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We report record high Si-29 spin polarization obtained using dynamic nuclear polarization in microcrystalline silicon powder. Unpaired electrons in this silicon powder are due to dangling bonds in the amorphous region of this intrinsically…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 A. E. Dementyev , D. G. Cory , C. Ramanathan

Magnetic nanomaterials are considered, formed by magnetic nanomolecules with high spins. The problem of spin reversal in these materials is analyzed, which is of interest for the possible use of such materials for quantum information…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 V. K. Henner , V. I. Yukalov , P. V. Kharebov , E. P. Yukalova

The inherent polarization gradients in tight optical tweezers can be used to couple the atomic spins to the two-body motion under the action of a microwave spin-flip transition, so that such a spin-motion coupling offers an important…

In ultrafast experiments with gas phase molecules, the alignment of the molecular axis relative to the polarization of the interacting laser pulses plays a crucial role in determining the dynamics following this light-matter interaction.…

Chemical Physics · Physics 2025-04-14 Shashank Kumar , Eric Liu , Liang Z. Tan , Varun Makhija , Niranjan Shivaram

Detecting the internal state of polar molecules is a substantial challenge when standard techniques such as resonance-enhanced multi photon ionization (REMPI) or laser-induced fluorescense (LIF) do not work. As this is the case for most…

Atomic Physics · Physics 2014-12-01 Rosa Glöckner , Alexander Prehn , Gerhard Rempe , Martin Zeppenfeld

Ultrafast characterization and control of many-body interactions and elementary excitations are critical to understanding and manipulating emergent phenomena in strongly correlated systems. In particular, spin interaction plays an important…

Strongly Correlated Electrons · Physics 2018-12-06 Yao Wang , Thomas P. Devereaux , Cheng-Chien Chen

Coherent manipulation of quantum bits (qubits) on time scales much shorter than the coherence time is a key prerequisite for quantum information processing. Electron spins in quantum dots (QDs) are particularly attractive for…

Mesoscale and Nanoscale Physics · Physics 2011-10-03 A. Greilich , Sophia E. Economou , S. Spatzek , D. R. Yakovlev , D. Reuter , A. D. Wieck , T. L. Reinecke , M. Bayer

We propose a new, more efficient, and potentially cost effective, solid-state nuclear spin hyperpolarization method combining the Cross Effect mechanism and electron spin optical hyperpolarization in rotating solids. We first demonstrate…

Quantum Physics · Physics 2022-01-25 Frederic Mentink-Vigier , Vinayak Rane , Thierry Dubroca , Krishnendu Kundu

The scattering of a flying photon by a two-level system ultrastrongly coupled to a one-dimensional photonic waveguide is studied numerically. The photonic medium is modeled as an array of coupled cavities and the whole system is analyzed…

A new type of spectroscopy for high-resolution studies of spin waves that relies on resonant scattering of hard x-rays is introduced. The energy transfer in the scattering process is encoded in the precession of the polarization vector of…

Materials Science · Physics 2019-03-25 Ralf Röhlsberger

We demonstrate time reversal of nuclear spin dynamics in highly magnetized dilute liquid 3He-4He mixtures through effective inversion of long-range dipolar interactions. These experiments, which involve using magic sandwich NMR pulse…

Other Condensed Matter · Physics 2007-10-10 Michael E. Hayden , Emmanuel Baudin , Geneviève Tastevin , Pierre-Jean Nacher

Recently developed circularly polarized X-ray light sources can probe ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism (TRCD)…

Chemical Physics · Physics 2017-02-08 Jérémy R. Rouxel , Markus Kowalewski , Shaul Mukamel

Semiconductor quantum dot molecules are considered as promising candidates for quantum technological applications due to their wide tunability of optical properties and coverage of different energy scales associated with charge and spin…

We have investigated the angle-resolved ATI spectrum of oriented molecules in the IR+XUV co-rotating circular laser fields. According to the different roles of IR and XUV laser in the ionization process, we purposefully adjust the photon…

Atomic Physics · Physics 2024-01-15 Yu-Hong Li , Facheng Jin , Yujun Yang , Fei Li , Ying-Chun Guo , Zhi-Yi Wei , Jing Chen , Xiaojun Liu , Bingbing Wang

We consider solid surface scattering of molecules that were subject to strong non-resonant ultrashort laser pulses just before hitting the surface. The pulses modify the rotational states of the molecules, causing their field free…

Chemical Physics · Physics 2015-06-12 Yuri Khodorkovsky , J. R. Manson , Ilya Sh. Averbukh

The spin dynamics in Ni is studied by an exact diagonalization method on the ultrafast time scale. It is shown that the femtosecond relaxation of the magneto-optical response results from exchange interaction and spin-orbit coupling. Each…

Materials Science · Physics 2009-10-30 W. Hubner , G. P. Zhang

Linear polarization analysis of hard x-rays is employed to probe electronic anisotropies in metal-containing complexes with very high selectivity. We use the pronounced linear dichroism of nuclear resonant x-ray scattering to determine…

Impacts of spin-polarization of an ultrarelativistic electron beam head-on colliding with a strong laser pulse on emitted photon spectra and electron dynamics have been investigated in the quantum radiation regime. We simulate photon…

Plasma Physics · Physics 2019-07-31 Yan-Fei Li , Ren-Tong Guo , Rashid Shaisultanov , Karen Z. Hatsagortsyan , Jian-Xing Li

Synchronization is ubiquitous in nature at various scales and fields. This phenomenon not only offers a window into the intrinsic harmony of complex systems, but also serves as a robust probe for many-body quantum systems. One such system…

Spin dynamics of assemblies of magnetic nanomolecules and nanoclusters can be made coherent by inserting the sample into a coil of a resonant electric circuit. Coherence is organized through the arising feedback magnetic field of the coil.…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 V. I. Yukalov , V. K. Henner , E. P. Yukalova
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