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The lack of suitable vacuum ultraviolet (VUV) nonlinear optical (NLO) crystals has hindered the development of compact, high-power VUV sources via second harmonic generation (SHG). Here, we report on the development of the fluorooxoborate…

Following our ab initio nonlinear optical (NLO) materials design guidelines, in this Letter, we discovered a novel type of structure to realize potential deep-ultraviolet (DUV) NLO performance in the classical beryllium borate system. By…

Materials Science · Physics 2021-05-24 Lei Kang , Pifu Gong , Zheshuai Lin , Bing Huang

The structural symmetry of solids plays an important role in defining their linear and nonlinear optical properties. The quest for versatile, cost-effective, large-scale, and defect-free approaches and materials platforms for tailoring…

In modern optics, materials with large birefringence ({\Delta}n, where n is the refractive index) are sought after for polarization control (e.g. in wave plates, polarizing beam splitters, etc.), nonlinear optics and quantum optics (e.g.…

Lithium Niobate (LiNbO$_3$) is a piezoelectric crystal with a high electromechanical coupling coefficient. The development and miniaturization of acousto-electronics, and acousto-optics modulation filters, are primarily based on surface…

Applied Physics · Physics 2022-08-09 Varun Bhardwaj , Kaushik Shukla , Frank Melandsø , Anowarul Habib

Optical anisotropy is a fundamental attribute of some crystalline materials and is quantified via birefringence. A birefringent crystal not only gives rise to asymmetrical light propagation but also attenuation along two distinct…

Materials that exhibit high nonlinear optical (NLO) susceptibilities are considered as promising candidates for a wide range of photonic and electronic applications. Here we argue that the ferroelectric nematic (NF) materials have…

Soft Condensed Matter · Physics 2022-03-22 C. L. Folcia , J. Ortega , R. Vidal , T. Sierra , J. Etxebarria

Epsilon-near-zero materials are exceptional candidates for studying electrodynamics and nonlinear optical processes at the nanoscale. We demonstrate that by alternating a metal and a highly doped conducting-oxide, the epsilon-near-zero…

Tailoring the degrees of freedom (DoF) of light for a desired purpose, so-called structured light, has delivered numerous advances over the past decade, ranging from communications and quantum cryptography to optical trapping, and…

Optics · Physics 2025-01-31 Sachleen Singh , Isaac Nape , Andrew Forbes

The miniaturization of diagnostic devices that exploit optical detection schemes requires the design of light-sources combining small size, high performance for effective excitation of chromophores, and mechanical flexibility for easy…

Colossal optical anisotropy in the entire visible spectrum is crucial for advanced photonic applications, enabling precise light manipulation without optical loss across a broad spectral range. Here, we demonstrate that CuAlO2 exhibits…

Laser stimulated second and third harmonic generation effects in Fluorine doped tin oxide (F:SnO2) nanostructures versus the fluorine content is presented. The F:SnO2 nanostructures have been fabricated at various fluorine doping…

Nonlinear optical generation from a crystalline material can reveal the symmetries of both its lattice structure and underlying ordered electronic phases and can therefore be exploited as a complementary technique to diffraction based…

Strongly Correlated Electrons · Physics 2014-11-04 D. H. Torchinsky , H. Chu , T. Qi , G. Cao , D. Hsieh

Organic-inorganic hybrids may offer material properties not available from their inorganic components. However, they are typically less stable and disordered. Long-term stability study of the hybrid materials, over the anticipated lifespan…

The rapid development of metasurfaces - 2D ensembles of engineered nanostructures - is presently fostering a steady drive towards the miniaturization of many optical functionalities and devices to a subwavelength size. The material…

A binary mixture of ferroelectric liquid crystals (FLCs) was used for the design of a channel waveguide. The FLCs possess two important functionalities: a chromophore with a high hyperpolarizability $\beta$ and photoreactive groups. The…

Soft Condensed Matter · Physics 2009-10-31 Valentina S. U. Fazio , S. T. Lagerwall , V. Zauls , S. Schrader , P. Busson , A. Hult , H. Motschmann

The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…

Materials Science · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , S. W. Wu , Chunlei Guo

The optical properties of two-dimensional materials are exceptional in several respects. They are highly anisotropic and frequently dominated by excitonic effects. Dipole-allowed second order non-linear optical properties require broken…

Mesoscale and Nanoscale Physics · Physics 2023-07-05 M. F. C. Martins Quintela , T. Garm Pedersen

Organic exciton-photon polariton lasers have recently been shown to be remarkable candidates for the realization of efficient sources of coherent light operating at room temperature. While their thresholds are now comparable with…

Optics · Physics 2022-02-22 F. Le Roux , A. Mischok , D. D. C. Bradley , M. C. Gather

Clarifying the contribution of various atoms and structural units formed in nonlinear optical (NLO) crystal materials to macroscopic optical response is crucial for NLO crystal design. In this work, the rigorous atomic space tessellating…

Optics · Physics 2024-10-08 Yang Chi
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