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High-throughput density functional theory (DFT) calculations allow for a systematic search for conventional superconductors. With the recent interest in two-dimensional (2D) superconductors, we used a high-throughput workflow to screen over…

Superconductivity · Physics 2023-02-13 Daniel Wines , Kamal Choudhary , Adam J. Biacchi , Kevin F. Garrity , Francesca Tavazza

Recently, ternary clathrate hydrides are promising candidates for high-temperature superconductor. However, it is a formidable challenge to effectively hunt high-temperature superconductivity among multinary hydrides due to the expensive…

Superconductivity · Physics 2024-10-29 Bowen Jiang , Xiaoshan Luo , Toshiaki Iitaka , Ying Sun , Xin Zhong , Jian Lv , Yu Xie , Yanming Ma , Hanyu Liu

The discovery of high-$T_c$ conventional superconductivity in high-pressure hydrides has helped establish computational methods as a formidable tool to guide material discoveries in a field traditionally dominated by serendipitous…

The discovery of novel high-temperature superconductor materials holds transformative potential for a wide array of technological applications. However, the combinatorially vast chemical and configurational search space poses a significant…

Superconductivity · Physics 2025-02-25 Xiaoyang Wang , Chengqian Zhang , Zhenyu Wang , Hanyu Liu , Jian Lv , Han Wang , Weinan E , Yanming Ma

The measurement of superconductivity at above 200K in compressed samples of hydrogen sulfide and lanthanum hydride at 250K is reinvigorating the search for conventional high temperature superconductors. At the same time it exposes a…

Superconductivity · Physics 2019-10-02 Chris J. Pickard , Ion Errea , Mikhail I. Eremets

Searching for superconducting hydrides has so far largely focused on finding materials exhibiting the highest possible critical temperatures ($T_c$). This has led to a bias towards materials stabilised at very high pressures, which…

Superconductivity · Physics 2020-04-29 Michael J. Hutcheon , Alice M. Shipley , Richard J. Needs

The high critical superconducting temperatures ($T_c$s) of metal hydride phases with clathrate-like hydrogen networks have generated great interest. Herein, we employ the Density Functional Theory-Chemical Pressure (DFT-CP) method to…

Superconductivity · Physics 2022-05-25 Katerina P. Hilleke , Eva Zurek

Hydrides are considered to be one of the most promising families of compounds for achieving high temperature superconductivity. However, there are very few experimental reports of ambient-pressure hydride superconductivity, and the…

Superconductivity · Physics 2026-03-18 Antonio Sanna , Tiago F. T. Cerqueira , Ekin Dogus Cubuk , Ion Errea , Yue-Wen Fang

Hydrogen-rich superhydrides are believed to be very promising high-T$_c$ superconductors, with experimentally observed critical temperatures near room temperature, as shown in recently discovered lanthanide superhydrides at very high…

Superconductivity · Physics 2021-09-09 Evgeny Plekhanov , Zelong Zhao , Francesco Macheda , Yao Wei , Nicola Bonini , Cedric Weber

The theoretical exploration of the phase diagrams of binary hydrides under pressure using \emph{ab initio} crystal structure prediction techniques coupled with first-principles calculations has led to the \emph{in silico} discovery of…

Superconductivity · Physics 2019-02-25 Eva Zurek , Tiange Bi

We survey the landscape of binary hydrides across the entire periodic table from 10 to 500 GPa using a crystal structure prediction method. Building a critical temperature ($T_c$) model, with inputs arising from density of states…

Superconductivity · Physics 2021-08-11 Alice M. Shipley , Michael J. Hutcheon , Richard J. Needs , Chris J. Pickard

We employed a machine-learning assisted approach to search for superconducting hydrides under ambient pressure within an extensive dataset comprising over 150 000 compounds. Our investigation yielded around 50 systems with transition…

Superconductivity · Physics 2024-03-21 Tiago F. T. Cerqueira , Yue-Wen Fang , Ion Errea , Antonio Sanna , Miguel A. L. Marques

The primary challenge in the field of high-temperature superconductivity in hydrides is to achieve a superconducting state at ambient pressure rather than the extreme pressures that have been required in experiments so far. Here, we propose…

The 2014-2015 prediction, discovery, and confirmation of record high temperature superconductivity above 200K in H$_3$S, followed by the 2018 extension to superconductivity in the 250-280K range in lanthanum hydride, marks a new era in the…

Superconductivity · Physics 2019-11-13 Yundi Quan , Soham S. Ghosh , Warren E. Pickett

A key challenge in materials discovery is to find high-temperature superconductors. Hydrogen and hydride materials have long been considered promising materials displaying conventional phonon-mediated superconductivity. However, the high…

For half a century after the discovery of superconductivity, materials exploration for better superconductors proceeded without knowledge of the underlying mechanism. The 1957 BCS theory cleared that up: the superconducting state occurs due…

Superconductivity · Physics 2023-04-19 Warren E. Pickett

It has been a hot issue to search for hydrides at high pressure with high superconducting transition temperature (Tc). In this work, ternary hydrogen-rich compounds KYHn (n = 1-16) were studied and calculated using the density function…

Superconductivity · Physics 2021-10-27 LingYan Chen

Over the past decade, a combination of crystal structure prediction techniques and experimental synthetic work has thoroughly explored the phase diagrams of binary hydrides under pressure. The fruitfulness of this dual approach is…

Superconductivity · Physics 2022-02-21 Katerina P. Hilleke , Eva Zurek

Metallic hydrogen, existing in remarkably extreme environments, was predicted to exhibit long-sought room-temperature superconductivity. Although the superconductivity of metallic hydrogen has not been confirmed experimentally,…

Superconductivity · Physics 2024-06-12 Zihan Zhang , Wendi Zhao , Defang Duan , Tian Cui

The use of high pressure to realize superconductivity in the vicinity of room temperature has a long history, much of it focused on achieving this in hydrogen rich materials. This paper provides a brief overview of the work presented at…

Superconductivity · Physics 2019-06-11 Russell J. Hemley , Muhtar Ahart , Hanyu Liu , Maddury Somayazulu
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