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Progress in the emerging field of engineered quantum systems requires the development of devices that can act as quantum memories. The realisation of such devices by doping solid state cavities with paramagnetic ions imposes a trade-off…

Materials Science · Physics 2013-11-06 Warrick G. Farr , Daniel L. Creedon , Maxim Goryachev , Karim Benmassai , Michael E. Tobar

This investigation employed microwave whispering gallery mode (WGM) analysis to characterize the dielectric properties of a cylindrical, single-crystal sample of calcium tungstate (CaWO$_4$). Through investigation of…

Low-loss crystals with defects due to paramagnetic or rare earth impurity ions is a major area of investigation for quantum hybrid systems at both optical and microwave frequencies. In this work we examine the single crystal yttrium…

Materials Science · Physics 2017-08-02 N. C. Carvalho , M. Goryachev , J. Krupka , P. Bushev , M. E. Tobar

Properties of doped and natural impurities in Lithium Niobate single crystals are studied using the Whispering Gallery Mode method at low temperatures as a function of magnetic field. The study reveals considerable coupling of microwave…

Materials Science · Physics 2015-08-19 Maxim Goryachev , Nikita Kostylev , Michael E. Tobar

Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been introduced as a sensitive new method for electron paramagnetic resonance spectroscopy at millikelvin temperatures. Here,…

The low dielectric losses of an isotropically pure single crystal $^{28}$Si sample were determined at a temperature of 20 mK and at powers equivalent to that of a single photon. Whispering Gallery Mode (WGM) analysis revealed large Quality…

Mesoscale and Nanoscale Physics · Physics 2017-07-26 Nikita Kostylev , Maxim Goryachev , Andrey D. Bulanov , Vladimir A. Gavva , Michael E. Tobar

We report the first observation of Rabi oscillations in the spin-7/2 ensemble of trivalent gadolinium ions hosted in CaWO$_4$ single crystal. A number of transitions within the lowest electronic multiplet $^8S_{7/2}$ of Gd$^{3+}$ ion are…

Mesoscale and Nanoscale Physics · Physics 2017-02-27 E. I. Baibekov , M. R. Gafurov , D. G. Zverev , I. N. Kurkin , A. A. Rodionov , B. Z. Malkin , B. Barbara

The microwave properties of a crystalline sapphire dielectric whispering gallery mode resonator have been measured at very low excitation strength (E/hf=1) and low temperatures (T = 30 mK). The measurements were sensitive enough to observe…

The development of a new era of quantum devices requires an understanding of how paramagnetic dopants or impurity spins behave in crystal hosts. Here, we describe a new spectroscopic technique which uses traditional Electron Spin Resonance…

We report the realization of a strong coupling between a Gd$^{3+}$ spin ensemble hosted in a scheelite (CaWO$_4$) single crystal and the resonant mode of a coplanar stripline superconducting cavity leading to a large separation of…

A low-noise cryogenic microwave spectroscopy experiment was performed on a high-purity lithium fluoride (LiF) crystal. The spectroscopy data revealed avoided level crossing interactions in whispering gallery modes, indicative of electron…

Quantum Physics · Physics 2026-01-21 Steven Samuels , William Campbell , Michael E. Tobar , Maxim Goryachev

This work demonstrates strong coupling regime between an Erbium ion spin ensemble and microwave Hybrid Cavity-Whispering Gallery Modes in a Yttrium Aluminium Garnet dielectric crystal. Coupling strengths of $220$~MHz and mode quality…

Materials Science · Physics 2015-09-23 W. G. Farr , M. Goryachev , J. M. le Floch , P. Bushev , M. E. Tobar

We investigate the magnetization dynamics of $TmFeO_3$ single crystals across the spin-reorientation phase transition using broadband microwave absorption spectroscopy up to 87.5 GHz. Temperature- and magnetic-field-dependent…

The rare-earth-metal-oxide based electronic materials were produced via a conventional mixed-oxide route. Thermal analysis, XRD and SEM were used to follow phase evolution and demonstrate the phase purity. Analytical TEM were used to…

Materials Science · Physics 2023-01-31 Kouros Khamoushi

Contrary to the well known spin qubits, rare-earth qubits are characterized by a strong influence of crystal field due to large spin-orbit coupling. At low temperature and in the presence of resonance microwaves, it is the magnetic moment…

Strongly Correlated Electrons · Physics 2009-11-26 Sylvain Bertaina , J. H. Shim , S. Gambarelli , B. Z. Malkin , B. Barbara

The reflectivity of single-crystalline CoO has been studied by optical spectroscopy for wave numbers ranging from 100 to 28,000\wn and for temperatures 8 $< T <$ 325 K\@. A splitting of the cubic IR-active phonon mode on passing the…

Strongly Correlated Electrons · Physics 2009-01-20 Ch. Kant , T. Rudolf , F. Schrettle , F. Mayr , J. Deisenhofer , P. Lunkenheimer , M. V. Eremin , A. Loidl

Rare-earth doped crystals have long coherence times and the potential to provide quantum interfaces between microwave and optical photons. Such applications benefit from a high cooperativity between the spin ensemble and a microwave cavity…

Interaction of Whispering Gallery Modes (WGM) with dilute spin ensembles in solids is an interesting paradigm of Hybrid Quantum Systems potentially beneficial for Quantum Signal Processing applications. In the present work, WGM spectroscopy…

We have demonstrated electron-electron and electron-nuclear spin manipulations of Gd3+ ion in CaWO4 crystal. The results suggest that the studied system is perspective for multiqubit implementation in quantum computing.

Mesoscale and Nanoscale Physics · Physics 2018-12-03 M. R. Gafurov , G. V. Mamin , E. I. Baibekov , I. N. Kurkin , F. F. Murzakhanov , S. B. Orlinskii

The local environment of Gd3+ (4f7 S=7/2) ions in single crystals of Ca1-xGdxB6 (0.0001 < x < 0.01) is studied by means of Electron Spin Resonance (ESR). The spectra for low concentration samples (x < 0.001) show a split spectrum due to…

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