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When a laser pulse excites a ferromagnet, its spin undergoes a dramatic change. The initial demagnetization process is very fast. Experimentally, it is found that the demagnetization time is related to the spin moment in the sample. In this…

Materials Science · Physics 2016-11-11 G. P. Zhang , M. S. Si , Thomas F. George

The microscopic origin of laser-induced ultrafast demagnetization remains an open question, to which the non-thermal electronic distribution plays a vital role at the initial stage. Herein, we investigate the connection between the…

Materials Science · Physics 2025-12-25 Yu-Hui Song , Huan-Cheng Yang , Kai Liu , Zhong-Yi Lu

The ultrafast demagnetization (UFD) dynamics of itinerant ferromagnets is theoretically investigated as a function of the characteristics of the initial laser excitation. A many-body pd-band Hamiltonian is considered which takes into…

Strongly Correlated Electrons · Physics 2019-07-10 W. Töws , G. M. Pastor

Exact calculated time evolutions in the framework of a many-electron model of itinerant magnetism provide new insights into the laser-induced ultrafast demagnetization observed in ferromagnetic (FM) transition metal thin films. The…

Strongly Correlated Electrons · Physics 2015-11-25 W. Töws , G. M. Pastor

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

Laser-induced ultrafast demagnetization has puzzled researchers around the world for over two decades. Intrinsic complexity in electronic, magnetic, and phononic subsystems is difficult to understand microscopically. So far it is not…

Materials Science · Physics 2021-05-19 G. P. Zhang , Y. H. Bai , Thomas F. George

Here we carry out a first-principles time-dependent calculation to investigate how fast electrons actually move under laser excitation and how large the electron transport affects demagnetization on the shortest time scale. To take into…

Materials Science · Physics 2018-11-14 G. P. Zhang , Y. H. Bai , T. Jenkins , T. F. George

Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…

Materials Science · Physics 2010-07-06 Adrian Glaubitz

Laser-induced ultrafast demagnetization is a phenomenon of utmost interest and attracts significant attention because it enables potential applications in ultrafast optoelectronics and spintronics. As a spin-orbit coupling assisted magnetic…

Laser induced ultrafast demagnetization is the process whereby the magnetic moment of a ferromagnetic material is seen to drop significantly on a timescale of $10-100$s of femtoseconds due to the application of a strong laser pulse. If this…

Materials Science · Physics 2016-01-20 P. Elliott , K. Krieger , J. K. Dewhurst , S. Sharma , E. K. U. Gross

Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

Strongly Correlated Electrons · Physics 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

Mesoscale and Nanoscale Physics · Physics 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

This year the discovery of femtosecond demagnetization by laser pulses is 20 years old. For the first time this milestone work by Bigot and coworkers gave insight in a very direct way into the time scales of microscopic interactions that…

Mesoscale and Nanoscale Physics · Physics 2016-09-14 J. Walowski , M. Münzenberg

The magnetization of a non-magnetic semiconductor by femtosecond light pulses is crucial to achieve an all-optical control of the spin dynamics in materials and to develop faster memory devices. However, the conditions for its detection are…

Materials Science · Physics 2022-06-29 Giovanni Marini , Matteo Calandra

We demonstrate ultrafast magnetization dynamics in a 5d transition metal using circularly-polarized x-ray free electron laser in the hard x-ray region. A decay time of light-induced demagnetization of L1${}_0$-FePt was determined to be…

Optically induced demagnetization of 3d metallic ferromagnets proceeds as fast as ~100 fs and is a crucial prerequisite for spintronic applications, such as ultrafast magnetization switching and spin transport. On the 100 fs time scale, the…

We theoretically investigate the optically-induced demagnetization of ferromagnetic FePt using the time-dependent density functional theory (TDDFT). We compare the demagnetization mechanism in the perturbative and nonperturbative limits of…

Materials Science · Physics 2024-04-26 M. S. Mrudul , Peter M. Oppeneer

A decade ago Rhie \et (Phys. Rev. Lett. {\bf 90}, 247201 (2003)) reported that when ferromagnetic nickel is subject to an intense ultrashort laser pulse, its exchange splitting is reduced quickly. But to simulate such reduction remains a…

Materials Science · Physics 2016-11-15 G. P. Zhang , Y. H. Bai , Thomas F. George

The ultrafast and element-specific response of magnetic systems containing ferromagnetic 3d transition metals and 4d/5d heavy metals is of interest both from a fundamental as well as an applied research perspective. However, to date no…

Interest in femtosecond demagnetization experiments was sparked by Bigot's discovery in 1995. These experiments unveil the elementary mechanisms coupling the electrons' temperature to their spin order. Even though first quantitative models…

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