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We present a practical roadmap to achieve optical cycling and laser cooling of asymmetric top molecules (ATMs). Our theoretical analysis describes how reduced molecular symmetry, as compared to diatomic and symmetric non-linear molecules,…

Atomic Physics · Physics 2020-08-05 Benjamin L. Augenbraun , John M. Doyle , Tanya Zelevinsky , Ivan Kozyryev

Laser cycling of resonances can remove entropy from a system via spontaneously emitted photons, with electronic resonances providing the fastest cooling timescales because of their rapid relaxation rates. Although atoms are routinely laser…

A novel type of particle "cooling", called Ionization Cooling, is applicable to slow (v of the order of 0.1c) ions stored in a small ring. The many traversals through a thin foil enhance the nuclear reaction probability, in a steady…

High Energy Physics - Phenomenology · Physics 2011-05-18 C. Rubbia , A. Ferrari , Y. Kadi , V. Vlachoudis

We present the first experimental demonstration of radiation pressure force deflection and direct laser cooling for barium monohydride (BaH) molecules resulting from multiple photon scattering. Despite a small recoil velocity (2.7 mm/s) and…

We have recently demonstrated that optical pumping methods combined with photoassociation of ultra-cold atoms can produce ultra-cold and dense samples of molecules in their absolute rovibronic ground state. More generally, both the external…

Atomic Physics · Physics 2013-08-01 I. Manai , R. Horchani , M. Hamamda , A. Fioretti , M. Allegrini , H. Lignier , P. Pillet , D. Comparat

The efficiency of cavity sideband cooling of trapped molecules is theoretically investigated for the case where the IR transition between two rovibrational states is used as a cycling transition. The molecules are assumed to be trapped…

Quantum Physics · Physics 2011-11-30 Markus Kowalewski , Giovanna Morigi , Pepijn W. H. Pinkse , Regina de Vivie-Riedle

Cooling the motion of trapped ions to near the quantum ground state is crucial for many applications in quantum information processing and quantum metrology. However, certain motional modes of trapped-ion crystals can be difficult to cool…

Hybrid systems of laser-cooled trapped ions and ultracold atoms combined in a single experimental setup have recently emerged as a new platform for fundamental research in quantum physics. This paper reviews the theoretical and experimental…

Cold molecular ions are promising candidates in various fields ranging from precision spectroscopy and test of fundamental physics to ultra-cold chemistry. Control of internal and external degrees of freedom is a prerequisite for many of…

Quantum Physics · Physics 2015-05-06 Yong Wan , Florian Gebert , Fabian Wolf , Piet O. Schmidt

Molecular ions can be held in a chain of laser-cooled atomic ions by sympathetic cooling. This system is ideal for performing high-precision molecular spectroscopy with applications in astrochemistry and fundamental physics. Here we show…

Atomic Physics · Physics 2015-08-20 Ncamiso B. Khanyile , Gang Shu , Kenneth R. Brown

We study cooling of the collective vibrational motion of two 138Ba+ ions confined in an electrodynamic trap and irradiated with laser light close to the resonances S_1/2-P_1/2 (493 nm) and P_1/2-D_3/2 (650 nm). The motional state of the…

Quantum Physics · Physics 2009-11-07 D. Reiss , K. Abich , W. Neuhauser , Ch. Wunderlich , P. E. Toschek

We demonstrate the ability to load, cool and detect singly-charged calcium ions in a surface electrode trap using only visible and infrared lasers for the trapped-ion control. As opposed to the standard methods of cooling using…

Atomic Physics · Physics 2017-07-27 F. Lindenfelser , M. Marinelli , V. Negnevitsky , S. Ragg , J. P. Home

The translational motion of molecular ions can be effectively cooled sympathetically to translational temperatures below 100 mK in ion traps through Coulomb interactions with laser-cooled atomic ions. The ro-vibrational degrees of freedom,…

Atomic Physics · Physics 2009-11-10 I. S. Vogelius , L. B. Madsen , M. Drewsen

We demonstrate the mixing of rotational states in the ground electronic state using microwave radiation to enhance optical cycling in the molecule yttrium (II) monoxide (YO). This mixing technique is used in conjunction with a frequency…

The last few years have seen rapid progress in the application of laser cooling to molecules. In this review, we examine what kinds of molecules can be laser cooled, how to design a suitable cooling scheme, and how the cooling can be…

Atomic Physics · Physics 2021-12-14 N. J. Fitch , M. R. Tarbutt

The two most widely used ion cooling methods are laser cooling and sympathetic cooling by elastic collisions (ECs). Here we demonstrate another method of cooling ions that is based on resonant charge exchange (RCE) between the trapped ion…

Atomic Physics · Physics 2018-04-11 Sourav Dutta , S. A. Rangwala

Sympathetic cooling of trapped ions has been established as a powerful technique for manipulation of non-laser-coolable ions (Raizen1992,Waki1992,Bowe1999,Barrett2003). For molecular ions, it promises vastly enhanced spectroscopic…

Quantum Physics · Physics 2018-06-06 Soroosh Alighanbari , Michael Georg Hansen , Vladimir Korobov , Stephan Schiller

We are proposing to test experimentally the new idea of Enhanced Optical Cooling (EOC) in an electron storage ring. This experiment will confirm new fundamental processes in beam physics and will demonstrate new unique possibilities with…

Accelerator Physics · Physics 2008-11-26 E. G. Bessonov , M. V. Gorbunkov , A. A. Mikhailichenko

We present a laser cooling scheme for trapped ions and atoms using a combination of laser couplings and a magnetic gradient field. In a Schrieffer-Wolff transformed picture, this setup cancels the carrier and blue sideband terms completely…

Quantum Physics · Physics 2011-03-18 Andreas Albrecht , Alex Retzker , Christof Wunderlich , Martin B. Plenio

A laser cooling scheme for trapped ions is presented which is based on the fast dynamical Stark shift gate, described in [Jonathan etal, PRA 62, 042307]. Since this cooling method does not contain an off resonant carrier transition, low…

Quantum Physics · Physics 2009-11-13 A. Retzker , M. B. Plenio