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Two-dimensional (2D) vibrational spectroscopy is a powerful means of investigating the structure and dynamics of complex molecules in condensed phases. However, even in theory, analysis of 2D spectra resulting from complex inter- and…

Chemical Physics · Physics 2025-01-07 Ryotaro Hoshino , Yoshitaka Tanimura

We propose phonon spectroscopy by electric measurements of the low-temperature conductance of coupled-quantum dots, specifically employing dephasing of the quantum electronic transport by the phonons. The setup we consider consists of a…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 A. Ueda , O. Entin-Wohlman , M. Eto , A. Aharony

Uhrig's dynamical decoupling pulse sequence has emerged as one universal and highly promising approach to decoherence suppression. So far both the theoretical and experimental studies have examined single-qubit decoherence only. This work…

Quantum Physics · Physics 2015-05-14 Musawwadah Mukhtar , Thuan Beng Saw , Wee Tee Soh , Jiangbin Gong

We employ ultrafast pump-probe spectroscopy to directly monitor electron tunneling between discrete orbital states in a pair of spatially separated quantum dots. Immediately after excitation, several peaks are observed in the pump-probe…

Proposals for scalable quantum computing devices suffer not only from decoherence due to the interaction with their environment, but also from severe engineering constraints. Here we introduce a practical solution to these major concerns,…

Quantum Physics · Physics 2009-11-07 Mark S. Byrd , Daniel A. Lidar

Dual-comb interferometry harnesses the interference of two laser frequency combs to provide unprecedented capability in spectroscopy applications. In the past decade, the state-of-the-art systems have reached a point where the…

Quantum Physics · Physics 2023-09-20 Haowei Shi , Zaijun Chen , Scott E. Fraser , Mengjie Yu , Zheshen Zhang , Quntao Zhuang

When a two-dimensional electron gas is exposed to a perpendicular magnetic field and an in-plane electric field, its conductance becomes quantized in the transverse in-plane direction: this is known as the quantum Hall (QH) effect. This…

We propose two dimensional x-ray coherent correlation spectroscopy (2DXCS) for the study of interactions between core-electron and valence transitions. This technique might find experimental applications in the future when very high…

Quantum Physics · Physics 2009-11-13 Igor V. Schweigert , Shaul Mukamel

Shot noise measurements are widely used for the characterization of nonequilibrium configurations in electronic conductors. The recently introduced quantum tomography approach was implemented for the studies of electronic wavefunctions of…

Mesoscale and Nanoscale Physics · Physics 2020-08-20 E. S. Tikhonov , A. O. Denisov , S. U. Piatrusha , I. N. Khrapach , J. P. Pekola , B. Karimi , R. N. Jabdaraghi , V. S. Khrapai

We identify carrier scattering at densities below which it has previously been observed in semiconductor quantum wells. These effects are evident in the peakshapes of 2D double-quantum spectra, which change as a function of excitation…

Optics · Physics 2016-05-25 Jonathan O. Tollerud , Jeffrey A. Davis

Dual comb spectroscopy allows for high-resolution spectra to be measured over broad bandwidths, but an essential requirement for coherent integration is the availability of a phase reference. Usually, this means that the combs' phase and…

Optics · Physics 2016-06-01 David Burghoff , Yang Yang , Qing Hu

Quantum coherence is the key resource for quantum technology, with applications in quantum optics, information processing, metrology and cryptography. Yet, there is no universally efficient method for quantifying coherence either in…

Quantum Physics · Physics 2014-10-24 Davide Girolami

Background-free fluorescence detection in multidimensional electronic spectroscopy promises high sensitivity compared to conventional approaches. Here we explore the sensitivity limits of multidimensional electronic spectroscopy. We present…

Chemical Physics · Physics 2022-10-18 Amitav Sahu , Vivek N. Bhat , Sanjoy Patra , Vivek Tiwari

We theoretically investigate the implementation of the two-mode squeezing operator in circuit quantum electrodynamics. Inspired by a previous scheme for optical cavities [Phys. Rev. A $\textbf{73}$, 043803(2006)], we employ a…

Quantum Physics · Physics 2018-07-04 E. C. Diniz , D. Z. Rossatto , C. J. Villas-Boas

Non-equilibrium photon correlations of coherently excited single quantum systems can reveal their internal quantum dynamics and provide spectroscopic access. Here we propose and discuss the fundamentals of a coherent photon coincidence…

Quantum Physics · Physics 2020-11-04 Matthew Otten , Tristan Kenneweg , Matthias Hensen , Stephen K. Gray , Walter Pfeiffer

We propose an approach to measuring nonresonant coupled systems, which gives a parametrically smaller error than the conventional fast projective measurements. The approach takes into account that, due to the coupling, excitations are not…

Quantum Physics · Physics 2009-03-05 L. Fedichkin , M. Shapiro , M. I. Dykman

In quantum computation, it is of paramount importance to locate the parameter space where maximal coherence can be preserved in the qubit system. In recent years environment-induced decoherence based the quantum Brownian motion (QBM) models…

Quantum Physics · Physics 2015-06-26 B. L. Hu

We demonstrate a new technique for saturated-absorption spectroscopy using co-propagating beams that does not have the problem of crossover resonances. The pump beam is locked to a transition and its absorption signal is monitored while the…

Atomic Physics · Physics 2009-11-10 Ayan Banerjee , Vasant Natarajan

Ultrashort non-resonant electromagnetic pulses applied to effective one-electron systems may operate on the electronic state as a position or momentum translation operator. As derived here, extension to many-body correlated systems exposes…

Quantum Physics · Physics 2015-04-22 Y. Pavlyukh , J. Berakdar

In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…

Strongly Correlated Electrons · Physics 2019-05-29 Chen-Yen Lai , Jian-Xin Zhu