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We discuss the construction of low-energy tight-binding Hamiltonians for condensed matter systems with a strong coupling to the quantum electromagnetic field. Such Hamiltonians can be obtained by projecting the continuum theory on a given…

Strongly Correlated Electrons · Physics 2020-05-27 Jiajun Li , Denis Golez , Giacomo Mazza , Andrew Millis , Antoine Georges , Martin Eckstein

The wave function and binding energy for shallow donors in GaAs are calculated within the tight binding (TB) approach, for supercells containing up to two million atoms. The resulting solutions, coupled with a scaling law, allow…

Materials Science · Physics 2009-11-07 A. S. Martins , J. G. Menchero , R. B. Capaz , Belita Koiller

Harrison's tight-binding theory provides an excellent qualitative description of the electronic structure of the elements across the periodic table. However, the resulting band structures are in significant disagreement with those found by…

Materials Science · Physics 2009-11-10 L. Shi , D. A. Papaconstantopoulos

The title material has a quasi-one-dimensional electronic structure and is of considerable interest because it has a metallic phase with properties different from a simple Fermi liquid, a poorly understood "insulating" phase, and a…

Strongly Correlated Electrons · Physics 2015-06-04 Jaime Merino , Ross H. McKenzie

This paper extends work done to date on quantum computation by associating potentials with different types of computation steps. Quantum Turing machine Hamiltonians, generalized to include potentials, correspond to sums over tight binding…

Quantum Physics · Physics 2009-01-23 Paul Benioff

A transferable tight-binding potential has been constructed for heteroatomic systems containing carbon and hydrogen. The electronic degree of freedom is treated explicitly in this potential using a small set of transferable parameters which…

chem-ph · Physics 2008-02-03 Yang Wang , C. H. Mak

The Empirical Tight Binding(ETB) method is widely used in atomistic device simulations. The reliability of such simulations depends very strongly on the choice of basis sets and the ETB parameters. The traditional way of obtaining the ETB…

With the help of a tight-binding (TB) electronic-structure toy model we investigate the matching of parameters across hetero-interfaces . We demonstrate that the virtual crystal approximation, commonly employed for this purpose, may not…

Mesoscale and Nanoscale Physics · Physics 2013-06-28 B. A. Stickler , W. Pötz

We present an accurate \textit{ab-initio} tight-binding hamiltonian for the transition-metal dichalcogenides, MoS$_2$, MoSe$_2$, WS$_2$, WSe$_2$, with a minimal basis (the \textit{d} orbitals for the metal atoms and \textit{p} orbitals for…

Mesoscale and Nanoscale Physics · Physics 2015-11-09 Shiang Fang , Rodrick Kuate Defo , Sharmila N. Shirodkar , Simon Lieu , Georgios A. Tritsaris , Efthimios Kaxiras

The Hubbard model, which augments independent-electron band theory with a single parameter to describe electron-electron correlations, is widely regarded to be the `standard model' of condensed matter physics. The model has been remarkably…

Strongly Correlated Electrons · Physics 2016-02-17 S. M. Griffin , P. Staar , T. C. Schulthess , M. Troyer , N. A. Spaldin

An empirical $s_cp^3_a$ tight-binding (TB) model is applied to the investigation of electronic states in semiconductor quantum dots. A basis set of three $p$-orbitals at the anions and one $s$-orbital at the cations is chosen. Matrix…

Other Condensed Matter · Physics 2009-11-11 Stefan Schulz , Gerd Czycholl

Machine-learned multi-orbital tight-binding (MMTB) Hamiltonian models have been developed to describe the electronic characteristics of intermetallic compounds $\rm Mg_2Si, Mg_2Ge, Mg_2Sn$, and $\rm Mg_2Pb$ subject to strain. The MMTB…

Materials Science · Physics 2022-07-04 Mohammad Alidoust , Erling Rothmund , Jaakko Akola

A non-perturbative relativistic tight-binding (TB) approximation method applicable to crystalline material immersed in a magnetic field was developed in 2015. To apply this method to any material in the magnetic field, the electronic…

Materials Science · Physics 2023-11-27 Rohin Sharma , Amit Shrestha , Masahiko Higuchi , Katsuhiko Higuchi , Dipendra B. Hamal

We present a scheme to controllably improve the accuracy of tight-binding Hamiltonian matrices derived by projecting the solutions of plane-wave ab initio calculations on atomic orbital basis sets. By systematically increasing the…

The need for accurate calculations on atoms and diatomic molecules is motivated by the opportunities and challenges of such studies. The most commonly-used approach for all-electron electronic structure calculations in general - the linear…

Chemical Physics · Physics 2019-08-19 Susi Lehtola

A procedure to obtain single-electron wavefunctions within the tight-binding formalism is proposed. It is based on linear combinations of Slater-type orbitals whose screening coefficients are extracted from the optical matrix elements of…

Materials Science · Physics 2016-09-16 R. Benchamekh , F. Raouafi , J. Even , F. Ben Cheikh Larbi , P. Voisin , J. -M. Jancu

For a previously published study of the titanium hcp (alpha) to omega (omega) transformation, a tight-binding model was developed for titanium that accurately reproduces the structural energies and electron eigenvalues from all-electron…

Materials Science · Physics 2008-07-24 D. R. Trinkle , M. D. Jones , R. G. Hennig , S. P. Rudin , R. C. Albers , J. W. Wilkins

Herein, we present a new method to efficiently calculate electronically excited states in large molecular assemblies, consisting of hundreds of molecules. For this purpose, we combine the long-range corrected tight-binding…

Chemical Physics · Physics 2023-02-08 Richard Einsele , Joscha Hoche , Roland Mitric

We examine the origin of the formation of narrow bands in LK-99 (Pb$_{9}$Cu(PO$_4$)$_6$O) and the parent compound without the Cu doping using density functional theory calculations and model Hamiltonian studies. Explicit analytical…

Superconductivity · Physics 2023-08-28 Mayank Gupta , S. Satpathy , B. R. K. Nanda

This article is a pedagogical introduction to density-functional tight-binding (DFTB) method. We derive it from the density-functional theory, give the details behind the tight-binding formalism, and give practical recipes for…

Materials Science · Physics 2009-11-02 Pekka Koskinen , Ville Mäkinen