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Excitation of localized surface plasmons (LSPs) of metal nanoparticles (NPs) residing on a flat metal film has attracted great attentions recently due to the enhanced electromagnetic (EM) fields found to be higher than the case of NPs on a…

Optics · Physics 2015-07-02 Anran Li , Sivan Isaacs , Ibrahim Abdulhalim , Shuzhou Li

Generation of energetic (hot) electrons is an intrinsic property of any plasmonic nanostructure under illumination. Simultaneously, a striking advantage of metal nanocrystals over semiconductors lies in their very large absorption cross…

Mesoscale and Nanoscale Physics · Physics 2017-08-31 Lucas V. Besteiro , Xiang-Tian Kong , Zhiming Wang , Gregory V. Hartland , Alexander O. Govorov

Nanostars (NSTs) are spiky nanocrystals with plasmonic hot spots. In this study, we show that strong electromagnetic fields localized in the nanostar tips are able to generate large numbers of energetic (hot) electrons, which can be used…

Mesoscale and Nanoscale Physics · Physics 2016-12-20 Xiang-Tian Kong , Zhiming Wang , Alexander O. Govorov

We theoretically study hot electron generation through the emission of a dipole source coupled to a nanoresonator on a metal surface. In our hybrid approach, we solve the time-harmonic Maxwell's equations numerically and apply a quantum…

Nanoscale gaps between adjacent metallic nanostructures give rise to extraordinarily large field enhancements, known as "hot spots", upon illumination. Incident light with the electric field polarized across the gap (along the interparticle…

Mesoscale and Nanoscale Physics · Physics 2013-03-27 Joseph B. Herzog , Mark W. Knight , Yajing Li , Kenneth M. Evans , Naomi J. Halas , Douglas Natelson

In this paper, we investigate the photothermal effects of the plasmon resonance. Metal nanoparticles efficiently generate heat in the presence of electromagnetic radiation. The process is strongly enhanced when a fixed frequency of the…

Analysis of PDEs · Mathematics 2013-12-17 Xiaoping Fang , Youjun Deng , Jing Li

We present a semiclassical model for plasmon-enhanced high-harmonic generation (HHG) in the vicinity of metal nanostructures. We show that both the inhomogeneity of the enhanced local fields and electron absorption by the metal surface play…

Optics · Physics 2015-07-29 A. Husakou , S. -J. Im , J. Herrmann

We study theoretically the photoelectron emission in noble gases using plasmonic enhanced near-fields. We demonstrate that these fields have a great potential to generate high energy electrons by direct mid-infrared laser pulses of the…

We have investigated the effects of tuning the localized surface plasmon resonances (LSPRs) of silver nanoparticles on the fluorescence intensity, lifetime, and Raman signal from nearby fluorophores. The presence of a metallic structure can…

Other Condensed Matter · Physics 2009-11-13 N. I. Cade , T. Ritman-Meer , D. Richards

The coherent oscillations of mobile charge carriers near the surface of good conductors-surface plasmons-are been exploited in many applications in information technologies, clean energy, high-density data storage, photovoltaics, chemistry,…

Mesoscale and Nanoscale Physics · Physics 2023-12-20 Jacob Khurgin , Anton Yu. Bykov , Anatoly V. Zayats

Surface plasmon enhanced processes and hot-carrier dynamics in plasmonic nanostructures are of great fundamental interest to reveal light-matter interactions at the nanoscale. Using plasmonic tunnel junctions as a platform supporting both…

In plasmonics, and particularly in plasmonic photochemistry, the effect of hot-electron generation is an exciting phenomenon driving new fundamental and applied research. However, obtaining a microscopic description of the hot-electron…

New type of plasmonic nanoparticles - silver octopods that can be synthesized with a variety of shapes - have been demonstrated to show versatile optical response using the discrete dipole approximation. The octopods show a complex behavior…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Ivan I. Naumov , Zhiyong Li , Alexander M. Bratkovsky

We present theoretical investigations of high-order harmonic generation (HHG) resulting from the interaction of noble gases with localized surface plasmons. These plasmonic fields are produced when a metal nanoparticle is subject to a…

Efficient conversion of photons to electrical energy has a wide variety of applications including imaging, energy harvesting, and infrared detection. The coupling of electromagnetic radiation to free electron oscillations at a metal…

Applied Physics · Physics 2018-02-14 Shiva Piltan , Dan Sievenpiper

We theoretically study the characteristics of photoelectron emission in plasmonic nanoparticle arrays. Nanoparticles are partially embedded in a semiconductor, forming Schottky barriers at metal/semiconductor interfaces through which…

We propose to use collective lattice resonances in plasmonic nanoparticle arrays to enhance photoelectron emission in Schottky-barrier photodetectors and solar cells. We show that the interaction of lattice resonances (the Rayleigh anomaly)…

Metal nanoparticles are attractive for plasmon-enhanced generation of hot carriers, which may be harnessed in photochemical reactions. In this work, we analyze the coherent femtosecond dynamics of photon absorption, plasmon formation, and…

Mesoscale and Nanoscale Physics · Physics 2021-01-14 Tuomas P. Rossi , Paul Erhart , Mikael Kuisma

This study found that plasmonic hotspots (HSs) between silver nanoparticles (NPs) and silver nanowires (NWs) generated two-photon excited emissions, including hyper-Rayleigh, hyper-Raman, and two-photon fluorescence of dye molecules with…

Optics · Physics 2025-07-22 Tamitake Itoh , Yuko S. Yamamoto

Experiments on the excitation of propagating surface plasmons (SPs) by ultrashort, high intensity laser interaction with "grating" targets are reviewed. At intensities exceeding $10^{19}~\mbox{W cm}^{-2}$ on target, i.e. in the strongly…

Plasma Physics · Physics 2019-05-01 A. Macchi , G. Cantono , L. Fedeli , F. Pisani , T. Ceccotti
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