare the results with other methods and available experiments. The orbitals…

Chemical Physics · Physics 2017-12-01 M. Chandler Bennett , Adem H. Kulahlioglu , Lubos Mitas

We develop a formalism to directly evaluate the matrix of force constants within a Quantum Monte Carlo calculation. We utilize the matrix of force constants to accurately relax the positions of atoms in molecules and determine their…

Computational Physics · Physics 2020-04-06 Yu Yang Fredrik Liu , Bartholomew Andrews , Gareth J. Conduit

We explore correlated electron states in harmonically confined few-electron quantum dots in an external magnetic field by the path-integral Monte Carlo method for a wide range of the field and the Coulomb interaction strength. Using the…

Strongly Correlated Electrons · Physics 2020-01-07 Csaba Tőke , Tamás Haidekker Galambos

Metropolis Monte Carlo simulation is a powerful tool for studying the equilibrium properties of matter. In complex condensed-phase systems, however, it is difficult to design Monte Carlo moves with high acceptance probabilities that also…

Statistical Mechanics · Physics 2014-05-27 Jerome P. Nilmeier , Gavin E. Crooks , David D. L. Minh , John D. Chodera

Markov Chain Monte Carlo inference of target posterior distributions in machine learning is predominately conducted via Hamiltonian Monte Carlo and its variants. This is due to Hamiltonian Monte Carlo based samplers ability to suppress…

Machine Learning · Statistics 2021-07-06 Wilson Tsakane Mongwe , Rendani Mbuvha , Tshilidzi Marwala

Computer simulations of structure formation in network forming materials (such as amorphous semiconductors, glasses, or fluids containing hydrogen bonds) are challenging. The problem is that large structural changes in the network topology…

Statistical Mechanics · Physics 2015-06-18 Richard Vink

The energy per particle of zero-temperature neutron matter is investigated, with particular emphasis on the role of the $\vec L\cdot\vec S$ interaction. An analysis of the importance of explicit spin--orbit correlations in the description…

Nuclear Theory · Physics 2009-11-10 L. Brualla , S. Fantoni , A. Sarsa , K. E Schmidt , S. A. Vitiello

Calculations of the binding energy of the transition metal oxide molecules TiO and MnO are presented, using a recently developed phaseless auxiliary field quantum Monte Carlo approach. This method maps the interacting many-body problem onto…

Strongly Correlated Electrons · Physics 2007-05-23 W. A. Al-Saidi , Henry Krakauer , Shiwei Zhang

Spin-orbit torque manifested as an accumulated spin-polarized moment at nonmagnetic normal metal, and ferromagnet interfaces is a promising magnetization switching mechanism for spintronic devices. To fully exploit this in practice,…

In nuclear fusion and fission, fluctuation and dissipation arise due to the coupling of collective degrees of freedom with internal excitations. Close to the barrier, both quantum, statistical and non-Markovian effects are expected to be…

Nuclear Theory · Physics 2010-04-06 G. Hupin , D. Lacroix

In this work, we test a recently developed method to enhance classical auxiliary-field quantum Monte Carlo (AFQMC) calculations with quantum computers against examples from chemistry and material science, representatives of classes of…

Electron-electron (e-e) interactions assume a cardinal role in solid-state physics. Quantifying the e-e scattering length is hence critical. In this paper we show that the mesoscopic phenomenon of transverse magnetic focusing (TMF) in…

Mesoscale and Nanoscale Physics · Physics 2022-07-07 Adbhut Gupta , Jean J. Heremans , Gitansh Kataria , Mani Chandra , Saeed Fallahi , Geoffrey C. Gardner , Michael J. Manfra

We explore the applicability of the transcorrelated method to the elements in the second row of the periodic table. We use transcorrelated Hamiltonians in conjunction with full configuration interaction quantum Monte Carlo and coupled…

Describing correlated electron systems near phase transitions has been a major challenge in computational condensed-matter physics. In this paper, we apply highly accurate fixed node quantum Monte Carlo techniques, which directly work with…

Strongly Correlated Electrons · Physics 2018-01-10 Li Chen , Lucas K. Wagner

We study the nearest-neighbor spin-ice model subjected to a magnetic field applied along the global [111] and [110] directions, focusing on the role of sample geometry in stabilizing topological phase transitions. While no Kasteleyn…

Statistical Mechanics · Physics 2026-04-30 R. A. Borzi , E. S. Loscar , S. A. Grigera

Spin-ordered states close to metal-insulator transitions are poorly understood theoretically and challenging to probe in experiments. Here, we propose that the quantum twisting microscope, which provides direct access to the energy-momentum…

Strongly Correlated Electrons · Physics 2024-07-11 Fabian Pichler , Wilhelm Kadow , Clemens Kuhlenkamp , Michael Knap

Performing Monte Carlo simulations we study the temperature dependent self--organization of magnetic moments coupled to itinerant electrons in a finite--size one--dimensional nanostructure proximitized to a superconducting reservoir. At low…

Mesoscale and Nanoscale Physics · Physics 2019-07-03 Anna Gorczyca-Goraj , Tadeusz Domanski , Maciej M. Maska

Using fermionic representation of spin degrees of freedom within the Popov-Fedotov approach we develop an algorithm for Monte Carlo sampling of skeleton Feynman diagrams for Heisenberg type models. Our scheme works without modifications for…

Strongly Correlated Electrons · Physics 2013-02-07 Sergey Kulagin , Nikolay Prokof'ev , Oleg Starykh , Boris Svistunov , Christopher N. Varney

We report diffusion Monte Carlo (DMC) calculations on MgO in the rock-salt and CsCl structures. The calculations are based on Hartree-Fock pseudopotentials, with the single-particle orbitals entering the correlated wave function being…

Strongly Correlated Electrons · Physics 2016-08-16 D. Alfè , M. Alfredsson , J. Brodholt , M. J. Gillan M. D. Towler , R. J. Needs

We derive an automatic procedure for generating a set of highly localized, non-orthogonal orbitals for linear scaling quantum Monte Carlo calculations. We demonstrate the advantage of these orbitals in calculations of the total energy of…

Materials Science · Physics 2007-05-23 F. A. Reboredo , A. J. Williamson