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Magnetic molecules, modelled as finite-size spin systems, are test-beds for quantum phenomena and could constitute key elements in future spintronics devices, long-lasting nanoscale memories or noise-resilient quantum computing platforms.…

Quantum Physics · Physics 2021-03-16 A. Chiesa , F. Tacchino , M. Grossi , P. Santini , I. Tavernelli , D. Gerace , S. Carretta

Linear-scaling electronic structure methods based on the calculation of moments of the underlying electronic Hamiltonian offer a computationally efficient and numerically robust scheme to drive large-scale atomistic simulations, in which…

Materials Science · Physics 2017-01-09 Eunan J. McEniry , Ralf Drautz

The kernel polynomial method allows to sample overall spectral properties of a quantum system, while sparse diagonalization provides accurate information about a few important states. We present a method combining these two approaches…

Efficient and stable algorithms for the calculation of spectral quantities and correlation functions are some of the key tools in computational condensed matter physics. In this article we review basic properties and recent developments of…

Other Condensed Matter · Physics 2007-05-23 Alexander Weisse , Gerhard Wellein , Andreas Alvermann , Holger Fehske

We employ so-called quantum kernel estimation to exploit complex quantum dynamics of solid-state nuclear magnetic resonance for machine learning. We propose to map an input to a feature space by input-dependent Hamiltonian evolution, and…

Quantum Physics · Physics 2022-03-14 Takeru Kusumoto , Kosuke Mitarai , Keisuke Fujii , Masahiro Kitagawa , Makoto Negoro

We demonstrate that a numerical linked cluster expansion method is a powerful tool to calculate quantum dynamics. We calculate the dynamics of the magnetization and spin correlations in the two-dimensional transverse field Ising and XXZ…

Quantum Physics · Physics 2021-06-03 Ian G. White , Bhuvanesh Sundar , Kaden R. A. Hazzard

The determination of the energy spectra of small spin systems as for instance given by magnetic molecules is a demanding numerical problem. In this work we review numerical approaches to diagonalize the Heisenberg Hamiltonian that employ…

Strongly Correlated Electrons · Physics 2010-08-30 R. Schnalle , J. Schnack

This work describes a new version of the Fast Multipole Method for summing pairwise particle interactions that arise from discretizing integral transforms and convolutions on the sphere. The kernel approximations use barycentric Lagrange…

Numerical Analysis · Mathematics 2026-04-01 Anthony Chen , Robert Krasny

Targeting simulations on parallel hardware architectures, this paper presents computational kernels for efficient computations in mortar finite element methods. Mortar methods enable a variationally consistent imposition of coupling…

Numerical Analysis · Mathematics 2023-08-25 Matthias Mayr , Alexander Popp

Efficient numerical methods are required for the design of optimised devices. In magnonics, the primary computational tool is micromagnetic simulations, which solve the Landau-Lifshitz equation discretised in time and space. However, their…

Mesoscale and Nanoscale Physics · Physics 2023-07-26 Wojciech Śmigaj , Krzysztof Sobucki , Paweł Gruszecki , Maciej Krawczyk

Molecular Nanomagnets have attracted the attention of the scientific community since the rich physics behind their magnetic behaviour make them ideal test-beds for fundamental concepts in quantum mechanics. Sophisticated experiments and…

Mesoscale and Nanoscale Physics · Physics 2021-01-19 Elena Garlatti , Alessandro Chiesa , Tatiana Guidi , Giuseppe Amoretti , Paolo Santini , Stefano Carretta

In this work, we describe essential tools of linear algebra necessary for calculating the effect of chemical exchange on spin dynamics and polarization transfer in various nuclear magnetic resonance (NMR) experiments. We show how to…

Chemical Physics · Physics 2023-08-01 Jingyan Xu , Danila A. Barskiy

The procedure for simulating the nuclear magnetic resonance spectrum linked to the spin system of a molecule for a certain nucleus entails diagonalizing the associated Hamiltonian matrix. As the dimensions of said matrix grow exponentially…

Quantum Physics · Physics 2024-10-29 Joaquín Ossorio-Castillo , Alexandre Rodríguez-Coello

We propose a non-collinear spin-constrained method that generates training data for deep-learning-based magnetic model, which provides a powerful tool for studying complex magnetic phenomena that requires large-scale simulations at the…

Atomistic spin dynamics simulations provide valuable information about the energy spectrum of magnetic materials in different phases, allowing one to identify instabilities and the nature of their excitations. However, the time cost of…

Computational Physics · Physics 2023-08-09 Hongwei Chen , Yujia Zhai , Joshua J. Turner , Adrian Feiguin

We describe a simple quantum mechanical method that can be used to obtain accurate numerical results over long time scales for the spin correlation tensor of an electron spin that is hyperfine coupled to a large number of nuclear spins.…

Quantum Physics · Physics 2018-08-13 Lachlan P. Lindoy , David E. Manolopoulos

Coulomb interactions that occur in electronic structure calculations are correlated by allowing basis function components of the interacting densities to polarize, thereby reducing the magnitude of the interaction. Exchange integrals of…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

We present a new particle-based (discrete element) numerical method for the simulation of granular dynamics, with application to motions of particles on small solar system body and planetary surfaces. The method employs the parallel N-body…

Earth and Planetary Astrophysics · Physics 2013-06-12 Derek C. Richardson , Kevin J. Walsh , Naomi Murdoch , Patrick Michel

These proceedings sketch how combining recent theoretical advances with data from the new generation of high-precision Compton scattering experiments on both the proton and few-nucleon systems offers fresh, detailed insight into the Physics…

Nuclear Theory · Physics 2009-11-10 Harald W. Griesshammer

Vibronic coupling has a dramatic influence over a large number of molecular processes, ranging from photo-chemistry, to spin relaxation and electronic transport. The simulation of vibronic coupling with multi-reference wavefunction methods…

Chemical Physics · Physics 2023-10-17 Lorenzo A. Mariano , Sourav Mondal , Alessandro Lunghi
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