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We present high-resolution optically detected magnetic resonance (ODMR) spectroscopy on single nitrogen-vacancy (NV) center spins in diamond at and around zero magnetic field. The experimentally observed transitions depend sensitively on…

Mesoscale and Nanoscale Physics · Physics 2019-11-22 Johannes Kölbl , Mark Kasperczyk , Beat Bürgler , Arne Barfuss , Patrick Maletinsky

Optically detected magnetic resonance (ODMR) is an efficient and reliable method that enables initialization and readout of spin states through spin-photon interface. In general, high quantum efficiency and large spin-dependent…

Materials Science · Physics 2024-10-10 Kejun Li , Vsevolod D. Dergachev , Ilya D. Dergachev , Shimin Zhang , Sergey A. Varganov , Yuan Ping

The nitrogen-vacancy (NV) center has enabled widespread study of nanoscale nuclear magnetic resonance (NMR) spectroscopy at low magnetic fields. NMR spectroscopy at high magnetic fields significantly improves the technique's spectral…

Mesoscale and Nanoscale Physics · Physics 2021-09-15 Benjamin Fortman , Laura Mugica-Sanchez , Noah Tischler , Cooper Selco , Yuxiao Hang , Karoly Holczer , Susumu Takahashi

Enrichment of nuclear spin isomers of molecules by infrared radiation resonant to molecular rovibrational transition is considered. Special attention is given to the enrichment by light-induced crossing of far separated ortho and para…

Chemical Physics · Physics 2007-05-23 Pavel Chapovsky

Magnetic resonance detection is one of the most important tools used in life-sciences today. However, as the technique detects the magnetization of large ensembles of spins it is fundamentally limited in spatial resolution to mesoscopic…

The nitrogen-vacancy (NV) center in diamond is a leading solid-state platform for room-temperature quantum magnetometry owing to its long spin coherence times, optical spin initialization and readout, and high sensitivity to magnetic,…

Quantum Physics · Physics 2026-01-21 Satyam Pandey , Abhimanyu Magapu , Prabhat Anand , Ankit Khandelwal , M. Girish Chandra

A controlled qubit in a rotating frame opens new opportunities to probe fundamental quantum physics, such as geometric phases in physically rotating frames, and can potentially enhance detection of magnetic fields. Realising a single qubit…

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform…

Temperature sensing with nitrogen vacancy (NV) centers using quantum techniques is very promising and further development is expected. Recently, the optically detected magnetic resonance (ODMR) spectrum of a high-density ensemble of the NV…

Machine learning is a powerful tool in finding hidden data patterns for quantum information processing. Here, we introduce this method into the optical readout of electron-spin states in diamond via single-photon collection and demonstrate…

Quantum Physics · Physics 2021-03-17 Peng Qian , Xue Lin , Feifei Zhou , Runchuan Ye , Yunlan Ji , Bing Chen , Guangjun Xie , Nanyang Xu

Nitrogen-vacancy (NV) centers in diamond are extensively utilized as quantum sensors for imaging fields at the nanoscale. The ultra-high sensitivity of NV magnetometers has enabled the detection and spectroscopy of individual electron…

Nitrogen-vacancy (NV) magnetometry is a new technique for imaging spin waves in magnetic materials. It detects spin waves by their microwave magnetic stray fields, which decay evanescently on the scale of the spin-wavelength. Here, we use…

Mesoscale and Nanoscale Physics · Physics 2022-12-08 Brecht G. Simon , Samer Kurdi , Joris J. Carmiggelt , Michael Borst , Allard Katan , Toeno van der Sar

Measuring spins is the corner stone of a variety of analytical techniques including modern magnetic resonance imaging (MRI). The full potential of spin imaging and sensing across length scales is hindered by the achievable signal-to-noise…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 S. Steinert , F. Ziem , L. Hall , A. Zappe , M. Schweikert , A. Aird , G. Balasubramanian , L. Hollenberg , J. Wrachtrup

We consider an electronic spin, such as a nitrogen-vacancy (NV) center in diamond, weakly coupled to a large number (bath) of nuclear spins, and subjected to the Rabi driving with a periodically alternating phase (multiple rotary echo). We…

Mesoscale and Nanoscale Physics · Physics 2015-03-25 V. V. Mkhitaryan , F. Jelezko , V. V. Dobrovitski

The ability to control and manipulate spins via electrical, magnetic and optical means has generated numerous applications in metrology and quantum information science in recent years. A promising alternative method for spin manipulation is…

Mesoscale and Nanoscale Physics · Physics 2013-04-04 Sungkun Hong , Michael S. Grinolds , Patrick Maletinsky , Ronald L. Walsworth , Mikhail D. Lukin , Amir Yacoby

The Nitrogen-Vacancy (NV) defect in diamond is a unique quantum system that offers precision sensing of nanoscale physical quantities beyond the current state-of-the-art. Here we present a method to controllably encode the interactions in…

The nitrogen-vacancy (NV) color center in diamond has demonstrated great promise in a wide range of quantum sensing. Recently, there have been a series of proposals and experiments using NV centers to detect spin noise of quantum materials…

Mesoscale and Nanoscale Physics · Physics 2023-04-14 Jacob Henshaw , Pauli Kehayias , Luca Basso , Michael Jaris , Rong Cong , Michael Titze , Tzu-Ming Lu , Michael P. Lilly , Andrew M. Mounce

Quantum defects in solids have emerged as a transformative platform for advancing quantum technologies. A key requirement for these applications is achieving high-fidelity single-spin readout, particularly at room temperature for quantum…

We present a protocol that detects molecular conformational changes with two nitroxide electron-spin labels and a nitrogen-vacancy (NV) center in diamond. More specifically, we demonstrate that the NV can detect energy shifts induced by the…

Quantum Physics · Physics 2022-12-21 C. Munuera-Javaloy , R. Puebla , B. D'Anjou , M. B. Plenio , J. Casanova

Quantum sensing based on nitrogen-vacancy (NV) centers in diamond has been developed as a powerful tool for microscopic magnetic resonance. However, the reported sensor-to-sample distance is limited within tens of nanometers because the…