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We present coincidence measurements of two-photon double-ionization (TPDI) of argon driven by femtosecond pulses tunable around 26.5 eV photon energy, which are obtained from a high-harmonic generation source. The measured photoelectron…

Enantioselective photochemistry provides access to unique molecular structures and functions, with deep implications for fundamental science and industrial applications. Current methods for highly enantioselective photochemistry critically…

Chemical Physics · Physics 2025-03-07 Andrés Ordóñez , Patricia Vindel-Zandbergen , David Ayuso

Light-induced states are commonly observed in the photoionization spectra of laser-dressed atoms. The properties of autoionizing polaritons, entangled states of light and Auger resonances, however, are largely unexplored. We employ…

Atomic Physics · Physics 2021-07-14 Nathan Harkema , Coleman Cariker , Eva Lindroth , Luca Argenti , Arvinder Sandhu

We derive here a new highly selective photoelectron-based chirality-sensing technique that utilizes 'locally-chiral' laser pulses. We show that this approach results in strong chiral discrimination, where the standard forwards/backwards…

Chemical Physics · Physics 2021-07-14 Ofer Neufeld , Hannes Hübener , Angel Rubio , Umberto De Giovannini

Exciting electrons in solids with intense light pulses offers the possibility of generating new states of matter through nonthermal means and controlling their macroscopic properties on femto- to picosecond timescales. One way to manipulate…

Materials Science · Physics 2021-10-07 Alfred Zong , Anshul Kogar , Nuh Gedik

With the recently introduced particle interpretation of the double-slit experiment for light fields [Phys. Rev. Lett. 134, 13360 (2025)], all related interference phenomena can be reinterpreted in terms of light particle states that either…

We present a theoretical analysis of high-order harmonic generation from ion-atom collisions in the presence of linearly polarized intense laser pulses. Photons with frequencies significantly higher than in standard atomic high-harmonic…

Atomic Physics · Physics 2009-11-10 Manfred Lein , Jan M. Rost

We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…

Quantum Physics · Physics 2015-05-18 Kamal P Singh , Jan M Rost

It has been long recognized that the spatial polarization of the electronic clouds in molecules, and the spatial arrangements of atoms into chiral molecular structures, play crucial roles in physics, chemistry and biology. However, these…

Optics · Physics 2020-04-14 David Ayuso , Andres Ordonez , Piero Decleva , Misha Ivanov , Olga Smirnova

We experimentally demonstrate spatiotemporal steering of photoelectron emission in multiphoton above-threshold single ionization of atoms exposed to a phase-controlled orthogonally polarized two-color (OTC) laser pulse. Spatial and energy…

We analyse recently measured nonlinear photoemission spectra from Ag surfaces that reveal resonances whose energies do not scale with the applied photon energy but stay pinned to multiples of bulk plasmon energy $\hbar\omega_p$ above the…

Materials Science · Physics 2021-05-05 Dino Novko , Vito Despoja , Marcel Reutzel , Andi Li , Hrvoje Petek , Branko Gumhalter

The interaction of two laser pulses in an underdense plasma has proven to be able to inject electrons in plasma waves, thus providing a stable and tunable source of electrons. Whereas previous works focused on the "beatwave" injection…

Plasma Physics · Physics 2009-02-12 C. Rechatin , J. Faure , A. Lifschitz , X. Davoine , E. Lefebvre , V. Malka

Strong-field phenomena driven by an intense infrared (IR) laser depend on during what part of the field cycle they are initiated. By changing the sub-cycle character of the laser electric field it is possible to control such phenomena. For…

Partial polarization is the manifestation of the correlation between two mutually orthogonal transverse field components associated with a light beam. We show both theoretically and experimentally that the origin of this correlation can be…

The polarization of light is utilized in many technologies throughout science and engineering. The ability to transform one state of polarization to another is a key enabling technology. Common polarization transformers are simple…

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

Quantum Physics · Physics 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

Twisted light (TL), a special kind of light carrying orbital angular momentum, provides a powerful tool for driving symmetry resolved transitions in quantum confined nanostructures. We study a realistic model where a TL pulse excites two…

Mesoscale and Nanoscale Physics · Physics 2025-09-10 F. J. Rodríguez , L. Quiroga , N. F. Johnson

Measurements and calculations of the absolute carrier-envelope phase (CEP) effects in the photodissociation of the simplest molecule, H2+, with a 4.5-fs Ti:Sapphire laser pulse at intensities up to (4 +- 2)x10^14 Watt/cm^2 are presented.…

Chemical Physics · Physics 2013-09-23 T. Rathje , A. M. Sayler , S. Zeng , P. Wustelt , H. Figger , B. D. Esry , G. G. Paulus

Tunneling ionization of an atom in ultrashort laser pulses is considered. When the driving laser pulse is switched-on and -off with a steep slope, the photoelectron momentum distribution (PMD) shows an edge-effect because of the…

Atomic Physics · Physics 2022-07-07 M. Klaiber , Q. Z. Lv , K. Z. Hatsagortsyan , C. H. Keitel

Molecular polaritons are the optical excitations which emerge when molecular transitions interact strongly with confined electromagnetic fields. Increasing interest in the hybrid molecular-photonic materials that host these excitations…

Mesoscale and Nanoscale Physics · Physics 2018-02-26 Raphael F. Ribeiro , Luis A. Martínez-Martínez , Matthew Du , Jorge Campos-Gonzalez-Angulo , Joel Yuen-Zhou