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We study the role of the electrical double layer (EDL) in the formation of the quasistatic electrical conductivity of suspensions of nanosized particles. A suspension is viewed as a system of hard-core--penetrable-shell particles. The…

Soft Condensed Matter · Physics 2024-01-15 M. Ya. Sushko , S. D. Balika

The classical Poisson-Boltzmann (PB) theory of electrolytes assumes a dilute solution of point charges with mean-field electrostatic forces. Even for very dilute solutions, however, it predicts absurdly large ion concentrations (exceeding…

Chemical Physics · Physics 2007-05-23 Mustafa Sabri Kilic , Martin Z. Bazant , Armand Ajdari

An active electrical network contains a voltage or current source that creates electromagnetic energy through a method of transduction that enables the separation of opposite polarity charges from an external source. The end result is the…

Classical Physics · Physics 2022-10-06 Michael E. Tobar , Raymond Y. Chiao , Maxim Goryachev

We report the experimental determination of the structure and response to applied electric field of the lower-temperature nematic phase of the previously reported calamitic compound 4-[(4-nitrophenoxy)carbonyl]phenyl2,4-dimethoxybenzoate…

We derive an expression for the static dielectric constant of the colloidal susp ensions based on the electrokinetic equations. The analysis assumes that the ions have the same diffusivity, and that the double layer is much thinner than the…

Soft Condensed Matter · Physics 2009-11-07 C. -Y. D. Lu

The electric double layer (EDL) formed around charged nanostructures at the liquid-solid interface determines their electrochemical activity and influences their electrical and optical polarizability. We experimentally demonstrate that…

Soft Condensed Matter · Physics 2020-04-29 Kevin Namink , Xuanhui Meng , Marc T. M. Koper , Philipp Kukura , Sanli Faez

We analyze the simplest problem of electrochemical relaxation in more than one dimension - the response of an uncharged, ideally polarizable metallic sphere (or cylinder) in a symmetric, binary electrolyte to a uniform electric field. In…

Materials Science · Physics 2009-11-11 Kevin T. Chu , Martin Z. Bazant

Charge transport in QD solids is typically understood as thermally activated tunneling or hopping between states that are localized on individual QDs. Here, we show that the slow relaxation that is associated with the disorder-broadened…

Disordered Systems and Neural Networks · Physics 2025-11-19 Morteza Shokrani , Xinlu Wu , Ebbo Krahmer , Martijn Kemerink

A solid ionic conductor with cation conductivity in the interelectrode region is studied. Due to their large size, the anions are considered fixed and form a homogeneous neutralizing electric background. The model can be used to describe…

Statistical Mechanics · Physics 2022-07-04 I. Kravtsiv , G. Bokun , M. Holovko , N. Prokopchuk , D. di Caprio

We study the electric double layer near a charged soft surface by using a mean-field approach including non-uniform size effect and solvent polarization. Based on a free energy model, electrostatic potential and number densities of water…

Soft Condensed Matter · Physics 2022-02-10 Jun-Sik Sin , Nam-Hyok Kim , Chung-Sik Sin

We develop a theory of drag in graphene double layers near charge neutrality. We work in the regime of electron hydrodynamics and account for interlayer correlations of charge puddle disorder. The drag resistivity is expressed in terms of…

Mesoscale and Nanoscale Physics · Physics 2025-11-04 Dmitry Zverevich , Alex Levchenko , A. V. Andreev

The device of electric double-layer transistor (EDLT) with ionic liquid has been employed as an effective way to dope carriers over a wide range, which can induce metallic state, magnetic reconstruction and superconducting transition.…

Superconductivity · Physics 2018-08-30 Shuai Zhang , Moran Gao , Huanyan Fu , Xinmin Wang , Zhian Ren , Genfu Chen

In the recent experiments [Chmiola et al, Science 313, 1760 (2006); Largeot et al, J. Am. Chem. Soc. 130, 2730 (2008)] an anomalous increase of the capacitance with a decrease of the pore size of a carbon-based porous electric double-layer…

Soft Condensed Matter · Physics 2015-03-17 S. Kondrat , A. Kornyshev

The nanoscopic mass and charge distribution within the double layer at electrified interfaces plays a key role in electrochemical phenomena of huge technological relevance for energy production and conversion. However, in spite of its…

Chemical Physics · Physics 2019-05-29 Remi Khatib , Ashwinee Kumar , Stefano Sanvito , Marialore Sulpizi , Clotilde S. Cucinotta

Electrophoresis is a motion of charged dispersed particles relative to a fluid in a uniform electric field. The effect is widely used to separate macromolecules, to assemble colloidal structures, to transport particles in nano- and…

Soft Condensed Matter · Physics 2011-01-21 Oleg D. Lavrentovich , Israel Lazo , Oleg P. Pishnyak

This work presents a scalable method to produce robust all-solid electric double layer capacitors (EDLCs), compatible with roll-to-roll processes and structural laminate composite fabrication. It consists in sandwiching and pressing an…

The role of the discontinuity of the exchange-correlation potential of density functional theory is studied in the context of electron transport and shown to be intimately related to Coulomb blockade. By following the time evolution of an…

Mesoscale and Nanoscale Physics · Physics 2010-06-08 S. Kurth , G. Stefanucci , E. Khosravi , C. Verdozzi , E. K. U. Gross

The contact value theorem was originally derived for Coulomb fluids of mobile charged particles in thermal equilibrium, in the presence of interfaces carrying a {\em uniform} surface charge density and in the absence of dielectric…

Statistical Mechanics · Physics 2025-03-03 Ladislav Šamaj

The functionalities and applications of complex coacervates -- liquid condensates resulting from liquid-liquid phase separation of charged polymers -- are significantly influenced by the dispersion and aggregation states of guest…

Soft Condensed Matter · Physics 2025-08-05 Zongpei Wu , Shensheng Chen

Slide electrification is a spontaneous charge separation between a surface and a sliding drop. Here, we describe this effect in terms of a voltage generated at the three-phase contact line. This voltage moves charges between capacitors, one…

Soft Condensed Matter · Physics 2024-02-27 Pravash Bista , Amy Z. Stetten , William S. Y Wong , Hans-Jürgen Butt , Stefan A. L. Weber