Related papers: Two-dimensional coherent spectrum of high-spin mod…
Spectroscopy underpins modern scientific discovery across diverse disciplines. While experimental spectroscopy probes material properties through scattering or radiation measurements, computational spectroscopy combines theoretical models…
Multidimensional coherent spectroscopy (MDCS) has been established in quantum chemistry as a powerful tool for studying the nonlinear response and nonequilibrium dynamics of molecular systems. More recently, the technique has also been…
Energy spectroscopy is a powerful tool with diverse applications across various disciplines. The advent of programmable digital quantum simulators opens new possibilities for conducting spectroscopy on various models using a single device.…
Spin coherent states play a crucial role in defining QESM (quasi-exactly solvable models) establishing a strict correspondence between energy spectra of spin systems and low-lying quantum states for a particle moving in a potential field of…
Nuclear spins are highly coherent quantum objects. In large ensembles, their control and detection via magnetic resonance is widely exploited, e.g. in chemistry, medicine, materials science and mining. Nuclear spins also featured in early…
This work is a sequel to our work "The Spin Density Matrix I: General Theory and Exact Master Equations" (eprint arXiv:0708.0644 [cond-mat]). Here we compare pure- and pseudo-spin dynamics using as an example a system of two quantum dots, a…
We present a widefield two-dimensional electronic spectroscopy microscope (2DESM) that integrates multidimensional coherent spectroscopy with optical imaging, enabling femtosecond temporal and micrometer spatial resolution. The broadband…
We study a model of a quantum spin register interacting with an environment of spin particles in quantum-measurement limit. In the limit of collective decoherence we obtain the form of state vectors that constitute high-dimensional…
Simulating the unitary dynamics of a quantum system is a fundamental problem of quantum mechanics, in which quantum computers are believed to have significant advantage over their classical counterparts. One prominent such instance is the…
A central challenge in quantum computing is to identify more computational problems for which utilization of quantum resources can offer significant speedup. Here, we propose a hybrid quantum-classical scheme to tackle the quantum optimal…
Two-dimensional coherent spectroscopy (2DCS) provides insights into the nonlinear response of correlated lattice systems. We simulate multipulse excitations in the Hubbard model using nonequilibrium dynamical mean-field theory to extract…
We consider here the problem of a "central spin", with spin quantum number $S \gg 1$, interacting with a set of microscopic spins. Interactions between the microscopic spins are ignored. This model describes magnetic grains or magnetic…
In this paper, we report on a correctly scaling novel coupled cluster singles and doubles (CCSD) implementation for arbitrary high-spin open-shell states. The chosen cluster operator is completely spin-free, i.e. employs spatial…
We show that higher-dimensional versions of qubits, or qudits, can be encoded into spin systems and into harmonic oscillators, yielding important advantages for quantum computation. Whereas qubit-based quantum computation is adequate for…
Control over spin dynamics has been obtained in NMR via coherent averaging, which is implemented through a sequence of RF pulses, and via quantum codes which can protect against incoherent evolution. Here, we discuss the design and…
Interacting spin systems in solids underpin a wide range of quantum technologies, from quantum sensors and single-photon sources to spin-defect-based quantum registers and processors. We develop a quantum-computer-aided framework for…
Extending the coherence lifetime of a qubit is central to the implementation and deployment of quantum technologies, particularly in the solid-state where various noise sources intrinsic to the material host play a limiting role. Here, we…
We present a comprehensive comparison of spin and energy dynamics in quantum and classical spin models on different geometries, ranging from one-dimensional chains, over quasi-one-dimensional ladders, to two-dimensional square lattices.…
The coherent dynamics and control of spin qubits are essential requirements for quantum technology. A prominent challenge for coherent control of a spin qubit in a set of qubits is the destructive effect of the applied magnetic field on the…
The quantum-to-classical correspondence (QCC) in spin models is a puzzling phenomenon where the static susceptibility of a quantum system agrees with its classical-system counterpart, at a different corresponding temperature, within the…