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Related papers: Bulk Photovoltaic Effects in Helimagnets

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Broadband, efficient and fast conversion of light to electricity is crucial for sensing and clean energy. Here we reveal the largest observed bulk photo-voltaic effect (BPVE), an intrinsic mechanism predicted to be ultrafast and exceed the…

The bulk photovoltaic effect (BPVE) refers to current generation due to illumination by light in a homogeneous bulk material lacking inversion symmetry. In addition to the intensively studied shift current, the ballistic current, which…

Materials Science · Physics 2021-05-05 Zhenbang Dai , Aaron M. Schankler , Lingyuan Gao , Liang Z. Tan , Andrew M. Rappe

The bulk photovoltaic effect exhibited by the non-centrosymmetric system gains research interest due to the observed large open-circuit voltage. The ferroelectric systems exhibiting anomalous photovoltaic effect are mostly crystallized with…

Materials Science · Physics 2021-04-08 Subhajit Pal , S. Muthukrishnan , Banasree Sadhukhan , Sarath N. , D. Murali , Pattukkannu Murugavel

Photogalvanic effect (PGE) occurs in materials with non-centrosymmetric structures when irradiated by linearly or circularly polarized light. Here, using non-equilibrium Green's function combined with density functional theory (NEGF-DFT),…

Materials Science · Physics 2023-05-26 Li-Wen Zhang , Ya-Qing Yang , Jun Chen , Lei Zhang

The bulk photovoltaic effect (BPVE), a manifestation of broken centrosymmetry, has attracted interest as a probe of the symmetry and quantum geometry of materials, and for use in novel optoelectronic devices. Despite its bulk nature, the…

A bulk material without inversion symmetry can generate a direct current under illumination. This interface-free current generation mechanism, referred to as the bulk photovoltaic effect (BPVE), does not rely on $p$-$n$ junctions. Here, we…

Materials Science · Physics 2023-05-01 Zhuang Qian , Jian Zhou , Hua Wang , Shi Liu

Spontaneous polarization and bulk photovoltaic effect (BPVE) are two concomitant physical properties in ferroelectric materials. The flipping of ferroelectric order usually accompanies with the switching of BPVE as both of them are reversed…

Materials Science · Physics 2022-07-04 Rui-Chun Xiao , Yang Gao , Hua Jiang , Wei Gan , Changjin Zhang , Hui Li

Realization of giant and continuously tunable second-order photocurrent is desired for many nonlinear optical (NLO) and optoelectronic applications, which remains to be a great challenge. Here, based on a simple two-band model, we propose a…

Materials Science · Physics 2023-07-05 Xiao Jiang , Lei Kang , Jianfeng Wang , Bing Huang

Magnetic fields break time-reversal symmetry (TRS) and reshape a material's spatial symmetry. Because the bulk photovoltaic effect (BPVE) is exquisitely sensitive to symmetry, it offers a natural arena for magnetic-field control. Here, we…

Mesoscale and Nanoscale Physics · Physics 2025-12-01 Yuncheng Mao , Claudio Attaccalite

Bulk photovoltaic (BPVE) effect in crystals lacking inversion symmetry offers great potential for optoelectronic applications due to its unique properties such as above bandgap photovoltage and switchable photocurrent. Because of their…

Materials Science · Physics 2021-10-27 Amr Abdelsamie , Lu You , Le Wang , Shuzhou Li , Mingqiang Gu , Junling Wang

The bulk photovoltaic effect provides a fundamental pathway for direct light-to-current conversion in quantum materials. However, these nonlinear currents are often strictly constrained or forbidden by crystal symmetries, hindering their…

Mesoscale and Nanoscale Physics · Physics 2026-05-25 Zhuocheng Lu , Zhuang Qian , Zhichao Guo , Likun Shi , Shi Liu , Hua Wang , Kai Chang

Nonlinear optical (NLO) effects have attracted great interest recently. However, by far the computational studies on NLO use the independent particle approximation and ignore many-body effects. Here we develop a generic Green's function…

Materials Science · Physics 2022-07-05 Haowei Xu , Hua Wang , Ju Li

Bulk photovoltaic effect is a non-linear response in noncentrosymmetric materials that converts light into DC current. In this work, we investigate the optical linear and non-linear responses in a chalcopyrite semiconductor ZnGeP$_2$. We…

Materials Science · Physics 2024-10-15 Banasree Sadhukhan

Converting light into steady currents and spin-currents in two-dimensional (2D) platform is essential for future energy harvesting and spintronics. We show that the giant and modulable bulk photovoltaic effects (BPVEs) can be achieved in…

Materials Science · Physics 2023-01-10 Liang Liu , Weikang Liu , Bin Cheng , Bin Cui , Jifan Hu

The bulk photovoltaic effect (BPVE) has attracted an increasing interest due to its potential to overcome the efficiency limit of traditional photovoltaics, and much effort has been devoted to understanding its underlying physics. However,…

Materials Science · Physics 2022-01-05 Zhenbang Dai , Andrew M. Rappe

We theoretically predict a generation of a current in Weyl semimetals by applying circularly polarized light. The electric field of the light can drive an effective magnetic field of order of ten Tesla. For lower frequency light, a…

Mesoscale and Nanoscale Physics · Physics 2016-05-18 Katsuhisa Taguchi , Tatsushi Imaeda , Masatoshi Sato , Yukio Tanaka

We elucidate light-induced orbital and spin current through nonlinear response theory, which generalizes the well-known bulk photovoltaic effect in centrosymmetric broken materials from charge to the spin and orbital degrees of freedom. We…

Materials Science · Physics 2021-08-30 Xingchi Mu , Jian Zhou

The nonlinear shift current, also known as the bulk photovoltaic current generated by linearly polarized light, has long been known to be absent in crystals with inversion symmetry. Here we argue that a non-zero shift current in…

Mesoscale and Nanoscale Physics · Physics 2021-05-19 Li-kun Shi , Dong Zhang , Kai Chang , Justin C. W. Song

We calculate the bulk photovoltaic response of the ferroelectrics BaTiO$_3$ and PbTiO$_3$ from first principles by applying "shift current" theory to the electronic structure from density functional theory. The first principles results for…

Materials Science · Physics 2015-06-04 Steve M. Young , Andrew M. Rappe

Bulk photovoltaic effect, which arises from crystal symmetry-driven charge carrier separation, is an intriguing physical phenomenon that has attracted extensive interest in photovoltaic application due to its junction-free photovoltaic and…

Materials Science · Physics 2023-08-22 Xiaojuan Chen , Kang Xu , Tingxiao Qin , Yubin Wang , Yuzhong Chen , Haiyun Liu , Qihua Xiong