Related papers: Ultrafast Field-Resolved Nonlinear Optical Spectro…
A novel polarization-modulation transient method has been developed for studying fast anisotropic relaxation in electronic excited states of polyatomic and biologically relevant molecules under excitation with femtosecond laser pulses. The…
Measuring the dispersion of photonic devices with small dispersion-length products is challenging due to the phase-sensitive, and alignment-intensive nature of conventional methods. In this letter, we demonstrate a quantum technique to…
We present a computational study of the pump-probe response of a single atom to assess any microscopic nonlinear optical anisotropy due to freed electrons for non-resonant optical excitation. Using simulations of the Schr\"odinger equation…
A finite element method simulation of a carbon fibre reinforced polymer block is used to analyse the nonlinearities arising from a contacting delamination gap inside the material. The ultrasonic signal is amplified and nonlinearities are…
We have investigated strong-field-induced electronic coherences in argon and molecular nitrogen ions created by high-intensity, few-cycle infrared laser pulses. This is a step toward the long-sought goal of strong-field coherent control in…
Although high field laser-induced ionization is a fundamental process underlying many applications, there have been no absolute measurements of the nonlinear polarizability of atoms and molecules in the presence of ionization. Such…
Based on Document (1), by considering the retarded interaction of radiation fields, the third order transition probabilities of stimulated radiations and absorptions of light are calculated. The revised formulas of nonlinear polarizations…
We studied the ultrafast third-order optical nonlinearity in a single crystal of multiferroic bismuth ferrite (BiFeO3) in the near-infrared range of 0.5-1.0 eV, where the material is fundamentally transparent,at room temperature. With pump…
Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{\AA}ngstr\"om spatial and femtosecond temporal resolution. Here, we provide the…
Optical phase measurements play a key role in the detection of macroscopic parameters such as position, velocity, and displacement. They also permit to qualify the microscopic properties of photonic waveguides such as polarization mode…
Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…
We discuss a novel application of matter wave interferometry to characterize the scalar optical polarizability of molecules at 532 nm. The interferometer presented here consists of two material absorptive gratings and one central optical…
We report the direct observation of the non-reciprocity of the velocity of light, induced in a gas by electric and magnetic fields. This bilinear magneto-electro-optical phenomenon appears in the presence of crossed electric and magnetic…
Knowledge of molecular structure is paramount in understanding, and ultimately influencing, chemical reactivity. For nearly a century, diffractive imaging has been used to identify the structures of many biologically-relevant gas-phase…
By measuring the polarization changes in THz, infrared, and visible radiation over an extended energy range (3-2330 meV), we observe symmetry-breaking in cuprate high temperature superconductors over wide energy, doping, and temperature…
Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution…
We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…
We present ultra-fast quantum chemical methods for the calculation of infrared and ultraviolet-visible spectra designed to provide fingerprint information during autonomous and interactive explorations of molecular structures.…
We present a method for a complete characterization of a femtosecond ultraviolet pulse when a fundamental near-infrared beam is also available. Our approach relies on generation of second harmonic from the pre-characterized fundamental,…
The electronic wavefunction is at the heart of physical phenomena, defining the frontiers of quantum materials research. While the amplitude of the electron wavefunction in crystals can be measured with state-of-the-art probes in…