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Layered 2D organic-inorganic perovskite semiconductors support strongly confined excitons that offer significant potential for ultrathin polaritonic devices due to their tunability and huge oscillator strength. The application of a magnetic…

Mesoscale and Nanoscale Physics · Physics 2025-02-26 Jonas K. König , Jamie M. Fitzgerald , Ermin Malic

We demonstrate dynamic pressure tuning (0-6.6 GPa) of layer-hybridized excitons in AB-stacked trilayer WSe$_2$ via diamond-anvil-cell-integrated reflectance spectroscopy. Pressure-controlled interlayer coupling manifests in enhanced…

Materials Science · Physics 2025-03-04 Xuan Zhao , Jing Song , Wenqi Xiong , Qianying Hu , Yuxuan Song , Xin He , Tianzhong Yang , Song Liu , Shengjun Yuan , Hongyi Yu , Yang Xu

Semiconductors in all dimensionalities ranging from 0D quantum dots and molecules to 3D bulk crystals support bound electron-hole pair quasiparticles termed as excitons. Over the past two decades, the emergence of a variety of…

Materials Science · Physics 2021-08-03 Surendra B. Anantharaman , Kiyoung Jo , Deep Jariwala

Two-dimensional (2D) transition-metal dichalcogenides (TMDC) are considered highly promising platforms for next-generation optoelectronic devices. Owing to its atomically thin structure, device performance is strongly impacted by a minute…

Mesoscale and Nanoscale Physics · Physics 2024-04-16 Sergey Trishin , Christian Lotze , Nils Krane , Katharina J. Franke

We present a novel experimental protocol using Cathodoluminescence measurements as a function of the electron incident energy to study both exciton diffusion in a directional way and surface exciton recombination. Our approach overcomes the…

The limited quantum yield of strained monolayer transition metal dichalcogenides grown by vapor-phase methods and during transfer-based stacking poses a fundamental challenge for their optoelectronic applications. Here, we introduce the…

Tuning magnetic anisotropy through chemical doping is a powerful strategy for designing functional materials with enhanced magnetic properties. Here, we report an enhanced Er^3+ magnetic moment resulting from nonmagnetic Lu^3+ substitution…

In this work, we have systematically studied the role of point defects in the recombination time of monolayer MoS$_2$ using time-dependent ab initio non-adiabatic molecular dynamics simulations. Various types of point defects, such as S…

Materials Science · Physics 2021-07-07 Raquel Esteban-Puyuelo , Biplab Sanyal

Defect-assisted recombination is an important limitation on efficiency of optoelectronic devices. However, since nonradiative capture rates decrease exponentially with energy of the transition, the mechanisms by which such recombination can…

Materials Science · Physics 2016-06-08 Audrius Alkauskas , Cyrus E. Dreyer , John L. Lyons , Chris G. Van de Walle

The ultra-strong light-matter coupling regime has been demonstrated in a novel three-dimensional inductor-capacitor (LC) circuit resonator, embedding a semiconductor two-dimensional electron gas in the capacitive part. The fundamental…

Bright excitons in ferromagnetic monolayers CrI$_3$ efficiently interact with lattice magnetization, which makes possible all-optical resonant magnetization control in this material. Using the combination of ab-initio simulations within…

Mesoscale and Nanoscale Physics · Physics 2023-05-23 A. Kudlis , M. Kazemi , Y. Zhumagulov , H. Schrautzer , P. F. Bessarab , I. V. Iorsh , I. A. Shelykh

Semiconductor heterostructures are backbones for solid state based optoelectronic devices. Recent advances in assembly techniques for van der Waals heterostructures has enabled the band engineering of semiconductor heterojunctions for…

Two-dimensional (2D) monolayer phosphorene, a 2D system with quasi-one-dimensional (quasi-1D) excitons, provides a unique 2D platform for investigating the dynamics of excitons in reduced dimensions and fundamental many-body interactions.…

Materials Science · Physics 2016-02-03 Renjing Xu , Jiong Yang , Ye Win Myint , Jiajie Pei , Han Yan , Fan Wang , Yuerui Lu

We investigate exciton emission of quantum well embedded in a semiconductor microcavity. The analytical expressions of the light intensity for the cases of excitonic number state and coherent state are presented by using secular…

Quantum Physics · Physics 2009-11-10 Guang-Ri Jin , Wu-Ming Liu

The recent experimental discovery of intrinsic ferromagnetism in single-layer CrI3 opens a new avenue to low-dimensional spintronics. However, the low Curie temperature Tc=45 K is still a large obstacle to its realistic device application.…

Materials Science · Physics 2019-06-26 Hongxing Li , Yuan-Kai Xu , Kang Lai , Wei-Bing Zhang

Even the best quality 2D materials have non-negligible concentrations of vacancies and impurities. It is critical to understand and quantify how defects change intrinsic properties, and use this knowledge to generate functionality. This…

Other Condensed Matter · Physics 2020-10-22 Pedro Miguel M. C. de Melo , Zeila Zanolli , Matthieu Jean Verstraete

Auger-ionized carriers in a one-dimensional semiconductor are predicted to result in a strong band-gap renormalization. Isolated single-walled carbon nanotubes (SWCNT) under high-intensity laser irradiation exhibit strong nonlinear…

Mesoscale and Nanoscale Physics · Physics 2016-02-26 Mitchell D. Anderson , Meghan N. Beattie , Jack A. Alexander-Webber , Robin J. Nicholas , James M. Fraser

Materials with large second-order nonlinearities are crucial for next-generation integrated photonics. Spontaneously oriented organic thin films prepared by physical vapor deposition offer a promising poling-free and scalable approach. This…

Semiconducting single-wall carbon nanotubes (SWCNTs) are a promising material platform for near-infrared in-vivo imaging, optical sensing, and single-photon emission at telecommunication wavelengths. The functionalization of SWCNTs with…

Materials Science · Physics 2024-11-20 Finn L. Sebastian , Simon Settele , Han Li , Benjamin S. Flavel , Jana Zaumseil

Explaining the mechanism of superconductivity in the high-$T_c$ cuprates requires an understanding of what causes electrons to form Cooper pairs. Pairing can be mediated by phonons, the screened Coulomb force, spin or charge fluctuations,…

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