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The spin-orbit interaction (SOI) of light generated by tight focusing in optical tweezers has been regularly employed in generating angular momentum - both spin and orbital - in trapped mesoscopic particles. Specifically, the transverse…

Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To…

Electronic states in two-dimensional layered materials can exhibit a remarkable variety of correlated phases including Wigner-crystals, Mott insulators, charge density waves, and superconductivity. Recent experimental and theoretical…

Mesoscale and Nanoscale Physics · Physics 2021-08-16 Kai Hao , Robert Shreiner , Alexander A. High

We performed spin-polarized density functional calculations of lanthanide-series (Ln) iron oxypnictides LnFeAsO (Ln=La, Ce, Pr, Nd, Sm, and Gd) with constrained Fe magnetic moments, finding that in-plane dxy and out-of-plane dyz orbital…

Superconductivity · Physics 2013-12-30 Hyungju Oh , Donghan Shin , Hyoung Joon Choi

By using intense coherent electromagnetic radiation, it may be possible to manipulate the properties of quantum materials very quickly, or even induce new and potentially useful phases that are absent in equilibrium. For instance, ultrafast…

Strongly Correlated Electrons · Physics 2023-03-30 Jonathan B. Curtis , Ankit Disa , Michael Fechner , Andrea Cavalleri , Prineha Narang

We have imaged magnetization textures of permalloy films patterned into Penrose P2 tilings (P2T) using scanning electron microscopy with polarization analysis (SEMPA). P2T film segments have near-uniform, bipolar magnetization, similar to…

Mesoscale and Nanoscale Physics · Physics 2015-01-13 V. S. Bhat , A. Balk , B. Farmer , E. Teipel , N. Smith , J. Unguris , J. T. Hastings , L. E. De Long

We use single-cycle THz fields and the femtosecond magneto-optical Kerr effect to respectively excite and probe the magnetization dynamics in two thin-film ferromagnets with different lattice structure: crystalline Fe and amorphous CoFeB.…

Materials Science · Physics 2016-08-24 S. Bonetti , M. C. Hoffmann , M. -J. Sher , Z. Chen , S. -H. Yang , M. Samant , S. S. P. Parkin , H. A. Dürr

The coupling of laser light to matter can exert sub-cycle coherent control over material properties, with optically induced currents and magnetism shown to be controllable on ultrafast femtosecond time scales. Here, by employing laser light…

Optics · Physics 2024-06-19 Q. Z. Li , S. Shallcross , J. K. Dewhurst , S. Sharma , P. Elliott

We introduce a spin-orbit coupling scheme, where a retro-reflected laser beam selectively diffracts two spin components in opposite directions. Spin sensitivity is provided by sweeping through a magnetic-field sensitive transition while…

We report on an element- and time-resolved investigation of femtosecond laser induced ultrafast dynamics of 3d and 4f spins in a ferrimagnetic Co80Dy20 alloy as a function of temperature. We observe an increase of the Co3d characteristic…

We investigate the non-resonant all-optical switching of magnetization. We treat the inverse Faraday effect (IFE) theoretically in terms of the spin-selective optical Stark effect for linearly or circularly polarized light. In the dilute…

Mesoscale and Nanoscale Physics · Physics 2013-08-20 Alireza Qaiumzadeh , Gerrit E. W. Bauer , Arne Brataas

Ferrimagnets containing several partially compensated magnetic sublattices are considered the most promising materials for all-optical data storage and for ultrafast communications based on spin waves. There are two magnetic phases of the…

Ferrimagnets (FIMs) can function as high-frequency antiferromagnets while being easy to detect as ferromagnets, offering unique opportunities for ultrafast device applications. While the physical behavior of FIMs near the compensation point…

Mesoscale and Nanoscale Physics · Physics 2022-02-09 Mingda Guo , Hantao Zhang , Ran Cheng

Altermagnetism (AM), a collinear magnetic phase with momentum-dependent spin splitting, is a promising candidate for strong magnetoelectric coupling. However, realizing direct and tunable coupling between ferroelectricity (FE) and AM within…

Materials Science · Physics 2026-05-07 Tao Yao , Quan Shen , Wenhu Liao , Jianing Tan , Jiansheng Dong

Understanding ultrafast magnetization dynamics on the microscopic level is of strong current interest due to the potential for applications in information storage. In recent years, the spin-lattice coupling has been recognized to be…

Manipulation of the intersublattice interaction strengh (JRE-TM) in rare earth (RE)-transition metal (TM) alloys is a key issue to understand how efficiently the laser-induced angular momentum transfers from 3d to 4f spins and to have a…

Materials Science · Physics 2021-01-01 Y. Ren , L. L. Zhang , X. D. He , G. J. Wu , J. W. Gao , P. Ran , L. Z. Dan , T. Wang , X. W. Zhou , Z. Liu , J. Y. Xie , Q. Y. Jin , Zongzhi Zhang

Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

Strongly Correlated Electrons · Physics 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

High-resolution angle-resolved photoelectron spectroscopy is used to examine the electronic band structure of FeTe$_{0.5}$Se$_{0.5}$ near the Brillouin zone center. A consistent separation of the $\alpha_{1}$ and $\alpha_{2}$ bands is…

Strongly Correlated Electrons · Physics 2016-06-14 P. D. Johnson , H. -B. Yang , J. D. Rameau , G. D. Gu , Z. -H. Pan , T. Valla , M. Weinert , A. V. Fedorov

The interaction between light's angular momentum (AM) and material systems has unlocked new avenues in structured photonics, including in magneto-optical (MO) materials. While spin angular momentum (SAM) effects in MO systems are…

Optics · Physics 2025-07-04 Seth Nelson , Cong Yu , Daniel Watson , Shahrzad Ramtinfard , Miguel Levy

We demonstrate an effective and optimal strategy for generating spatially resolved longitudinal spin angular momentum (LSAM) in optical tweezers by tightly focusing first-order azimuthally radially polarized (ARP) vector beams with zero…