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We demonstrate optical control of magnons using femtosecond laser pulses by performing ab-initio real-time time-dependent density functional theory (TDDFT) simulations. We predict that the spin-wave dynamics in Fe$_{50}$Ni$_{50}$ can be…

Materials Science · Physics 2021-04-07 N. Singh , P. Elliott , J. K. Dewhurst , S. Sharma

We develop a theory of the magnetization dynamics triggered by ultrafast optical excitation of ferromagnetic semiconductors. We describe the effects of the strong carrier spin relaxation on the nonlinear optical response by using the…

Strongly Correlated Electrons · Physics 2008-08-04 J. Chovan , E. G. Kavousanaki , I. E. Perakis

The recent discovery of magnetism in two-dimensional van der Waals systems opens the door to discovering exciting physics. We investigate how a current can control the ferromagnetic properties of such materials. Using symmetry arguments, we…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 Øyvind Johansen , Vetle Risinggård , Asle Sudbø , Jacob Linder , Arne Brataas

With the goal of pushing Spintronic devices towards faster and faster timescales, we demonstrate, using ab-intio time-dependent density functional theory simulations of bulk Heusler compounds subject to ultrashort intense laser pulses, that…

Materials Science · Physics 2016-03-18 P. Elliott , T. Müller , J. K. Dewhurst , S. Sharma , E. K. U. Gross

All-optical helicity dependent switching (AO-HDS), deterministic control of magnetization by circularly polarized laser pulses, allows to efficiently manipulate spins without the need of a magnetic field. However, AO-HDS in ferromagnetic…

A central prospect of antiferromagnetic spintronics is to exploit magnetic properties that are unavailable with ferromagnets. However, this poses the challenge of accessing such properties for readout and control. To this end, light-induced…

Irradiating solids with ultrashort laser pulses is known to initiate femtosecond timescale magnetization dynamics. However, sub-femtosecond spin dynamics have not yet been observed or predicted. Here, we explore ultrafast light-driven spin…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 Ofer Neufeld , Nicolas Tancogne-Dejean , Umberto De Giovannini , Hannes Hübener , Angel Rubio

Non-thermal laser induced spin excitations, recently discovered in conventional oxide and metal ferromagnets, open unprecedented opportunities for research and applications of ultrafast optical manipulation of magnetic systems.…

Materials Science · Physics 2011-01-06 P. Nemec , E. Rozkotova , N. Tesarova , F. Trojanek , K. Olejnik , J. Zemen , V. Novak , M. Cukr , P. Maly , T. Jungwirth

Laser-induced ultrafast demagnetization is a phenomenon of utmost interest and attracts significant attention because it enables potential applications in ultrafast optoelectronics and spintronics. As a spin-orbit coupling assisted magnetic…

Laser-induced femtosecond demagnetization, femtomagnetism, offers a potential route to develop faster magnetic storage devices. It is generally believed that the traditional spin-wave theory, which is developed for thermally driven slow…

Materials Science · Physics 2019-12-05 G. P. Zhang , M. Murakami , Y. H. Bai , Thomas F. George , X. S. Wu

Optically-induced phase transitions of the manganite $\rm Pr_{1/3}Ca_{2/3}MnO_3$ have been simulated using a model Hamiltonian, that captures the dynamics of strongly correlated charge, orbital, lattice, and spin degrees of freedom. Its…

Strongly Correlated Electrons · Physics 2020-12-01 Sangeeta Rajpurohit , Liang Z. Tan , Christian Jooss , P. E. Blöchl

Multiferroic altermagnets offer new opportunities for magnetoelectric coupling and electrically tunable spintronics. However, due to intrinsic symmetry conflicts between altermagnetism and ferroelectricity, achieving their coexistence,…

Materials Science · Physics 2025-05-27 Ziye Zhu , Xunkai Duan , Jiayong Zhang , Bowen Hao , Igor Zutic , Tong Zhou

X-ray magnetic circular dichroism spectroscopy using an X-ray free electron laser is demonstrated with spectra over the Fe L$_{3,2}$-edges. This new ultrafast time-resolved capability is then applied to a fluence-dependent study of…

We unravel the dynamical stability of a fully polarized one-dimensional ultracold few-fermion spin-1/2 gas subjected to inhomogeneous driving of the itinerant spins. Despite the unstable character of the total spin-polarization the…

Quantum Gases · Physics 2019-05-09 G. M. Koutentakis , S. I. Mistakidis , P. Schmelcher

Femtosecond laser excitation of materials that exhibit magnetic spin textures promises advanced magnetic control via the generation of ultrafast and non-equilibrium spin dynamics. We explore such possibilities in ferrimagnetic [Fe(0.35…

Laser-induced terahertz spin transport (TST) and ultrafast demagnetization (UDM) are central but so far disconnected phenomena in femtomagnetism and terahertz spintronics. Here, we use broadband terahertz emission spectroscopy to reliably…

Mesoscale and Nanoscale Physics · Physics 2021-05-27 R. Rouzegar , L. Brandt , L. Nadvornik , D. A. Reiss , A. L. Chekhov , O. Gueckstock , C. In , M. Wolf , T. S. Seifert , P. W. Brouwer , G. Woltersdorf , T. Kampfrath

Understanding the coherent interplay of light with the magnetization in metals has been a long-standing problem in ultrafast magnetism. While it is known that when laser light acts on a metal it can induce magnetization via the process…

Mesoscale and Nanoscale Physics · Physics 2025-07-08 Theodoros Adamantopoulos , Dongwook Go , Peter M. Oppeneer , Yuriy Mokrousov

Using density matrix equations of motion, we predict a femtosecond collective spin tilt triggered by nonlinear, near--ultraviolet ($\sim$3eV), coherent photoexcitation of (Ga,Mn)As ferromagnetic semiconductors with linearly polarized light.…

Strongly Correlated Electrons · Physics 2009-08-06 M. D. Kapetanakis , I. E. Perakis , K. J. Wickey , C. Piermarocchi , J. Wang

In this letter we propose a method to realize a kind of spin-orbit coupling in ultracold Bose and Fermi gases whose format and strength depend on density of atoms. Our method combines two-photon Raman transition and periodical modulation of…

Quantum Gases · Physics 2021-06-23 Peng Xu , Tianshu Deng , Wei Zheng , Hui Zhai

Unveiling the key mechanisms that determine optically driven spin dynamics is essential both to probe the fundamental nature of ultrafast light-matter interactions, but also to drive future technologies of smaller, faster, and more energy…