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The formation of complexes between like-charged polyelectrolytes challenges conventional electrostatic intuition and highlights the central role of ions in mediating macromolecular organization. Here, we investigate the salt-dependent…

Soft Condensed Matter · Physics 2026-01-29 Sisem Ektirici , Vagelis Harmandaris , Christos N. Likos , Terpsichori S. Alexiou

The intricate role of shear viscosity and ion-pair relaxations on ionic conductivity mechanisms and the underlying changes induced by salt concentration ($c$) in organic liquid electrolytes remain poorly understood despite their widespread…

The self-assembling behaviour of ionic liquids in aqueous solution is important for understanding their physicochemical properties and for their industrial applications. While the influence of ionic liquids on surfactant micellization has…

Soft Condensed Matter · Physics 2026-04-01 Devansh Kaushik , Sajal K. Ghosh , Syed M. Kamil

Experiments using the Surface Force Apparatus (SFA) have found anomalously long-ranged interactions between charged surfaces in concentrated salt solutions. Ion clustering have been suggested as a possible origin of this behaviour. In this…

Soft Condensed Matter · Physics 2025-08-05 David Ribar , Clifford E. Woodward , Jan Forsman

Understanding the structure and thermodynamics of solvated ions is essential for advancing applications in electrochemistry, water treatment, and energy storage. While ab initio molecular dynamics methods are highly accurate, they are…

Chemical Physics · Physics 2025-07-15 Ademola Soyemi , Tibor Szilvasi

Clays control carbon, water and nutrient transport in the lithosphere, promote cloud formation5 and lubricate fault slip through interactions among hydrated mineral interfaces. Clay mineral properties are difficult to model because their…

We develop a simulation method which allows us to calculate the critical micelle concentrations for ionic surfactants in the presence of different salts. The results are in good agreement with the experimental data. The simulations are…

Chemical Physics · Physics 2014-04-15 Alexandre P. dos Santos , Wagner Figueiredo , Yan Levin

Many ionic surfactants, such as sodium dodecyl sulphate (SDS) crystallize out of solution if the temperature falls below the crystallization boundary. The crystallization temperature is impacted by solution properties, and can be decreased…

Porous magnetic silica beads are promising materials for biological and environmental applications due to their enhanced adsorption and ease of recovery. This work aims to develop a new, inexpensive and environmentally friendly approach…

Applied Physics · Physics 2020-05-21 David Franck Frederic Brossault , Alexander F. Routh

Ionic liquids are widely used as electrolytes in electrochemical devices. In this context, many experimental and theoretical approaches have been recently developed for characterizing their interface with electrodes. In this perspective…

Materials Science · Physics 2017-09-13 Céline Merlet , Benjamin Rotenberg , Paul Madden , Mathieu Salanne

Recent experimental results by the Surface Force Apparatus (SFA) have identified a dramatic deviation from previously established theories of simple electrolytes. This deviation, referred to as anomalous underscreening, suggests that the…

Soft Condensed Matter · Physics 2025-08-05 David Ribar , Clifford E. Woodward , Jan Forsman

Hypotheses: The aggregation number and length of spherocylindrical (rodlike, wormlike) micelles in solutions of an ionic surfactant and salt can be predicted knowing the molecular parameters and the input concentrations of the species. This…

Soft Condensed Matter · Physics 2020-10-20 K. D. Danov , P. A. Kralchevsky , R. D. Stanimirova , S. D. Stoyanov , J. L. Cook , I. P. Stott

Suspensions of calcite in water are employed in many industrial fields such as paper filling, pharmaceutics, heritage conservation or building construction, where the rheological properties of the paste need to be controlled. We measure the…

Solid-ion conductors (SICs) comprising non-ionic plastic crystals and lithium salts often require compositing with polymers to render them processable for use in solid-state lithium-metal batteries. Here, we show that polymer-doped plastic…

Computing the solubility of crystals in a solvent using atomistic simulations is notoriously challenging due to the complexities and convergence issues associated with free-energy methods, as well as the slow equilibration in…

Statistical Mechanics · Physics 2023-11-15 Aleks Reinhardt , Pin Yu Chew , Bingqing Cheng

The interaction between polyelectrolyte and ionic surfactant is of great importance in different areas of chemistry and biology. In this paper we present a theory of polyelectrolyte ionic-surfactant solutions. The new theory successfully…

Condensed Matter · Physics 2009-10-31 Paulo S. Kuhn , Yan Levin , Marcia C. Barbosa

Surface active ionic liquids (SAILs) combine useful characteristics of both ionic liquids (ILs) and surfactants, hence are promising candidates for a wide range of applications. However, the effect of SAIL ionic structures on their…

Humid hydrophobic ionic liquids, widely used as electrolytes, have narrowed electrochemical windows, because their water, absorbed on the electrode surface, gets involved in electrolysis. In this work, we performed molecular dynamics…

Applied Physics · Physics 2020-12-02 Ming Chen , Jiedu Wu , Ting Ye , Jinyu Ye , Sheng Bi , Jiawei Yan , Bingwei Mao , Guang Feng

We explore interactions between equally charged surfaces, in the presence of simple salt and either neutral or monovalently charged polyampholytes. We consider the possibility of using these charged polymers as crude models of ion clusters.…

Soft Condensed Matter · Physics 2026-03-19 David Ribar , Clifford E Woodward , Jan Forsman

Experiments using the Surface Force Apparatus (SFA) have found anomalously long ranged charge-charge underscreening in concentrated salt solutions. Meanwhile, theory and simulations have suggested ion clustering to be the possible origin of…

Soft Condensed Matter · Physics 2024-08-13 David Ribar , Clifford E. Woodward , Sture Nordholm , Jan Forsman
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