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Related papers: Calculation of electron-impact and photo-ionizatio…

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We develop and implement a Gaussian approach to calculate partial cross-sections and asymmetry parameters for molecular photoionization. Optimal sets of complex Gaussian-type orbitals (cGTOs) are first obtained by non-linear optimization,…

Chemical Physics · Physics 2021-11-17 Abdallah Ammar , Lorenzo Ugo Ancarani , Arnaud Leclerc

Multicentric integrals that involve a continuum state cannot be evaluated with the usual quantum chemistry tools and require a special treatment. We consider an initial molecular bound state described by multicenter spherical or cartesian…

Quantum Physics · Physics 2021-11-17 Abdallah Ammar , Arnaud Leclerc , Lorenzo Ugo Ancarani

Calculations are performed for electron collision with the methylene molecular ion CH$_2^+$ in its bent equilibrium geometry, with the goal to obtain cross sections for electron impact excitation and dissociation. The polyatomic version of…

Plasma Physics · Physics 2024-05-22 K. Chakrabarti , J. Zs Mezei , I. F. Schneider , J. Tennyson

We implement a full nonlinear optimization method to fit continuum states with complex Gaussians. The application to a set of regular scattering Coulomb functions allows us to validate the numerical feasibility, to explore the range of…

Computational Physics · Physics 2020-08-28 Abdallah Ammar , Arnaud Leclerc , Lorenzo Ugo Ancarani

A classical description of electron emission differential ionization cross sections for highly-charged high-velocity ions ($\sim$ 10 a.u.) impinging on water molecules is presented. We investigate the validity of the classical statistical…

Atomic Physics · Physics 2020-01-22 Alba Jorge , Marko Horbatsch , Clara Illescas , Tom Kirchner

Two models for the calculation of ionization cross sections by electron impact on atoms, the Binary-Encouter-Bethe and the Deutsch-Maerk models, have been implemented; they are intended to extend and improve Geant4 simulation capabilities…

Computational Physics · Physics 2015-05-30 Hee Seo , Maria Grazia Pia , Paolo Saracco , Chan Hyeong Kim

A review of some recently developed methods of calculating multiple differential cross-sections of photoionization and electron impactionization of atoms and molecules having two active electrons is presented. The methods imply original…

We present a theoretical method for calculating multiphoton ionization amplitudes and cross sections of few-electron atoms. The present approach is based on an extraction of partial wave amplitudes from a scattering wave function, which is…

Atomic Physics · Physics 2021-04-21 Andrej Mihelic , Martin Horvat

An apparatus for production of various atomic and molecular ions inside a linear Paul trap has been set up. The system applies a custom-made, low energy, pulsed electron gun to produce ions in electron impact process. Such ionization method…

Instrumentation and Detectors · Physics 2018-05-07 Łukasz Kłosowski , Mariusz Piwiński , Szymon Wójtewicz , Daniel Lisak

We present a method to compute the photoionization spectra of atoms and molecules in linear response time-dependent density functional theory. The electronic orbital variations corresponding to ionized electrons are expanded on a basis set…

Computational Physics · Physics 2023-05-24 Ivan Duchemin , Antoine Levitt

Electronic excitations and ionisations produced by electron impact are key processes in the radiation-induced damage mechanisms in materials of biological relevance, underlying important medical and technological applications, including…

Chemical Physics · Physics 2021-08-04 Pablo de Vera , Isabel Abril , Rafael Garcia-Molina

The total cross section for double ionization of lithiumlike ions by a high-energy photon is calculated in leading order of the nonrelativistic perturbation theory. The partial contributions due to simultaneous and sequential emissions of…

Atomic Physics · Physics 2009-11-11 A. I. Mikhailov , I. A. Mikhailov , A. V. Nefiodov , G. Plunien

We propose a semi-empirical formula for the cross section of ionization by electron impact. The formula involves adjustable parameters which are determined by comparison with measured or numerically calculated cross sections. In the latter…

Atomic Physics · Physics 2024-04-09 Djamel Benredjem , Jean-Christophe Pain

The calculation of partial two-photon ionization cross sections in the above-threshold energy region is discussed in the framework of exterior complex scaling. It is shown that with a minor modification of the usual procedure, which is…

Atomic Physics · Physics 2018-08-17 Andrej Mihelič

A quasi classical approximation to quantum mechanical scattering in the Moeller formalism is developed. While keeping the numerical advantage of a standard Classical--Trajectory--Monte--Carlo calculation, our approach is no longer…

Atomic Physics · Physics 2009-11-07 Tihamer Geyer , Jan M. Rost

We use the recently introduced independent-atom-model pixel counting method to calculate proton-impact net ionization cross sections for a large class of biologically relevant systems including pyrimidines, purines, amino acids, and…

Atomic and Molecular Clusters · Physics 2019-10-02 Hans Jürgen Lüdde , Marko Horbatsch , Tom Kirchner

With a recently proposed quasiclassical ansatz [Geyer and Rost, J. Phys. B 35 (2002) 1479] it is possible to perform classical trajectory ionization calculations on many electron targets. The autoionization of the target is prevented by a…

Atomic Physics · Physics 2009-11-10 Tihamer Geyer

We study the electron-impact induced ionization of O$_{2}$ from threshold to 120 eV using the electron spectroscopy method. Our approach is simple in concept and embodies the ion source with a collision chamber and a mass spectrometer with…

Atomic Physics · Physics 2021-04-23 R. A. Lomsadze , M. R. Gochitashvili , R. Ya. Kezerashvili , M. Schulz

Electron-impact cross sections for the dissociation process of vibrationally excited He2+ molecular ion, as a function of the incident electron energy are calculated for the dissociative transition X2\Sigma+u \to A2\Sigma+g by using the…

Plasma Physics · Physics 2015-06-29 R. Celiberto , K. L. Baluja , R. K. Janev , V. Laporta

This paper presents a theoretical investigation of the cross sections for dissociative electron attachment and dissociative excitation processes in vibrationally excited CH radicals induced by electron impact. Resonant electron-CH…

Atomic Physics · Physics 2026-02-12 O. Abidi , I. Jendoubi , M. Telmini , R. Ghosh , K. Chakrabarti , V. Laporta
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