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Related papers: Hyperelastic swelling of stiff hydrogels

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Hydrogels of semiflexible biopolymers such as collagen have been shown to contract axially under shear strain, in contrast to the axial dilation observed for most elastic materials. Recent work has shown that this behavior can be understood…

Soft Condensed Matter · Physics 2019-05-13 Jordan Shivers , Jingchen Feng , Abhinav Sharma , Fred C. MacKintosh

\textbf{Background} Hydrogels are crosslinked polymer networks that can absorb and retain a large fraction of liquid. Near a critical sliding velocity, hydrogels pressed against smooth surfaces exhibit time-dependent frictional behavior…

Soft Condensed Matter · Physics 2021-01-13 Brady Wu , Joshua Méndez Harper , Justin C. Burton

From pasta to biological tissues to contact lenses, gel and gel-like materials inherently soften as they swell with water. In dry, low-relative-humidity environments, these materials stiffen as they de-swell with water. Here, we use…

Soft Condensed Matter · Physics 2021-09-29 Yiwei Gao , Nicholas K. K. Chai , Negin Garakani , Sujit S. Datta , H. Jeremy Cho

Biopolymer gels such as fibrin and collagen networks are known to develop tensile axial stress when subject to torsion. This negative normal stress is opposite to the classical Poynting effect observed for most elastic solids including…

Soft Condensed Matter · Physics 2018-04-04 Mahsa Vahabi , Bart E. Vos , Henri C. G. de Cagny , Daniel Bonn , Gijsje H. Koenderink , F. C. MacKintosh

Hydrogel consists of a crosslinked polymer matrix imbibed with a solvent such as water at volume fractions that can exceed 90\%. They are important in many scientific and engineering applications due to their tunable physiochemical…

Soft Condensed Matter · Physics 2020-06-11 Nicholas L. Cuccia , Suraj Pothineni , Brady Wu , Joshua Méndez-Harper , Justin C. Burton

Soft living tissues like cartilage can be considered as biphasic materials comprised of a fibrous complex biopolymer network and a viscous background liquid. Here, we show by a combination of experiment and theoretical analysis that both…

Soft Condensed Matter · Physics 2019-10-02 Melle T. J. J. M. Punter , Bart E. Vos , Bela M. Mulder , Gijsje H. Koenderink

Two types of high-strength composite hydrogels possessing the structure of interpenetrating polymer networks were synthesized via free-radical polymerization of acrylamide carried out straight within the matrix of plant or bacterial…

Chemical Physics · Physics 2019-04-02 Alexander Buyanov , Iosif Gofman , Natalya Saprykina

When sheared, most elastic solids such as metals, rubbers and polymer hydrogels dilate in the direction perpendicular to the shear plane. This well-known behaviour known as the Poynting effect is characterized by a positive normal stress.…

The deposition of droplets onto a swollen polymer network induces the formation of a wetting ridge at the contact line. Current models typically consider either viscoelastic effects or poroelastic effects, while polymeric gels often exhibit…

Soft Condensed Matter · Physics 2025-05-27 B. X. Zheng , T. S. Chan , E. H. van Brummelen , J. H. Snoeijer

It is established that the mechanical properties of hydrogels control the fate of (stem) cells. However, despite its importance, a one-to-one correspondence between gels' stiffness and cell behaviour is still missing from literature. In…

We present theoretical and experimental studies of the elastic response of fibrous networks subjected to uniaxial strain. Uniaxial compression or extension is applied to extracellular networks of fibrin and collagen using a shear rheometer…

Polymer gels are comprised of a three-dimensional, cross-linked network that can typically withstand the mechanical deformation associated with both swelling and de-swelling. Thus, gels can be designed with smart behaviors that require both…

Soft Condensed Matter · Physics 2024-06-24 Alyssa VanZanten , Shih-Yuan Chen , Michelle M. Driscoll , Caroline R. Szczepanski

From microactuators to biological tissues, non-porous materials with the ability to strongly expand when in contact with a solvent are ubiquitous. Consequently, the swelling of polymer systems such as hydrogel has received recently much…

Soft Condensed Matter · Physics 2024-11-04 George T. Fortune , Merlin A. Etzold , Julien R. Landel , Stuart B. Dalziel

Soft biological tissues exhibit a remarkable resilience to large mechanical loads, a property which is associated with the strain stiffening capability of the biopolymer networks that structurally support the tissues. Yet, recent studies…

Soft Condensed Matter · Physics 2024-03-19 Jake Song , Elad Deiss-Yehiely , Serra Yesilata , Gareth H. McKinley

In this work, we investigate the transient rheological behavior of two soft glassy materials: a clay dispersion and a silica gel, emphasizing their unconventional shear stress build-up behavior under conditions of constant imposed strain.…

Soft Condensed Matter · Physics 2025-04-02 Vivek Kumar , Gareth H McKinley , Yogesh M Joshi

Hydrogels have had a profound impact in the fields of tissue engineering, drug delivery, and materials science as a whole. Due to the network architecture of these materials, imbibement with water often results in uniform swelling and…

Swelling is a volumetric-growth process in which a porous material expands by spontaneous imbibition of additional pore fluid. Swelling is distinct from other growth processes in that it is inherently poromechanical: Local expansion of the…

Soft Condensed Matter · Physics 2025-05-13 Thibault Bertrand , Jorge Peixinho , Shomeek Mukhopadhyay , Christopher W. MacMinn

Understanding surface mechanics of soft solids, such as soft polymeric gels, is crucial in many engineering processes, such as dynamic wetting and adhesive failure. In these situations, a combination of capillary and elastic forces drives…

Soft Condensed Matter · Physics 2020-12-02 Qin Xu , Lawrence A. Wilen , Katharine E. Jensen , Robert W. Style , Eric R. Dufresne

Hydrogels are increasingly recognized as a versatile platform for applications spanning from tissue engineering to soft robotics or flexible electronics. Recent efforts have focused on enhancing and tailoring their mechanical performance to…

Soft Condensed Matter · Physics 2025-12-29 Agniva Dutta , Valeriy V. Ginzburg , Gleb Vasilyev , Eyal Zussman

Hybrid double-network hydrogels are a class of material that comprise transiently and permanently crosslinked polymer networks and exhibit an enhanced toughness that is believed to be governed by the yielding of the transient polymer…

Soft Condensed Matter · Physics 2024-09-10 Vinay Kopnar , Adam O'Connell , Natasha Shirshova , Anders Aufderhorst-Roberts
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