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We present a robust but still efficient simulation approach for high-resolution scanning tunneling microscopy with a flexible tip apex showing sharp submolecular features. The approach takes into account the electronic structure of sample…

Mesoscale and Nanoscale Physics · Physics 2017-01-11 O. Krejci , P. Hapala , M. Ondracek , P. Jelinek

Here, we introduce and experimentally demonstrate optical amplification and stimulated emission from a single optically pumped molecular tunneling junction of a scanning tunneling microscope. The gap between a sharp gold tip and a flat gold…

Optics · Physics 2014-01-09 K. Braun , A. M. Kern , X. Wang , H. Adler , H. Peisert , T. Chasse , D. Zhang , A. J. Meixner

A Scanning Tunneling Microscope (STM) is one of the most important scanning probe tools available to study and manipulate matter at the nanoscale. In a STM, a tip is scanned on top of a surface with a separation of a few \AA. Often, the…

A molecular wire containing an emitting molecular center is controllably suspended between the plasmonic electrodes of a cryogenic scanning tunneling microscope. Passing current through this circuit generates an ultra narrow-line emission…

Mesoscale and Nanoscale Physics · Physics 2016-01-27 Michael C. Chong , Gaël Reecht , Hervé Bulou , Alex Boeglin , Fabrice Scheurer , Fabrice Mathevet , Guillame Schull

We explore theoretically the scanning tunneling microscopy of single molecules on substrates using a framework of two local probes. This framework is appropriate for studying electron flow in tip/molecule/substrate systems where a thin…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 John Buker , George Kirczenow

A gated probe for scanning tunnelling microscopy (STM) has been developed. The probe extends normal STM operations by means of an additional electrode fabricated next to the tunnelling tip. The extra electrode does not make contact with the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 L. Gurevich , L. Canali , L. P. Kouwenhoven

The junction of a scanning tunneling microscope (STM) operating in the tunneling regime was irradiated with femtosecond laser pulses. A photo-excited hot electron in the STM tip resonantly tunnels into an excited state of a single molecule…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Shiwei Wu , Wilson Ho

We study the light emission from a Ag(111) surface when the bias voltage on a scanning tunneling microscope (STM) junction is ramped into the field emission regime. Above the vacuum level, scanning tunneling spectroscopy (STS) shows a…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Jesús Martínez-Blanco , Stefan Fölsch

We present a probe-type scanning tunneling microscope (STM) with atomic resolution that is designed to be directly inserted and work in a harsh vibrational cryogen-free superconducting magnet system. When a commercial variable temperature…

Instrumentation and Detectors · Physics 2018-06-01 Wenjie Meng , Jihao Wang , Yubin Hou , Mengqiao Sui , Junting Wang , Gang Wu , Junyun Li , Qingyou Lu

The scanning-tunneling-microscope-induced luminescence emerges recently as an incisive tool to measure the molecular properties down to the single-molecule level. The rapid experimental progress is far ahead of the theoretical effort to…

Mesoscale and Nanoscale Physics · Physics 2020-11-24 Guohui Dong , Yining You , Hui Dong

Using the highly localized current of electrons tunneling through a double barrier Scanning Tunneling Microscope (STM) junction, we excite luminescence from a selected C$_{60}$ molecule in the surface layer of fullerene nanocrystals grown…

A microscopic theory of the transport in a scanning tunnelling microscope (STM) set-up is introduced for \pi-conjugated molecules on insulating films, based on the density matrix formalism. A key role is played in the theory by the energy…

Mesoscale and Nanoscale Physics · Physics 2012-05-23 Sandra Sobczyk , Andrea Donarini , Milena Grifoni

Scanning probe microscopy (SPM) images of regularly arranged spatially periodic objects can be processed crystallographically. The resulting information may be used to remove from the SPM image distortions that are due to a less than…

Materials Science · Physics 2020-12-16 Peter Moeck

We consider to detect the electron spin of a doped atom, i.e., a nitrogen or a phosphorus, caged in a fullerene by currently available technique of the scanning tunneling microscope (STM), which actually corresponds to the readout of a…

Quantum Physics · Physics 2009-11-13 M. Feng , G. J. Dong , B. Hu

We use fluorescent nanospheres as scalar detectors for the electric-field intensity in order to probe the near-field of an optical tip used in aperture-type near-field scanning optical microscopy (NSOM). Surprisingly, the recorded…

Optics · Physics 2007-05-23 A. Drezet , M. J. Nasse , S. Huant , J. C. Woehl

We propose a mechanism to use scanning tunneling microscopy (STM) for direct measurements of the two-electron singlet-triplet exchange splitting $J$ in diatomic molecular systems, unsing the coupling between the molecule and the substrate…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. Fransson , A. V. Balatsky

We report the construction and performance of a low temperature, high field scanning tunneling microscope (STM) operating down to 350mK and in magnetic fields up to 9T, with thin film deposition and in-situ cleaving capabilities. The main…

Vortices play a crucial role in determining the properties of superconductors as well as their applications. Therefore, characterization and manipulation of vortices, especially at the single vortex level, is of great importance. Among many…

A scanning tunneling microscope (STM) with a magnetic tip that has a sufficiently strong spin-polarization can be used to map the sample's spin structure down to the atomic scale but usually lacks the possibility to absolutely determine the…

Superconductivity · Physics 2021-04-26 Lucas Schneider , Philip Beck , Jens Wiebe , Roland Wiesendanger

Scanning tunneling microscope (STM) is a powerful tool for studying the structural and electronic properties of materials at the atomic scale. The combination of low temperature and high magnetic field for STM and related spectroscopy…

Materials Science · Physics 2018-11-13 Syu-You Guan , Hsien-Shun Liao , Bo-Jing Juang , Shu-Cheng Chin , Tien-Ming Chuang , Chia-Seng Chang