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This study explores the pressure evolution of the double perovskite Ba$_2$NiTeO$_6$ by employing experimental and computational techniques. For the study of structural and vibrational properties, synchrotron X-ray diffraction (XRD) and…

We report the decomposition of La2-xSrxCuO4 into La2O3 and Cu nanoparticles in ultra-high vacuum, observed by in-situ heating experiments in a transmission electron microscope (TEM). The analysis of electron diffraction data reveals that…

In this work we have investigated the orthorhombic to tetragonal phase transition in the Ba2Cu3O4Cl2 compound. This transition was observed by X-ray powder diffractometry carried out in samples heat treated between 700 and 750OC and also in…

Materials Science · Physics 2007-05-23 M. S. da Luz , C. A. M. dos Santos , B. Ferreira , A. J. S. Machado

First principles linear response calculations are used to investigate the lattice dynamics of what is thought to be the third most abundant phase in the lower mantle, CaSiO_3 perovskite. The commonly assumed cubic structure (Pm3m) is found…

Geophysics · Physics 2016-09-08 Lars Stixrude , Ronald E. Cohen , Rici Yu , Henry Krakauer

We report the time and temperature dependent response of thermopower in the non-magnetic perovskite oxide NdNiO$_3$. We find that on cooling below the metal-insulator transition temperature the system evolves into a phase separated state…

Other Condensed Matter · Physics 2011-04-26 Devendra Kumar , K. P. Rajeev , J. A. Alonso , M. J. Martinez Lope

Shape memory alloys (SMAs) exhibit hysteresis behaviors upon stress and temperature induced loadings. In this contribution, we focus on numerical simulations of microstructure evolution of cubic-to-tetragonal martensitic phase…

Materials Science · Physics 2014-03-25 R. Dhote , H. Gomez , R. Melnik , J. Zu

We report on a systematic study of a number of structurally identical but chemically distinct transition metal oxides in order to determine how the material-specific properties such as the composition and the strain affect the properties at…

The crystallographic and magnetic properties of the cleavable 4d3 transition metal compound a-MoCl3 are reported, with a focus on the behavior above room temperature. Crystals were grown by chemical vapor transport and characterized using…

We present a coordinated study of the paramagnetic-to-antiferromagnetic, rhombohedral-to-monoclinic, and metal-to-insulator transitions in thin-film specimens of the classic Mott insulator V$_2$O$_3$ using low-energy muon spin relaxation,…

Magnetic phase transitions have been explored in a superlattice formed by stacking monolayers of $\rm LaTiO_{3}$ and $\rm LaVO_{3}$ alternately, using ab-initio density functional theory (DFT) and Monte-Carlo (MC) simulations. DFT derived…

Computational Physics · Physics 2022-05-10 Mukesh Sharma , Tulika Maitra

On the basis of the first-principles evolutionary crystal structure prediction of stable compounds in the Cu-F system, we predict two experimentally unknown stable phases -- Cu2F5 and CuF3. Cu2F5 comprises two interacting magnetic…

The junction magnetoresistivity and domain phase transition were studied between ZnO and La0.4Gd0.1Sr0.5CoO3 thin films grown on LaAlO3 (100) substrates epitaxially by pulse laser deposit. The ferromagnetic transformation into…

Materials Science · Physics 2013-11-08 Ren R , Weiren Wang , Xuan Li , Zhongxia Zhao

Semi-local DFT methods exhibit significant errors for the phase diagrams of transition-metal oxides that are caused by an incorrect description of molecular oxygen and the large self-interaction error in materials with strongly localized…

Materials Science · Physics 2022-03-29 Nongnuch Artrith , José Antonio Garrido Torres , Alexander Urban , Mark S. Hybertsen

Neutron diffraction studies have been carried out on a single crystal of oxygen-deficient perovskite TbBaCo2O5.5 in the temperature range of 7-370 K. There have been observed several magnetic or structural transitions. Among these, the…

Strongly Correlated Electrons · Physics 2009-11-10 Minoru Soda , Yukio Yasui , Toshiaki Fujita , Takeshi Miyashita , Masatoshi Sato , Kazuhisa Kakurai

Synchrotron X-ray diffraction patterns were measured and analyzed for a polycrystalline sample of the room-temperature ferromagnet Sr3.12Er0.88Co4O10.5 from 300 to 650 K, from which two structural phase transitions were found to occur…

Strongly Correlated Electrons · Physics 2009-11-13 Shintaro Ishiwata , Wataru Kobayashi , Ichiro Terasaki , Kenichi Kato , Masaki Takata

The defect chemistry of perovskite compounds is directly related to the stoichiometry and to the valence states of the transition-metal ions. Defect engineering has become increasingly popular as it offers the possibility to influence the…

${\lambda}$-RhO$_2$, a prototype 4d transition metal oxide, has been prepared by oxidative delithiation of spinel LiRh$_2$O$_4$ using ceric ammonium nitrate. Average-structure studies of this RhO$_2$ polytype, including synchrotron powder…

Uranium dioxide (UO$_2$) remains a formidable challenge for first-principles approaches, due to the complex interplay among spin-orbit coupling, Mott physics, magnetic ordering, and crystal distortions. Here we use DFT+$U$ to explore UO$_2$…

We analyze the symmetry changes of the paramagnetic to the A-type antiferromagnetic and to the ferromagnetic phase transitions in undoped and moderately doped LaMnO$_3$, respectively. We show that in the orthorhombic-distorted perovskite…

Strongly Correlated Electrons · Physics 2009-10-31 Fan Zhong , Z. D. Wang

We characterize perovskite TiF_3, a material which displays significant negative thermal expansion at elevated temperatures above its cubic-to-rhombohedral structural phase transition at 330 K. We find the optical response favors an…

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