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Hydrogen and deuterium chemisorption on a single layer of graphene has been studied by path-integral molecular dynamics simulations. Finite-temperature properties of these point defects were analyzed in the range from 200 to 1500 K, by…

Materials Science · Physics 2015-05-13 Carlos P. Herrero , Rafael Ramirez

We study the behavior of hydrated graphite oxide (GO) at high temperatures using thermally accelerated molecular dynamics simulations based on ab initio density functional theory. Our results suggest that GO, a viable candidate for water…

Materials Science · Physics 2022-03-31 Andrii Kyrylchuk , Pranav Surabhi , David Tománek

A density functional theory (DFT) study of the discrete breathers (DBs) in graphane (fully hydrogenated graphene) was performed. To the best of our knowledge, this is the first demonstration of the existence of DBs in a crystalline body…

Pattern Formation and Solitons · Physics 2015-06-19 G. M. Chechin , S. V. Dmitriev , I. P. Lobzenko , D. S. Ryabov

Thermal energy storage using sensible heating of a solid storage medium is a potential low-cost technology for long-duration energy storage. To effectively get heat in and out of the solid material, channels of heat transfer fluid can be…

Applied Physics · Physics 2024-02-13 Shomik Verma , Colin Kelsall , Kyle Buznitsky , Alina LaPotin , Ashwin Sandeep , Asegun Henry

We report the results of an experimental study of thermal and magnetic properties of nanostructured ferrimagnetic iron oxide composites with graphene and graphite fillers synthesized via the current activated pressure assisted…

Materials Science · Physics 2017-10-19 S. Ramirez , K. Chan , R. Hernandez , E. Recinos , E. Hernandez , R. Salgado , A. G. Khitun , J. E. Garay , A. A. Balandin

Among its many outstanding properties, graphene supports terahertz surface plasma waves -- sub-wavelength charge density oscillations connected with electromagnetic fields that are tightly localized near the surface[1,2]. When these waves…

The structure and stability of small hydrogen clusters adsorbed on graphene is studied by means of Density Functional Theory (DFT) calculations. Clusters containing up to six H atoms are investigated systematically -- the clusters having…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Zeljko Sljivancanin , Mie Andersen , Liv Hornekaer , Bjork Hammer

Nanomaterials are anticipated to be promising storage media, owing to their high surface-to-mass ratio. The high hydrogen capacity achieved by using graphene has reinforced this opinion and motivated investigations of the possibility to use…

Materials Science · Physics 2013-11-26 Yuanyue Liu , Vasilii I. Artyukhov , Mingjie Liu , Avetik R. Harutyunyan , Boris I. Yakobson

In this work, we have studied the hydrogen adsorption-desorption properties and storage capacities of Li functionalized [2,2,2]paracyclophane (PCP222) using dispersion-corrected density functional theory and molecular dynamic simulation.…

Chemical Physics · Physics 2023-01-11 Rakesh K. Sahoo , Sridhar Sahu

Room temperature ferromagnetic materials composed only by light elements like carbon, hydrogen and/or nitrogen, so called carbon magnet, are very attractive for creating new material categories both in science and industry. Recently several…

Mesoscale and Nanoscale Physics · Physics 2011-01-24 Norio Ota , Narjes Gorjizadeh , Yoshiyuki Kawazoe

The adsorption and dissociation of isolated water molecule on Zr(0001) surface are theoretically investigated for the first time by using density-functional theory calculations. Two kinds of adsorption configurations with almost the same…

Materials Science · Physics 2015-05-27 Shuang-Xi Wang , Ping Zhang , Peng Zhang , Jian Zhao , Shu-Shen Li

Proposing new ways to organize carbon in 2D nanomaterials has been a relevant strategy in the search for systems with targeted properties for different applications. One focus is the study of fully sp$^2$ non-graphitic networks, with…

Graphene is a new material that exhibits remarkable properties from both fundamental and applied issues. This is a 2D matter system whose physical and mechanical features have been approached by using tight binding model, first principle…

Strongly Correlated Electrons · Physics 2011-08-10 Lalla Btissam Drissi , El Hassan Saidi , Mosto Bousmina

The adsorption energies and orientation of methanol on graphene are determined from first-principles density functional calculations. We employ the well-tested vdW-DF method that seamlessly includes dispersion interactions with all of the…

Materials Science · Physics 2013-03-18 Elsebeth Schroder

Two-dimensional materials composed of transition metal carbides and nitrides (MXenes) are poised to revolutionize energy conversion and storage. In this work, we used density functional theory (DFT) to investigate adsorption of Mg and Na…

Materials Science · Physics 2021-12-01 G. Chaney , D. Çakır , F. M. Peeters , C. Ataca

We have used first-principles methods to investigate how metal atoms dispersed in the interlayer space of graphitic materials affect their hydrogen-binding properties. We have considered ideal stage-one metal-intercalated graphites of…

Materials Science · Physics 2008-06-19 Manuel Cobian , Jorge Iniguez

The variation in local atomic structure and chemical bonding of ZrHx (x=0.15, 0.30, 1.16) magnetron sputtered thin films are investigated by Zr K-edge (1s) X-ray absorption near-edge structure and extended X-ray absorption fine structure…

Materials Science · Physics 2017-11-28 Martin Magnuson , Fredrik Eriksson , Lars Hultman , Hans Högberg

Constrained density functional theory (CDFT) is used to evaluate the energy level alignment of a benzene molecule as it approaches a graphene sheet. Within CDFT the problem is conveniently mapped onto evaluating total energy differences…

Mesoscale and Nanoscale Physics · Physics 2016-01-27 Subhayan Roychoudhury , Carlo Motta , Stefano Sanvito

In graphene based materials, the energy storage capacity is usually improved by rich porous structures with extremely high surface area. By utilizing surface corrugations, this work shows an alternative strategy to activate graphene…

Applied Physics · Physics 2021-10-07 Longsheng Zhong , Chang Wu , Xiaojing Zhu , Shulai Lei , Guijie Liang , Sepidar Sayyar , Biao Gao , Liangxu Lin

As a new carbon allotrope, the recently fabricated graphdiyne has attracted much attention due to its interesting two-dimensional character. Here we demonstrate by multiscale computations that, unlike graphene, graphdiyne has a natural band…

Mesoscale and Nanoscale Physics · Physics 2015-04-30 L. Sun , P. H. Jiang , H. J. Liu , D. D. Fan , J. H. Liang , J. Wei , L. Cheng , J. Zhang , J. Shi