Related papers: Extracting double-quantum coherence in two-dimensi…
Coherent two-dimensional electronic spectroscopy probes ultrafast dynamics using femtosecond pulses. In case the timescale of the studied dynamics become comparable to the pulse duration, pulse overlap effects may compromise the…
We demonstrate an approach to two-dimensional electronic spectroscopy (2DES) that combines the benefits of shot-to-shot detection at high-repetition rates with the simplicity of a broadband white light continuum input and conventional…
Electron spin resonance (ESR) pulsed dipolar spectroscopy (PDS) is used in protein 3D structure determination. However, the accuracy of the signal analysis depends heavily on the background correction process. In this work, we derive the…
The term two-dimensional coherent spectroscopy (2DCS) usually refers to experimental setups where a coherently generated electric field in a sample is recorded over many runs as a function of two time variables: the delay $\tau$ between two…
Developing from the transient absorption (TA) spectroscopy, the two dimensional (2D) spectroscopy with pump-probe geometry has emerged as a versatile approach for alleviating the difficulty on implementing the 2D spectroscopy with other…
We present experimental coherent two-dimensional Fourier transform spectra of the exciton resonances in semiconductor quantum wells for a pulse sequence that isolates two-quantum coherences. By measuring the real part of the spectra, we can…
We discuss the potential creation and measurement of coherences in both dispersive solids and qubit-like single levels using current generation time- and angle-resolved photoemission technology. We show that in both cases, when both the…
A one-dimensional system with two $\delta$-like barriers or wells bi-chromaticaly oscillating at frequencies $\omega$ and $2\omega$ is considered. The alternating signal leads to the direct current across the structure (even in a symmetric…
Methods for reconstructing the spectral density of a vibrational environment from experimental data can yield key insights into the impact of the environment on molecular function. Although such experimental methods exist, they generally…
In this work, two experimentally feasible methods of decoherence engineering-one based on the application of stochastic classical kicks and the other based on temporally randomized pulse sequences are combined. A different coupling…
Dual comb spectroscopy (DCS) is a powerful technique for broadband spectroscopy with high precision and fast data acquisition. High-frequency resolution requires long data acquisition times, limiting the temporal resolution in time-resolved…
Superconducting quantum computing is experiencing a tremendous growth. Although major milestones have already been achieved, useful quantum-computing applications are hindered by a variety of decoherence phenomena. Decoherence due to…
We perform a beat-frequency-resolved analysis for two-dimensional electronic spectroscopy using a high-speed and stable 2D electronic spectrometer and few-cycle visible laser pulses to disentangle the vibrational coherences in an artificial…
The coupling between electronic excitations and collective bosonic modes is fundamental to the emergence of high-temperature superconductivity in cuprates. Despite extensive effort, conventional equilibrium and pump-probe optical…
A spectroscopic application of the atom laser is suggested. The spectroscopy termed 2PACC employs the coherent properties of matter-waves from a two pulse atom laser. These waves are employed to control a gas-surface chemical recombination…
Decoherence remains one of the most serious challenges to the implementation of quantum technology. It appears as a result of the transformation over time of a quantum superposition state into a classical mixture due to the quantum system…
Two-level systems (TLS) of unclear physical origin are a major contributor to decoherence in superconducting qubits. The interactions of individual TLS with a qubit can be detected via various spectroscopic methods, most of which have…
The single-particle spectral function measures the density of electronic states (DOS) in a material as a function of both momentum and energy, providing central insights into phenomena such as superconductivity and Mott insulators. While…
Multidimensional spectroscopy has a long history originating from nuclear magnetic resonance, and has now found widespread application at infrared and optical frequencies as well. However, the energy scales of traditional multidimensional…
Control over the joint spectral amplitude of a photon pair has proved highly desirable for many quantum applications, since it contains the spectral quantum correlations, and has crucial effects on the indistinguishability of photons, as…