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Magnon gap excitations selectively coupled to phonon modes have been studied in FePSe$_3$ layered antiferromagnet with magneto-Raman scattering experiments performed at different temperatures. The bare magnon excitation in this material has…

We report on magneto-optical studies of the quasi-two-dimensional van der Waals antiferromagnet FePS$_3$. Our measurements reveal an excitation that closely resembles the antiferromagnetic resonance mode typical of easy-axis…

Recently it was discovered that van der Waals-bonded magnetic materials retain long range magnetic ordering down to a single layer, opening many avenues in fundamental physics and potential applications of these fascinating materials. One…

Magneto-spectroscopy methods have been employed to study the zero-wavevector magnon excitations in MnPSe$_3$. Experiments carried out as a function of temperature and the applied magnetic field show that two low-energy magnon branches of…

The hybridization of magnons (spin waves) with phonons, if sufficiently strong and comprising long wavelength excitations, may offer a new playground when manipulating the magnetically ordered systems with light. Applying a magnetic field…

Van der Waals (vdW) magnets are an ideal platform for tailoring two-dimensional (2D) magnetism with immense potential for spintronics applications and are intensively investigated. However, little is known about the microscopic origin of…

Recent development in two-dimensional (2D) magnetic materials have motivated the search for new van der Waals magnetic materials, especially Ising-type magnets with strong magnetic anisotropy. Fe-based MPX3 (M = transition metal, X =…

Antiferromagnetic van der Waals family $\rm \textit{M}P\textit{X}_{3}\ (M=Fe,\ Mn,\ Co,\text{ and}\ Ni; X=S\text{ and}\ Se)$ have attracted significant research attention due to the possibility of realizing long-range magnetic order down to…

Strongly Correlated Electrons · Physics 2024-06-11 Junbo Liao , Zhentao Huang , Yanyan Shangguan , Bo Zhang , Shufan Cheng , Hao Xu , Ryoichi Kajimoto , Kazuya Kamazawa , Song Bao , Jinsheng Wen

Longitudinal magnons are a distinct type of multipolar excitations in magnetic materials with large spins $S\ge 1$ and strong easy-axis anisotropy. These excitations have angular momentum $S^z = \pm 2S$ and can be viewed as a propagating…

Strongly Correlated Electrons · Physics 2026-02-20 A. El Mendili , T. Ziman , M. E. Zhitomirsky

Antiferromagnetic FePS3 has recently gained significant interest in its potential applications in spin-related devices. Here, we show that in-plane structural anisotropy has a major impact in shaping the optical responses of FePS3…

We use elastic and inelastic neutron scattering (INS) to study the antiferromagnetic (AF) phase transitions and spin excitations in the two-dimensional (2D) zig-zag antiferromagnet FePSe$_3$. By determining the magnetic order parameter…

Strongly Correlated Electrons · Physics 2024-02-28 Lebing Chen , Xiaokun Teng , Ding Hu , Feng Ye , Garrett E. Granroth , Ming Yi , Jae-Ho Chung , Robert J. Birgeneau , Pengcheng Dai

We combine polarized infrared magneto-transmission and Faraday angle rotation measurements to map the collective excitations of the van der Waals antiferromagnet FePS$_3$. Below the N\'{e}el temperature ($T_\mathrm{N} \approx 118$ K), the…

Strongly Correlated Electrons · Physics 2025-08-21 Kartik Panda , Itzik Kapon , Dumitru Dumcenco , Dirk van der Marel , Alexey Kuzmenko , Nimrod Bachar

We report a detailed high-field/high-frequency ferromagnetic resonance (HF-FMR) study of low-energy magnon excitations in the van der Waals ferromagnet Fe$_3$GeTe$_2$. At 2 K, the field dependence of the magnon branches is well described by…

Strongly Correlated Electrons · Physics 2025-07-22 Birte Beier , Erik Walendy , Jan Arneth , Eva Brücher , Reinhard K. Kremer , Rüdiger Klingeler

Antiferromagnetic (AFM) FePS3 has gained significant interest recently for its potential applications in spin-related devices. A single layer is comprised of a honeycomb network, stabilized by long-range spin-exchange interactions, with a…

Emergent cooperative motions of individual degrees of freedom, i.e. collective excitations, govern the low-energy response of system ground states under external stimulations and play essential roles for understanding many-body phenomena in…

Magnetic layered materials have emerged recently as promising systems to introduce magnetism in structures based on two-dimensional (2D) materials and to investigate exotic magnetic ground states in the 2D limit. In this work, we apply high…

We report results of 57Fe Mossbauer and 31P NMR studies of a phosphide FeP powder sample performed in a wide temperature range including the point (TN ~ 120 K) of magnetic phase transitions. The 57Fe Mossbauer spectra at low temperatures T…

Layered van-der-Waals 2D magnetic materials are of great interest in fundamental condensed-matter physics research, as well as for potential applications in spintronics and device physics. We present neutron powder diffraction data using…

Optical magneto-spectroscopy methods (Raman scattering, far-infrared transmission, and photoluminescence) have been applied to investigate the properties of the NiPS3 semiconducting antiferromagnet. The fundamental magnon gap excitation in…

Mesoscale and Nanoscale Physics · Physics 2023-06-14 Dipankar Jana , P. Kapuscinski , I. Mohelsky , D. Vaclavkova , I. Breslavetz , M. Orlita , C. Faugeras , M. Potemski

Magnetic 2D materials enable novel tuning options of magnetism. As an example, the van der Waals material FePS3, a zigzag-type intralayer antiferromagnet, exhibits very strong magnetoelastic coupling due to the different bond lengths along…

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